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Magnetic excitations in the quasi-one-dimensional quantum antiferromagnets PbNi2V2O8 and SrNi2V2O8 are measured all the way up to the zone boundary energy using inelastic neutron scattering from powder samples. An estimate for…

Strongly Correlated Electrons · Physics 2009-11-07 A. Zheludev , T. Masuda , K. Uchinokura , S. E. Nagler

Magnetic susceptibility, high-field magnetization and inelastic neutron scattering experiments are used to study the magnetic properties of a new S=1 quasi-1-dimensional antiferromagnet PbNi2V2O8. Inter-chain interactions are shown to be…

Strongly Correlated Electrons · Physics 2009-10-31 Y. Uchiyama , Y. Sasago , I. Tsukada , K. Uchinokura , A. Zheludev , T. Hayashi , N. Miura , P. Böni

$R_2BaNiO_5$ ($R=$ rare earth) quasi-1-D antiferromagnets are structurally equivalent to the well-studied 1-D S=1 Haldane-gap compound Y_2BaNiO_5. Unlike the Y-nickelate though, these materials undergo 3-D magnetic ordering at finite…

Condensed Matter · Physics 2016-03-23 A. Zheludev

Inelastic neutron scattering experiments on the S=1 quasi-one-dimensional bond-alternating antiferromagnet Ni(C9D24N4)(NO2)ClO4 have been performed under magnetic fields below and above a critical field Hc at which the energy gap closes.…

Strongly Correlated Electrons · Physics 2007-05-23 M. Hagiwara , L. P. Regnault , A. Zheludev , A. Stunault , N. Metoki , T. Suzuki , S. Suga , K. Kakurai , Y. Koike , P. Vorderwisch , J. H. Chung

The $S=1$ Haldane state is constructed from a product of local singlet dimers in the bulk and topological states at the edges of a chain. It is a fundamental representative of topological quantum matter. Its well-known representative, the…

The magnetic ground state of the quasi-one-dimensional spin-1 antiferromagnetic chain is sensitive to the relative sizes of the single-ion anisotropy ($D$) and the intrachain ($J$) and interchain ($J'$) exchange interactions. The ratios…

Inelastic neutron scattering was used to probe edge states in a quantum spin liquid. The experiment was performed on finite length antiferromagnetic spin-1 chains in Y_2BaNi_{1-x}Mg_xO_5. At finite fields, there is a Zeeman resonance below…

Strongly Correlated Electrons · Physics 2009-11-07 M. Kenzelmann , G. Xu , I. A. Zaliznyak , C. Broholm , J. F. DiTusa , G. Aeppli , T. Ito , K. Oka , H. Takagi

Inelastic neutron scattering experiments on the Haldane-gap quantum antiferromagnet \nd are performed at mK temperatures in magnetic fields of almost twice the critical field $H_c$ applied perpendicular to the spin cahins. Above $H_c$ a…

Strongly Correlated Electrons · Physics 2009-11-10 A. Zheludev , Z. Honda , C. Broholm , K. Katsumata , S. M. shapiro , A. Kolezhuk , S. Park , Y. Qiu

Inelastic neutron scattering experiments on Nd2BaNiO5 single-crystals and powder samples are used to study the dynamic coupling of 1-dimensional Haldane-gap excitations in the S=1 Ni2+ -chains to local crystal-field transitions, associated…

Strongly Correlated Electrons · Physics 2019-08-17 A. Zheludev , S. Maslov , T. Yokoo , J. Akimitsu , S. Raymond , S. E. Nagler , K. Hirota

Field-induced magnetic ordering in the Haldane chain compound SrNi$_{2}$V$_{2}$O$_{8}$ and effect of anisotropy have been investigated using single crystals. Static susceptibility, inelastic neutron scattering, high-field magnetization, and…

Strongly Correlated Electrons · Physics 2013-10-02 A. K. Bera , B. Lake , A. T. M. N. Islam , B. Klemke , E. Faulhaber , J. M. Law

The spin dynamics of the S=1 Ni-chains in mixed-spin antiferromagnets Pr_2 Ba Ni O_5 and Nd_x Y_2-x Ba Ni O_5 is described in terms of a simple Ginzburg-Landau Lagrangian coupled to the sublattice of rare-earth ions. Within this framework…

Strongly Correlated Electrons · Physics 2009-10-30 S. Maslov , A. Zheludev

The structure and the magnetic properties of layered Li3Cu2SbO6 are investigated by powder X-ray diffraction, static susceptibility, and electron spin resonance studies up to 330 GHz. The XRD data experimentally verify the space group C2/m…

Recent experiments on the quasi-1D antiferromagnets $R_{2}BaNiO_{5}$ (R = rare earth) have shown the existence of purely 1D Haldane gap excitations propagating on the Ni chains. Below an ordering temperature, the gap excitations survive and…

Strongly Correlated Electrons · Physics 2009-10-31 Indrani Bose , Emily Chattopadhyay

Results of magnetization and high-field ESR studies of the new spin-1 Haldane-chain material [Ni(C2H8N2)2NO2](BF4) (NENB) are reported. A definite signature of the Haldane state in NENB was obtained. From the analysis of the frequency-field…

Materials composed of spin-1 antiferromagnetic (AFM) chains are known to adopt complex ground states which are sensitive to the single-ion-anisotropy (SIA) energy ($D$), and intrachain ($J_{0}$) and interchain ($J'_{i}$) exchange energy…

Low-lying excited states as well as the ground state of the spin-1 antiferromagnetic Heisenberg chain with a spin-1/2 impurity are studied by means of a method of numerical diagonalization. The isotropic nearest-neighbor exchange coupling…

Condensed Matter · Physics 2009-10-28 Takashi Tonegawa , Makoto Kaburagi

Impurity effect is systematically studied in doped Haldane material Pb(Ni$_{1-x}$$M_x$)$_2$V$_2$O$_8$ ($M$ = Mn, Co, Cu, and Mg) by use of DC and AC susceptibility, and heat capacity measurements. The occurrence of three-dimensional ordered…

Strongly Correlated Electrons · Physics 2007-05-23 S. Imai , T. Masuda , T. Matsuoka , K. Uchinokura

Inelastic neutron scattering is used to investigate magnetic excitations in the quasi-one-dimensional quantum spin-liquid system Cu2Cl4 D8C4SO2. Contrary to previously conjectured models that relied on bond-alternating nearest neighbor…

Strongly Correlated Electrons · Physics 2007-11-14 V. O. Garlea , A. Zheludev , L. -P. Regnault , J. -H. Chung , Y. Qiu , M. Boehm , K. Habicht , M. Meissner

We report the results of elastic and inelastic neutron scattering experiments on the Haldane gap quantum antiferromagnet Ni(C5D14N2)2N3(PF6) performed at mK temperatures in a wide range of magnetic field applied parallel to the S = 1 spin…

Effects of interchain couplings and anisotropy on a Haldane chain have been investigated by single crystal inelastic neutron scattering and density functional theory (DFT) calculations on the model compound SrNi$_2$V$_2$O$_8$. Significant…

Strongly Correlated Electrons · Physics 2015-06-02 A. K. Bera , B. Lake , A. T. M. N. Islam , O. Janson , H. Rosner , A. Schneidewind , J. T. Park , E. Wheeler , S. Zander
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