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Motivated by recent experimental observations of opposite Chern numbers in $R$-type twisted MoTe$_2$ and WSe$_2$ homobilayers, we perform large-scale density-functional-theory (DFT) calculations with machine learning force fields to…

Materials Science · Physics 2024-05-21 Xiao-Wei Zhang , Chong Wang , Xiaoyu Liu , Yueyao Fan , Ting Cao , Di Xiao

Two-dimensional transition metal dichalcogenides (TMDC) have shown promise for various applications in optoelectronics and so-called valleytronics. Their operation and performance strongly depend on the stacking of individual layers. Here,…

Materials Science · Physics 2020-09-28 J. E. Zimmermann , B. Li , J. Hone , U. Höfer , G. Mette

In transition metal dichalcogenides (TMDCs), charge carriers have spin, pseudospin, and valley degrees of freedom associated with magnetic moments. The monolayers and bilayers of the TMDCs, in particular, MoS$_2$, lead strong couplings…

Materials Science · Physics 2021-11-29 Yeon Lee , Dasol Kim , Dong Eon Kim , Alexis Chacón

New theoretical proposals and experimental findings on transition metal dichalcogenide 1T-TaS$_2$ have revived interests in its possible Mott insulating state. We perform a comprehensive scanning tunneling microscopy and spectroscopy…

Strongly Correlated Electrons · Physics 2022-01-11 Zongxiu Wu , Kunliang Bu , Wenhao Zhang , Ying Fei , Yuan Zheng , Jingjing Gao , Xuan Luo , Zheng Liu , Yu-ping Sun , Yi Yin

Transition metal dichalcogenide MoS2 is a two-dimensional material, attracting much attention for next-generation applications thanks to rich functionalities stemmed from the crystal structure. Many experimental and theoretical works have…

Twisted transition-metal dichalcogenides host highly tunable moir\'e potentials, flat bands, and correlated electronic phases, yet the role of disorder in shaping these emergent properties remains largely unresolved. Using scanning…

We theoretically study the interplay between magnetism and a heavy Fermi liquid in the AB stacked transition metal dichalcogenide bilayer system MoTe$_2$/WSe$_2$ in the regime in which the Mo layer supports localized magnetic moments…

Strongly Correlated Electrons · Physics 2023-05-03 Daniele Guerci , Jie Wang , Jiawei Zang , Jennifer Cano , J. H. Pixley , Andrew Millis

Recent advances in the field of vertically stacked 2D materials have revealed a rich exciton landscape. In particular, it has been demonstrated that out-of-plane electrical fields can be used to tune the spectral position of spatially…

Mesoscale and Nanoscale Physics · Physics 2023-01-18 Joakim Hagel , Samuel Brem , Ermin Malic

Transition-metal dichalcogenides (TMDs) are layered compounds that support many electronic phases, including various charge density waves, superconducting, and Mott insulating states. Their intercalation with magnetic ions introduces…

Moir\'e superlattices formed by transition metal dichalcogenide (TMD) heterobilayers provide a versatile platform for studying strongly correlated electronic, excitonic, and topological phenomena in solids. In particular, angle-aligned…

Transition metal dichalcogenides (TMDs), such as MoS$_2$, are known to undergo a structural phase transformation as well as a change in the electronic conductivity upon Li intercalation. These properties make them candidates for…

Materials Science · Physics 2021-07-28 C. D. Spataru , M. D. Witman , R. E. Jones

We simulate the electronic and transport properties of metal/two-dimensional material/metal vertical heterostructures, with a focus on graphene, hexagonal boron nitride and two phases of molybdenum diselenide. Using density functional…

Mesoscale and Nanoscale Physics · Physics 2025-02-06 Gaëlle Bigeard , Zineb Kerrami , François Triozon , Alessandro Cresti

Stacking-dependent magnetism in two-dimensional van der Waals materials offers an effective route for controlling magnetic order without chemical modification. Here, we present a combined first-principles and finite-temperature study of…

Materials Science · Physics 2026-05-19 Soumyajit Sarkar , Soham Chandra

The topological properties of Bloch bands are intimately tied to the structure of their electronic wavefunctions within the unit cell of a crystal. Here, we show that scanning tunneling microscopy (STM) measurements on the prototypical…

Moir\'e heterobilayers exhibiting spatially varying band alignment and electron and hole localization that can be precisely controlled through the twist angle have emerged as exciting platforms for studying complex quantum phenomena. While…

Moir\'e materials, with superlattice periodicity many times the atomic length scale, have enabled the studies of strong electronic correlations and band topology with unprecedented tunability. However, nonvolatile control of the moir\'e…

Mesoscale and Nanoscale Physics · Physics 2022-09-15 Kaifei Kang , Wenjin Zhao , Yihang Zeng , Kenji Watanabe , Takashi Taniguchi , Jie Shan , Kin Fai Mak

Electronic tunability in crystals with weakly-bound layers can be achieved through layer stacking order. One such example is MoTe$_2$, where the low-temperature orthorhombic T$_d$ phase is topological and host to Weyl quasiparticles. The…

Materials Science · Physics 2019-04-17 John A. Schneeloch , Chunruo Duan , Xiaoping Wang , Jun Liu , Junjie Yang , Despina Louca

The electronic band structure of crystals is generally influenced by the periodic arrangement of their constituent atoms. Specifically, the emerging two-dimensional (2D) layered structures have shown different band structures with respect…

Materials Science · Physics 2017-01-04 Seho Yi , Jin-Ho Choi , Kimoon Lee , Sung Wng Kim , Chul Hong Park , Jun-Hyung Cho

Transition metal dichalcogenide (TMD) bilayers with an interlayer twist exhibit a moire super-period, whose effects can manifest in both structural and electronic properties. Atomic displacements can lead to reconstruction into domains of…

Materials Science · Physics 2025-10-23 Madeleine Phillips , C. Stephen Hellberg

Little is known about the role of weak interlayer coupling in the second harmonic generation (SHG) effects of two-dimensional van der Waals (vdW) systems. In this article, taking homo-bilayer $MoS_2/MoS_2$ and hetero-bilayer $MoS_2/MoSe_2$…

Computational Physics · Physics 2022-02-02 Xiao Jiang , Lei Kang , Bing Huang