Related papers: Cavity-modified exciton-exciton annihilation in di…
We present a microscopic semi-analytical theory for the description of organic molecules interacting strongly with a cavity mode. Exciton-vibration coupling within the molecule and exciton-cavity interaction are treated on an equal footing…
The concept of modifying molecular dynamics in strongly coupled exciton-polariton systems is an emerging topic in photonics due to its potential to produce customized chemical systems with tailored photophysical properties. However, before…
The manipulation of molecular excited state processes through strong coupling has attracted significant interest for its potential to provide precise control of photochemical phenomena. However, the key limiting factor for achieving this…
Polaritons, formed as a result of strong hybridization of matter with light, are promising for important applications including organic solar cells, optical logic gates, and qubits. Owing to large binding energies of Frenkel excitons…
Exciton-exciton annihilation (EEA), in which two excitons interact to generate high-energy excitations, is an important non-radiative channel in light-induced excited-state relaxation. When efficient, this process offers an alternative…
Two-dimensional (2D) semiconductors possess strongly bound excitons, opening novel opportunities for engineering light-matter interaction at the nanoscale. However, their in-plane confinement leads to large non-radiative exciton-exciton…
Understanding the radiative decay of exciton-polaritons is essential for achieving long-lived polaritons - a key prerequisite for enhancing nonlinear and quantum polaritonic effects. However, conventional wisdom - the coupled oscillator…
We demonstrate a new type of transition within the strong coupling regime, which alters the coupling mechanism in multimode cavities. We show that this transition drastically modifies the Hamiltonian describing the polaritons, such that…
Semiconductor quantum dots are among the best sources of on-demand entangled photon pairs. The degree of entanglement, however, is generally limited by the fine structure splitting of exciton states. In this paper, we theoretically…
Multi-exciton correlations shape the photo-induced response of nanostructured materials, particularly when interactions are enhanced by light confinement. Here multidimensional coherent spectroscopy is used to quantify biexciton and…
A quantum dot strongly coupled to a photonic crystal has been recently proposed as a source of entangled photon pairs [R. Johne et al., Phys. Rev. Lett. 100, 240404 (2008)]. The biexction decay via intermediate polariton states can be used…
Modifying the energy landscape of existing molecular emitters is an attractive challenge with favourable outcomes in chemistry and organic optoelectronic research. It has recently been explored through strong light-matter coupling studies…
The rate of non-radiative decay between two molecular electronic states is succinctly described by the energy gap law, which suggests an approximately-exponential dependence of the rate on the electronic energy gap. Here, we inquire whether…
Exciton-polaritons in semiconductors are quasi-particles which have recently shown the capability to undergo phase transition into a coherent hybrid state of light and matter. The observation of such quasi-particles in organic microcavities…
Recently, we predicted theoretically that in cavities that support several longitudinal modes, strong coupling can occur in very different manners, depending on the system parameters. Distinct longitudinal cavity modes are either entangled…
We show that when following a simple cavity design metric, a quantum well exciton-microcavity photon coupling constant can be larger than the exciton binding energy in GaAs based optical microcavities. Such a very strong coupling…
We investigate the exciton complexes photoluminescence, dynamics and photon statistics in the concurrent strong weak coupling regime in our unique site controlled singular inverted pyramidal InGaAs/GaAs quantum dots photonic crystal…
We theoretically designed and experimentally demonstrated a mechanism to protect a spatially segregated mixed light-matter state, known as intercavity exciton-polariton in strongly coupled optical cavities. This excitation, shared across…
Very efficient amplification of light-matter waves (polaritons), that are a superposition of cavity photons and excitons [1] has recently been reported[2-11]. The optical gain curve versus the pump power shows a threshold and then saturates…
The exceptionally strong Coulomb interaction in semiconducting transition-metal dichalcogenides (TMDs) gives rise to a rich exciton landscape consisting of bright and dark exciton states. At elevated densities, excitons can interact through…