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We present the first full-potential method that solves the fully relativistic 4-component Dirac-Kohn-Sham equation for materials in the solid state within the framework of atom-centered Gaussian-type orbitals (GTOs). Our GTO-based method…

Chemical Physics · Physics 2019-05-07 Marius Kadek , Michal Repisky , Kenneth Ruud

We give a systematic and self-contained account of the construction of geometrically decomposed bases and degrees of freedom in finite element exterior calculus. In particular, we elaborate upon a previously overlooked basis for one of the…

Numerical Analysis · Mathematics 2022-10-24 Martin W. Licht

We show here that the Hamiltonian for an electronic system may be written exactly in terms of fluctuation operators that transition constituent fragments between internally correlated states, accounting rigorously for inter-fragment…

Chemical Physics · Physics 2019-05-24 Anthony D. Dutoi , Yuhong Liu

A key objective of computational solid state physics is to predict electronic properties of periodic materials. However, electronic structure simulations based on density functional theory fail to predict experimental results if…

We reconsider the non-equilibrium dynamics of closed quantum systems. In particular we focus on the thermalization of integrable systems. Here we show how the generalized Gibbs Ensemble (GGE) can be constructed as the best approximation to…

Quantum Physics · Physics 2017-05-11 Dries Sels , Michiel Wouters

We study ergodic properties of certain piecewise smooth two-dimensional systems by constructing countable Markov partitions. Using thermodynamic formalism we prove exponential decay of correleations.

Dynamical Systems · Mathematics 2016-01-25 Michael Jakobson

We present an efficient \textit{ab initio} method for calculating the electronic structure and total energy of strongly correlated electron systems. The method extends the traditional Gutzwiller approximation for one-particle operators to…

Strongly Correlated Electrons · Physics 2014-07-01 Y. X. Yao , J. Liu , C. Liu , W. C. Lu , C. Z. Wang , K. M. Ho

The Empirical Tight Binding(ETB) method is widely used in atomistic device simulations. The reliability of such simulations depends very strongly on the choice of basis sets and the ETB parameters. The traditional way of obtaining the ETB…

A generalized scheme for the construction of coherent states in the context of position-dependent effective mass systems has been presented. This formalism is based on the ladder operators and associated algebra of the system which are…

Quantum Physics · Physics 2017-01-04 Naila Amir , Shahid Iqbal

We derive global analytic representations of fundamental solutions for a class of linear parabolic systems with full coupling of first order derivative terms where coefficient may depend on space and time. Pointwise convergence of the…

Analysis of PDEs · Mathematics 2009-07-17 Joerg Kampen

To describe charged particles interacting with the quantized electromagnetic field, we point out the differences of working in the so-called generalized and the true Coulomb gauges. We find an explicit gauge transformation between them for…

Quantum Physics · Physics 2019-09-18 Robert Zietal , Claudia Eberlein

We present a simple and general method for construction of localized orbitals to describe electronic structure of extended periodic metals and insulators as well as confined systems. Spatial decay of these orbitals is found to exhibit…

Materials Science · Physics 2007-05-23 Joydeep Bhattacharjee , Umesh V Waghmare

A novel strategy is proposed for the coupling of field and circuit equations when modeling power devices in the low-frequency regime. The resulting systems of differential-algebraic equations have a particular geometric structure which…

Numerical Analysis · Mathematics 2024-04-25 Herbert Egger , Idoia Cortes Garcia , Vsevolod Shashkov , Michael Wiesheu

The cumulant expansion is a powerful approach for including correlation effects in electronic structure calculations beyond the GW approximation. However, current implementations are incomplete since they ignore terms that lead to partial…

Strongly Correlated Electrons · Physics 2014-02-04 J. J. Kas , J. J. Rehr , L. Reining

We solve elliptic systems of equations posed on highly heterogeneous materials. Examples of this class of problems are composite structures and geological processes. We focus on a model problem which is a second-order elliptic equation with…

Numerical Analysis · Mathematics 2015-12-11 Leonardo A. Poveda , Sebastian Huepo , Victor M. Calo , Juan Galvis

The envelope function method traditionally employs a single basis set which, in practice, relates to a single material because the $k\cdot p$ matrix elements are generally only known in a particular basis. In this work, we defined a basis…

Mesoscale and Nanoscale Physics · Physics 2018-01-29 Maarten L. Van de Put , William G. Vandenberghe , Wim Magnus , Bart Sorée

We analyze wave functions constructed as a sum of product of two-electron functions, or as a polynomial of geminals, to investigate their ability to represent the ground state of a strongly correlated few-body system. The known difficulty…

Chemical Physics · Physics 2018-05-17 Airi Kawasaki , Osamu Sugino

We define a class of quantum systems called regular quantum graphs. Although their dynamics is chaotic in the classical limit with positive topological entropy, the spectrum of regular quantum graphs is explicitly computable analytically…

Quantum Physics · Physics 2007-05-23 R. Blümel , Yu. Dabaghian , R. V. Jensen

We develop a discontinuous Galerkin (DG) framework for automatically constructing adaptive basis sets for electronic structure calculations. By allowing basis functions to be discontinuous across element interfaces, our approach supports…

Computational Physics · Physics 2026-03-03 Yulong Pan , Michael Lindsey

We treat a system (a molecule or a solid) in which electrons are coupled linearly to any number and type of harmonic oscillators and which is further subject to external forces of arbitrary symmetry. With the treatment restricted to the…

Other Condensed Matter · Physics 2009-11-10 Robert Englman , Asher Yahalom
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