English
Related papers

Related papers: Vacancy-Enhanced $N-N$ Bonding and Deep Level Comp…

200 papers

The formation of framework vacancies in Si- and Ge-based type-I clathrates is studied as function of filling the cages with K and Ba atoms using density-functional theory. Our analysis reveals the relevance of structural disorder, geometric…

Formation and excitation energies as well charge transition levels, are determined forthe substitutional nitrogen (Ns),the vacancy (V) and related point defects (NV, NVH, N2, N2V and V2) by screened non-local hybrid density functional…

Materials Science · Physics 2013-11-27 Peter Deák , Bálint Aradi , Moloud Kaviani , Thomas Frauenheim , Adam Gali

We studied the oxygen vacancies($V_{O}$) in rutile TiO2 by using $G_0W_0$ approximation on top of GGA+$U$ as a method of choice to improve the gap. Since there is no extensive agreement regarding the characteristic of electron localization…

Strongly Correlated Electrons · Physics 2010-12-30 Ali Kazempour , Seyed Javad Hashemifar , Hadi Akbarzadeh

The discovery of superconductivity in La3Ni2O7 has attracted significant research interest in the field of nickelate superconductors. Despite extensive studies on pristine La3Ni2O7, the impact of oxygen vacancies (VO), a common type of…

Materials Science · Physics 2024-06-07 Xuelei Sui , Xiangru Han , Xiaojun Chen , Liang Qiao , Xiaohong Shao , Bing Huang

In this work an overall electronic structure including the position and formation energies of various intrinsic defects are computed for anatase using Density Functional Theory aided by Hubbard correction (DFT+U). The intrinsic point…

Oxygen vacancies in strontium titanate surfaces (SrTiO3) have been linked to the presence of a two-dimensional electron gas with unique behavior. We perform a detailed density functional theory study of the lattice and electronic structure…

Strongly Correlated Electrons · Physics 2015-06-22 Harald O. Jeschke , Juan Shen , Roser Valenti

We develop an atomistic, nearest-neighbor sp3s* tight-binding Hamiltonian to investigate the electronic structure of dilute bismide alloys of GaP and GaAs. Using this model we calculate that the incorporation of dilute concentrations of Bi…

Materials Science · Physics 2011-12-12 Muhammad Usman , Christopher A. Broderick , Andrew Lindsay , Eoin P. O'Reilly

The role of intrinsic defects has been investigated to determine binding energies and the electronic structure of Gd complexes in ZnO. We use density-functional theory and the GW method to show that the presence of vacancies and…

Materials Science · Physics 2018-01-23 A. L. Rosa , Th. Frauenheim

Oxygen is the most common unintentional impurity found in GaN. We study the interaction between substitutional oxygen (ON) and the gallium vacancy (VGa) to form a point defect complex in GaN. The formation energy of the gallium vacancy is…

Materials Science · Physics 2018-06-29 Zijuan Xie , Yu Sui , John Buckeridge , Alexey A. Sokol , Thomas W. Keal , Aron Walsh

Characterizing the local internal environment surrounding solid-state spin defects is crucial to harnessing them as nanoscale sensors of external fields. This is especially germane to the case of defect ensembles which can exhibit a complex…

We analyze Ge-related defects in Ge-doped SiO_2 using first-principles density functional techniques. Ge is incorporated at the level of ~ 1 mol % and above. The growth conditions of Ge:SiO_2 naturally set up oxygen deficiency, with vacancy…

Materials Science · Physics 2009-11-07 C. M. Carbonaro , V. Fiorentini , F. Bernardini

We introduce a self-passivation of single lead (Pb) and oxygen (O) vacancies in the \alpha-PbO compound through formation of a Pb-O vacancy pair. The preferential mechanism for pair formation involves initial development of the single Pb…

Materials Science · Physics 2015-06-12 J. Berashevich , J. A. Rowlands , A. Reznik

The nitrogen-vacancy (NV) center occurs in GaAs bulk crystals doped or implanted with nitrogen. The local vibration of nitrogen gives rise to a sharp infrared absorption band at 638 cm$^{-1}$, exhibiting a fine structure due to the…

Materials Science · Physics 2018-02-07 Nicola Kovač , Christopher Künneth , Hans Christian Alt

Using first-principles calculations, we explored all the 21 defect-pairs in GaN and considered 6 configurations with different defect-defect distances for each defect-pair. 15 defect-pairs with short defect-defect distances are found to be…

Materials Science · Physics 2020-03-13 He Li , Menglin Huang , Shiyou Chen

Enhanced conductivity at ferroelectric domain walls in BiFeO$_3$ has been widely observed, yet the microscopic origins of this effect, including electronic contributions from domain-wall defects, are incompletely understood at the atomistic…

Materials Science · Physics 2025-07-17 Guo-Dong Zhao , Ismaila Dabo , Long-Qing Chen

In this paper we examine the electronic and geometrical structure of impurity-vacancy complexes in Si and Ge. Already Watkins suggested that in Si the pairing of Sn with the vacancy produces a complex with the Sn-atom at the bond center and…

Materials Science · Physics 2016-08-31 H. Hoehler , N. Atodiresei , K. Schroeder , R. Zeller , P. H. Dederichs

We report a study of the 3E excited-state structure of single nitrogen-vacancy (NV) defects in diamond, combining resonant excitation at cryogenic temperatures and optically detected magnetic resonance. A theoretical model of the…

The influence of atomic vacancy defects at different concentrations on electronic properties of MoS$_2$ and WS$_2$ monolayers is studied by means of Slater-Koster tight-binding model with non-orthogonal $sp^3d^5$ orbitals and including the…

Mesoscale and Nanoscale Physics · Physics 2016-05-30 Saboura Salehi , Alireza Saffarzadeh

Oxygen vacancies at the SnO2(110) and (101) surface and subsurface sites have been studied in the framework of density functional theory by using both all-electron Gaussian and pseudopotential plane-wave methods. The all-electron…

Materials Science · Physics 2008-06-06 F. Trani , M. Causa' , D. Ninno , G. Cantele , V. Barone

The structure and energetics of Ge substitutional defects on the alpha-Sn/Ge(111) surface are analyzed using Density Functional Theory (DFT) molecular dynamics (MD) simulations. An isolated Ge defect induces a very local distortion of the…

Materials Science · Physics 2009-11-07 Jose Ortega , Ruben Perez , Leszek Jurczyszyn , Fernando Flores