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We report on the fragmentation of the water molecule by $1$ MeV H$^{+}$, He$^{+}$ and 650 keV N$^{+}$ ion impact. The fragment-ion energy spectra were measured by an electrostatic spectrometer at different observation angles. The obtained…

Atomic Physics · Physics 2017-09-13 S. T. S. Kovács , P. Herczku , Z. Juhász , L. Sarkadi , L. Gulyás , B. Sulik

We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…

Atomic Physics · Physics 2016-04-12 Lun Yue , Lars Bojer Madsen

The time-dependent surface flux method developed for the description of electronic spectra [L. Tao and A. Scrinzi, New J. Phys. 14, 013021 (2012); A. Scrinzi, New J. Phys. 14, 085008 (2012)] is extended to treat dissociation and…

Atomic Physics · Physics 2014-10-09 Lun Yue , Lars Bojer Madsen

Partial photoionization cross sections from the ^1S ground and the ^3P metastable states of the Be isoelectronic series to different final states including a number of satellite (ionization plus excitation) channels are studied using the…

Atomic Physics · Physics 2012-05-25 W. -C. Chu , H. -L. Zhou , A. Hibbert , S. T. Manson

We study the resonant sequential two-photon ionization of neutral atoms by a combination of twisted- and plane-wave light within a fully relativistic framework. In particular, the ionization of an isotropic ensemble of neutral sodium atoms…

Atomic Physics · Physics 2021-01-04 V. P. Kosheleva , V. A. Zaytsev , R. A. Müller , A. Surzhykov , S. Fritzsche

The ultrafast electronic and nuclear dynamics of H2 laser-induced double ionization is studied using a time-dependent wave packet approach that goes beyond the fixed nuclei approximation. The double ionization pathways are analyzed by…

Quantum Physics · Physics 2011-11-09 Sebastien Saugout , Christian Cornaggia , Annick Suzor-Weiner , Eric Charron

We use transient absorption spectroscopy to monitor the ionization and dissociation products following two-photon excitation of pure liquid water. The two decay mechanisms occur with similar yield for an excitation energy of 9.3 eV, whereas…

Chemical Physics · Physics 2009-11-13 Christopher G. Elles , Ilya A. Shkrob , Robert A. Crowell , Stephen E. Bradforth

Molecular iodine was photoexcited by a strong 800 nm laser, driving several channels of multiphoton excitation. The motion following photoexcitation was probed using time-resolved X-ray scattering, which produces a scattering map…

Chemical Physics · Physics 2020-03-25 Philip H. Bucksbaum , Matthew R. Ware , Adi Natan , James P. Cryan , James M. Glownia

We report the results of a first-principles study of dissociative electron attachment to H2O. The cross sections are obtained from nuclear dynamics calculations carried out in full dimensionality within the local complex potential model by…

Chemical Physics · Physics 2007-10-10 Daniel J. Haxton , T. N. Rescigno , C. W. McCurdy

Macroscopic field quantization is presented for a nondispersive photonic dielectric environment, both in the absence and presence of guest atoms. Starting with a minimal-coupling Lagrangian, a careful look at functional derivatives shows…

Quantum Physics · Physics 2007-10-31 Martijn Wubs , L. G. Suttorp , A. Lagendijk

We consider photo ionization of an atom which, due to passing through a diffraction grating, is prepared in a multi-site state possessing a periodic space structure with alternating maxima and minima. It has been found that this process…

Atomic Physics · Physics 2020-08-07 S. F. Zhang , B. Najjari , X. Ma , A. B. Voitkiv

The two-photon decay in hydrogen-like ions is investigated within the framework of second order perturbation theory and Dirac's relativistic equation. Special attention is paid to the angular correlation of the emitted photons as well as to…

Atomic Physics · Physics 2014-10-23 P. Amaro , F. Fratini , S. Fritzsche , P. Indelicato , J. P. Santos , A. Surzhykov

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We have observed the signatures of valence electron rearrangement in photoexcited ammonia using ultrafast hard X-ray scattering. Time-resolved X-ray scattering is a powerful tool for imaging structural dynamics in molecules because of the…

The radiative recombination of a free electron into an excited state of a bare, high-Z ion is studied, together with its subsequent decay, within the framework of the density matrix theory and Dirac's relativistic equation. Special…

Atomic Physics · Physics 2010-11-29 A. V. Maiorova , A. Surzhykov , S. Tashenov , V. M. Shabaev , S. Fritzsche , G. Plunien , Th. Stoehlker

A new semiclassical approach to ionization by an oscillating field is presented. For a delta-function atom, an asymptotic analysis is performed with respect to a quantity h, defined as the ratio of photon energy to ponderomotive energy.…

Quantum Physics · Physics 2009-10-30 Klaus Ergenzinger

We present multilevel radiative transfer modeling of the scattering polarization observed in the solar O I infrared triplet around 777 nm. We demonstrate that the scattering polarization pattern observed on the solar disk forms in the…

Solar and Stellar Astrophysics · Physics 2015-08-06 T. del Pino Alemán , J. Trujillo Bueno

We demonstrate an optical method for detecting the mechanical oscillations of an atom with single-phonon sensitivity. The measurement signal results from the interference between the light scattered by a single trapped atomic ion and that…

Atomic Physics · Physics 2021-08-11 G. Cerchiari , G. Araneda , L. Podhora , L. Slodička , Y. Colombe , R. Blatt

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…

Chemical Physics · Physics 2018-08-21 P. Wustelt , F. Oppermann , Lun Yue , M. Möller , T. Stöhlker , S. Gräfe , M. Lein , G. G. Paulus , A. M. Sayler