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We utilize ultrafast photoexcitation to drive coherent lattice oscillations in the layered ferrimagnetic crystal Mn3Si2Te6, which significantly stiffen below the magnetic ordering temperature. We suggest that this is due to an…

Spin-orbit coupling (SOC) is a relativistic effect, where an electron moving in an electric field experiences an effective magnetic field in its rest frame. In crystals without inversion symmetry, it lifts the spin degeneracy and leads to…

Spin-orbit coupling (SOC) and electron-electron interaction can mutually influence each other and give rise to a plethora of intriguing phenomena in condensed matter systems. In pristine bilayer graphene, which has weak SOC, intrinsic…

Elucidating spin correlations in the parent compounds of high-temperature superconductors is crucial for understanding superconductivity. We used neutron scattering to study spin correlations in Li$_{1-x}$Fe$_x$ODFeSe, an insulating…

Superconductivity · Physics 2025-01-06 Hongliang Wo , Bingying Pan , Die Hu , Yu Feng , A. D. Christianson , Jun Zhao

Light fields at THz and mid-infrared frequencies allow for the direct excitation of collective modes in condensed matter, which can be driven to large amplitudes. For example, excitation of the crystal lattice, has been shown to stimulate…

The interlayer exchange coupling in Fe/MgO(001) superlattices is found to increase exponentially with decreasing temperature. Around 150~K, the field induced response changes from discrete switching, governed by field-driven domain…

A coupled atomistic spin and lattice dynamics approach is developed which merges the dynamics of these two degrees of freedom into a single set of coupled equations of motion. The underlying microscopic model comprises local exchange…

Materials Science · Physics 2018-01-24 J. Fransson , D. Thonig , P. F. Bessarab , S . Bhattacharjee , J. Hellsvik , L. Nordström

Magnetic frustrations and degeneracies profoundly affect ground-state magnetic properties emerging from competing exchange interactions. Controlling such frustrations using orbital and phonon engineering via the Kugel-Khomskii-type…

Electrochemical water splitting is an environmentally friendly technology to store renewable energy in the form of chemical fuels. Among the earth-abundant first-row transition metal-based catalysts, mixed Ni-Fe oxides have shown promising…

Spin spirals form inside the magnetic layers of antiferromagnetic and noncollinearly-coupled magnetic multilayers in the presence of an external magnetic field. This spin structure can be modeled to extract the direct exchange stiffness of…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 Elliot Wadge , Afan Terko , George Lertzman-Lepofsky , Paul Omelchenko , Bret Heinrich , Manuel Rojas , Erol Girt

Geometric frustration among competing spin exchanges can give rise to novel quantum phases by enhancing fluctuations that drive magnetic systems beyond the classical regime. We investigate the frustrated array of strongly correlated spin…

We introduce a theoretical framework for computaions of anisotropic multipolar exchange interactions found in many spin--orbit coupled magnetic systems and propose a method to extract these coupling constants using a density functional…

Strongly Correlated Electrons · Physics 2014-08-01 Shu-Ting Pi , Ravindra Nanguneri , Sergey Savrasov

We have investigated the coupling of lattice with spin via strain interactions in the CoFe2O4/PMN-PT composite system. X-ray diffraction and Raman spectroscopic studies illustrate a remarkable modification in CoFe2O4lattice across Curie…

We propose a powerful extension to combined molecular and spin dynamics that fully captures the coupling between the atomic and spin subsystems via spin-orbit interactions. Its foundation is the inclusion of the local magnetic anisotropies…

Materials Science · Physics 2016-12-28 Dilina Perera , Markus Eisenbach , Don M. Nicholson , G. Malcolm Stocks , David P. Landau

Nanocrystalline MnFe$_{2}$O$_{4}$ has shown promise as a catalyst for the oxygen reduction reaction (ORR) in alkaline solutions, but the material has been lightly studied as highly ordered thin film catalysts. To examine the role of surface…

Realizing room-temperature ferromagnetic insulators, critical enablers for low-power spintronics, is fundamentally challenged by the long-standing trade-off between ferromagnetic ordering and indirect exchange interactions in insulators.…

Materials Science · Physics 2025-09-09 Xuanchi Zhou , Jiahui Ji , Wentian Lu , Huihui Ji , Chunwei Yao , Xiaohui Yao , Xiaomei Qiao , Guowei Zhou , Xiaohong Xu

Emergent molecular-like excitations have been discovered in a series of pyrochlore antiferromagnets, yet their origins and relationships with the coexisting magnon excitations remain a puzzle. Here, by incorporating the dynamic spin-lattice…

Strongly Correlated Electrons · Physics 2024-12-31 Shang Gao

We theoretically study the dynamic time evolution following laser pulse pumping in an antiferromagnetic insulator Cr$_{2}$O$_{3}$. From the photoexcited high-spin quartet states to the long-lived low-spin doublet states, the ultrafast…

Strongly Correlated Electrons · Physics 2017-06-29 Feng Guo , Na Zhang , Wei Jin , Jun Chang

2D materials present an interesting platform for device designs. However, oxidation can drastically change the system's properties, which need to be accounted for. Through {\it ab initio} calculations, we investigated freestanding and…

Materials Science · Physics 2023-11-21 R. L. H. Freire , F. Crasto de Lima , A. Fazzio

Motivated by the recent wealth of exotic magnetic phases emerging in two-dimensional frustrated lattices, we investigate the origin of possible magnetism in the monolayer family of triangular lattice materials $MX_2$ ($M$={V, Mn, Ni},…