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We report a comprehensive high-field/high-frequency electron spin resonance (ESR) study on single crystals of the van der Waals magnet CrCl$_3$. This material, although being known for quite a while, has received recent significant…

Materials Science · Physics 2020-06-09 J. Zeisner , K. Mehlawat , A. Alfonsov , M. Roslova , T. Doert , A. Isaeva , B. Büchner , V. Kataev

Since their first observation in 2017, atomically thin van der Waals (vdW) magnets have attracted significant fundamental, and application-driven attention. However, their low ordering temperatures, $T_c$, sensitivity to atmospheric…

Changes in the spin configuration of atomically-thin, magnetic van-der-Waals multilayers can cause drastic modifications in their opto-electronic properties. Conversely, the opto-electronic response of these systems provides information…

Mesoscale and Nanoscale Physics · Physics 2020-05-28 Zhe Wang , Marco Gibertini , Dumitru Dumcenco , Takashi Taniguchi , Kenji Watanabe , Enrico Giannini , Alberto F. Morpurgo

CrCl3 is a layered insulator that undergoes a crystallographic phase transition below room temperature and orders antiferromagnetically at low temperature. Weak van der Waals bonding between the layers and ferromagnetic in-plane magnetic…

The magnetic nature of low dimensional compound, CrCl$_3$, was investigated by muon spin rotation, relaxation and resonance ($\mu^+$SR). The $\mu^+$SR measurements revealed three distinct phases as a function of temperature: an…

The discovery of two-dimensional (2D) systems hosting intrinsic long-range magnetic order represents a seminal addition to the rich physical landscape of van der Waals (vdW) materials. CrI3 has emerged as perhaps the most salient example,…

Investigating spin and charge noise in strongly correlated electron systems is a valuable way to analyze their physical properties and unlock new phases of matter. In this context, nitrogen-vacancy (NV) center-based magnetometry has been…

Van der Waals (vdW) magnet heterostructures have emerged as new platforms to explore exotic magnetic orders and quantum phenomena. Here, we study heterostructures of layered antiferromagnets, CrI3 and CrCl3, with perpendicular and in-plane…

We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 by specific heat and magnetization measurements of single crystals in high magnetic fields and by ab initio density functional theory calculations…

Two dimensional van der Waals ferromagnets with honeycomb structures are expected to host the bosonic version of Dirac particles in their magnon excitation spectra. Using inelastic neutron scattering, we study spin wave excitations in…

Strongly Correlated Electrons · Physics 2021-10-29 Lebing Chen , Matthew B. Stone , Alexander I. Kolesnikov , Barry Winn , Wonhyuk Shon , Pengcheng Dai , Jae-Ho Chung

Layered transition-metal compounds with controllable magnetic behaviors provide many fascinating opportunities for the fabrication of high-performance magneto-electric and spintronic devices. The tuning of their electronic and magnetic…

Cavity-magnon-polaritons are hybrid excitations from the interaction between cavity photons and magnons, the quanta of collective spin oscillations. Along with the tunability of the magnon-photon coupling strength, fast information transfer…

The magnetic moment in van der Waals (vdW) materials containing 3d transition metals originates from unpaired d-electron spins and their interaction with surrounding ligands. The interplay between exchange interactions and magnetic…

Two-dimensional honeycomb lattice ferromagnet chromium tri-iodide (CrI$_3$) has attracted tremendous interest because it retains ferromagnetism down to the monolayer limit and hosts intriguing topological magnons. As a prototypical van der…

Materials Science · Physics 2026-05-08 Weiliang Yao , Matthew B. Stone , Colin L. Sarkis , Yi Li , Ruixian Liu , Xingye Lu , Pengcheng Dai

Precision magnetometry is fundamental to the development of novel magnetic materials and devices. Recently, the nitrogen-vacancy (NV) center in diamond has emerged as a promising probe for static magnetism in 2D van der Waals materials,…

Two-dimensional (2D) magnetic materials offer unprecedented opportunities for fundamental physics and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI3 and Cr2Ge2Te6, this emerging field has expanded to…

Understanding and controlling spin dynamics in two-dimensional (2D) van der Waals (vdW) ferromagnets is essential for their application in magnonics and hybrid quantum platforms. Here, we investigate the spin dynamics of the vdW ferromagnet…

Spin-waves have been studied for data storage, communication and logic circuits in the field of spintronics based on their potential to substitute electrons. Recent discovery of magnetism in two-dimensional (2D) systems such as monolayer…

Understanding the coupling between lattice vibrations and magnetic order is crucial for controlling properties of two-dimensional magnetic materials. Here, we investigate the vibrational properties of bulk and thick-flake CrCl$_\textrm{3}$…

Manipulation of long-range order in two-dimensional (2D) van der Waals (vdW) magnetic materials (e.g., CrI$_3$, CrSiTe$_3$ etc.), exfoliated in few-atomic layer, can be achieved via application of electric field, mechanical-constraint,…

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