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The emergence of confined structures and pattern formation are exceptional manifestations of concurring nonlinear interactions found in a variety of physical, chemical and biological systems[1]. Optical solitons are a hallmark of extreme…

Optics · Physics 2020-01-29 Felix Kurtz , Claus Ropers , Georg Herink

The numerical solution for polarization for two-level atom in polyharmonic field has been made. The analytical solution for partial case of symmetrical position of carrier frequency relative to transition frequency is possible. The results…

We present an ab initio method for computing vibro-polariton and phonon-polariton spectra of molecules and solids coupled to the photon modes of optical cavities. We demonstrate that if interactions of cavity photon modes with both nuclear…

Chemical Physics · Physics 2025-12-23 John Bonini , Iman Ahmadabadi , Johannes Flick

We present a full microscopic many-body calculation of a recently-proposed nonlinear two-dimensional spectroscopy for Fermi polarons, and show that the quantum coherence between the attractive and repulsive polarons, which has never been…

Quantum Gases · Physics 2022-08-04 Jia Wang , Hui Hu , Xia-Ji Liu

Replacing independent single quantum wells inside a strongly-coupled semiconductor microcavity with double quantum wells produces a special type of polariton. Using asymmetric double quantum wells in devices processed into mesas allows the…

Ab initio computation of two-dimensional electronic spectra is an expanding field, whose goal is improving upon simple, few-dimensional models often employed to explain experiments. Here, we propose an accurate and computationally…

Chemical Physics · Physics 2024-09-26 Tomislav Begušić , Jiří Vaníček

Linear spectra of molecular polaritons formed by $N$ molecules coupled to a microcavity photon mode are usually well described by classical linear optics, raising the question of where the expected nonlinear effects in these strongly…

Quantum Physics · Physics 2024-11-19 Arghadip Koner , Joel Yuen-Zhou

We present a first-principles approach for calculating phonon-polariton dispersion relations. In this approach, phonon-photon interaction is described by quantization of a Hamiltonian that describes harmonic lattice vibrations coupled with…

Materials Science · Physics 2026-01-13 Olle Hellman , Leeor Kronik

We report the first experimental two-dimensional infrared (2D IR) spectra of novel molecular photonic excitations - vibrational-polaritons. The application of advanced 2D IR spectroscopy onto novel vibrational-polariton challenges and…

By means of analytical and numerical methods we analyze the phase diagram of polaritons in one-dimensional coupled cavities. We locate the phase boundary, discuss the behavior of the polariton compressibility and visibility fringes across…

Quantum Physics · Physics 2007-10-29 Davide Rossini , Rosario Fazio

Femtosecond coherent multidimensional spectroscopy is demonstrated for an ultracold gas. For this, a setup for phase modulation spectroscopy is used to probe the $3^2\mathrm{S}_{1/2} - 2^2\mathrm{P}_{1/2, 3/2}$ transition in an 800…

Atomic Physics · Physics 2023-01-16 Friedemann Landmesser , Tobias Sixt , Katrin Dulitz , Lukas Bruder , Frank Stienkemeier

We study a hybrid semiconductor-optomechanical system, which consists of a cavity with an oscillating mirror made by semiconducting materials or with a semiconducting membrane inside. The cavity photons and the excitons in the oscillating…

Quantum Physics · Physics 2018-10-03 Sai-Nan Huai , Yu-Long Liu , Yunbo Zhang , Yu-xi Liu

Recent experiments and theory demonstrate that the the ground state properties and chemical reactivity of molecules can be modified inside an optical cavity. The vibrational strong or ultrastrong coupling results in the formation of…

Chemical Physics · Physics 2022-12-01 Qi Yu

Rephasing and non-rephasing two-dimensional coherent spectra map the anti-crossing associated with normal-mode splitting in a semiconductor microcavity. For a 12-meV detuning range near zero detuning, it is observed that there are two…

Mesoscale and Nanoscale Physics · Physics 2015-05-26 Brian L. Wilmer , Felix Passmann , Michael Gehl , Galina Khitrova , Alan D. Bristow

A novel concept of self-phasematched optical frequency conversion in dispersive dielectric microcavities is studied theoretically and experimentally. We develop a time-dependent model, incorporating the dispersion into the structure of the…

Optics · Physics 2009-11-13 Alex Hayat , Meir Orenstein

We apply the Anharmonic Oscillator Symmetry Model to the description of vibrational excitations in ${\cal D}_{3h}$ and ${\cal T}_d$ molecules. A systematic procedure can be used to establish the relation between the algebraic and…

chem-ph · Physics 2008-02-03 A. Frank , R. Lemus , R. Bijker , F. Perez-Bernal , J. M. Arias

Entanglement generation in polariton systems is fundamentally constrained by high losses and decoherence, which typically outweigh polariton nonlinearities. Here, we propose a conceptually different approach that uses optomechanical…

We revisit scattering of electromagnetic waves from metallic and semiconducting cylinders in the framework of complex angular momentum techniques. We prove that "resonant surface polariton modes" are generated by a unique surface wave, i.e.…

Materials Science · Physics 2007-05-23 Stéphane Ancey , Yves Décanini , Antoine Folacci , Paul Gabrielli

Spectral properties of coupled cavity arrays in one dimension are investigated by means of the variational cluster approach. Coupled cavity arrays consist of two distinct "particles," namely, photons and atomiclike excitations. Spectral…

Other Condensed Matter · Physics 2015-03-13 Michael Knap , Enrico Arrigoni , Wolfgang von der Linden

We develop a non-Gaussian variational approach that enables us to study both equilibrium and far-from-equilibrium physics of the two-dimensional Fermi polaron. This method provides an unbiased analysis of the polaron-to-molecule phase…

Quantum Gases · Physics 2026-05-01 Yi-Fan Qu , Pavel E. Dolgirev , Eugene Demler , Tao Shi