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Intense, few-cycle pulses in the terahertz frequency range have strong potential for schemes of control over vibrational modes in solid-state materials in the electronic ground-state. Here we report an experiment using single cycle…

Recent experimental advances in atomically thin transition metal dichalcogenide (TMD) metals have unveiled a range of interesting phenomena including the coexistence of charge-density-wave (CDW) order and superconductivity down to the…

Superconductivity · Physics 2016-08-31 Xiaoxiang Xi , Helmuth Berger , László Forró , Jie Shan , Kin Fai Mak

Ultrafast photoexcitation offers a novel approach to manipulating quantum materials. One of the long-standing goals in this field is to achieve optical control over topological properties. However, the impact on their electronic structures,…

Materials Science · Physics 2024-12-10 Masataka Mogi , Dongsung Choi , Louis Primeau , Baiqing Lv , Doron Azoury , Yifan Su , Liang Fu , Yang Zhang , Nuh Gedik

Ferroelectric nematic liquid crystals represent not only interesting fundamental science, but they also hold promise for storage capacitors with high power density or new information display technology having sub-millisecond switching. In…

Due to the strong coupling between magnetism and ferroelectricity, $(\mathrm{ND}_4)_2\mathrm{FeCl}_5\cdot\mathrm{D}_2\mathrm{O}$ exhibits several intriguing magnetic and electric phases. In this letter, we include high-order onsite spin…

Materials Science · Physics 2021-08-25 Shaozhi Li , Randy S. Fishman

Coherent light-matter interactions mediated by opto-magnetic phenomena like the inverse Faraday effect (IFE) are expected to provide a non-thermal pathway for ultrafast manipulation of magnetism on timescales as short as the excitation…

Radio-frequency compressed ultrafast electron diffraction has been used to probe the coherent and incoherent coupling of impulsive electronic excitation at 1.55 eV (800 nm) to optical and acoustic phonon modes directly from the perspective…

Materials Science · Physics 2015-06-23 Robert P. Chatelain , Vance R. Morrison , Bart L. M. Klarenaar , Bradley J. Siwick

Functional renormalization yields a simple unified description of bosons at zero temperature, in arbitrary space dimension $d$ and for $M$ complex fields. We concentrate on nonrelativistic bosons and an action with a linear time derivative.…

Superconductivity · Physics 2009-11-13 C. Wetterich

We have used a combination of ultrafast coherent phonon spectroscopy, ultrafast thermometry, and time-dependent Landau theory to study the inversion symmetry breaking phase transition at $T_c = 200$ K in the strongly spin-orbit coupled…

Strongly Correlated Electrons · Physics 2018-01-26 J. W. Harter , D. M. Kennes , H. Chu , A. de la Torre , Z. Y. Zhao , J. -Q. Yan , D. G. Mandrus , A. J. Millis , D. Hsieh

The ability to tune material properties using gate electric field is at the heart of modern electronic technology. It is also a driving force behind recent advances in two-dimensional systems, such as gate-electric-field induced…

We calculate the ferroelectric polarization dynamics induced by a femtosecond midinfrared pulse as measured in the recent experiment by R. Mankowsky et al., Phys. Rev. Lett. 118, 197601 (2017). It is due to the nonlinear coupling of the…

Materials Science · Physics 2020-01-15 Veniamin A. Abalmasov

We report the optical perturbation of atomic arrangement in the layered GeTe/Sb_{2}Te_{3} phase change memory material. To observe the structural change, the coherent A_{1} mode of GeTe_{4} local structure is investigated at various…

Materials Science · Physics 2012-12-06 Kotaro Makino , Junji Tominaga , Alexander V. Kolobov , Paul Fons , Muneaki Hase

Two-dimensional (2D) multiferroic materials are ideal systems for exploring new coupling mechanisms between different ferroic orders and producing novel quantum phenomena with potential applications. We employed first-principles density…

Materials Science · Physics 2022-09-20 Weiwei Gao , Jijun Zhao , James R. Chelikowsky

We propose an efficient inverse design approach for multifunctional optical elements based on adaptive deep diffractive neural networks (a-D$^2$NNs). Specifically, we introduce a-D$^2$NNs and design two-layer diffractive devices that can…

Optics · Physics 2022-06-08 Yuyao Chen , Yilin Zhu , Wesley A. Britton , Luca Dal Negro

Two-dimensional (2D) layered ferroelectrics, as an emerging area of research, have attracted extensive attention, while memristors based on new 2D ferroelectric materials have yet to be fully explored, thereby limiting their applications in…

Two-dimensional (2D) multiferroics exhibit cross-control capacity between magnetic and electric responses in reduced spatial domain, making them well suited for next-generation nanoscale devices; however, progress has been slow in…

Materials Science · Physics 2020-05-15 Jing Shang , Chun Li , Aijun Du , Ting Liao , Yuantong Gu , Yandong Ma , Liangzhi Kou , Changfeng Chen

Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…

The symmetry breaking induced by the ferroelectric transition often triggers the emergence of topological electronic states such as Weyl fermions in ferroelectric-like metals/semimetals. Such strong coupling between the lattice deformation…

Materials Science · Physics 2022-04-14 Y. Okamura , H. Handa , R. Yoshimi , A. Tsukazaki , K. S. Takahashi , M. Kawasaki , Y. Tokura , Y. Takahashi

We report inelastic light scattering experiments on CaFe_2As_2 in the temperature range of 4 to 290 K. In in-plane polarizations two Raman-active phonon modes are observed at 189 and 211 cm-1, displaying A_1g and B_1g symmetries,…

Superconductivity · Physics 2009-11-13 K. -Y. Choi , D. Wulferding , P. Lemmens , N. Ni , S. L. Bud'ko , P. C. Canfield

Polaron formation following optical absorption is a key process that defines the photophysical properties of many semiconducting transition metal oxides, which comprise an important class of materials with potential optoelectronic and…

Materials Science · Physics 2022-11-11 Jacob L. Shelton , Kathryn E. Knowles