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The sign, magnitude, and range of the exchange couplings between pairs of Mn ions is determined for (Ga,Mn)N and (Ga,Mn)N:Si with x < 3%. The samples have been grown by metalorganic vapor phase epitaxy and characterized by secondary-ion…

Iridates abound with interesting magnetic behaviours because of their strong spin-orbit coupling. Sr$_3$NiIrO$_6$ brings together the spin-orbital entanglement of the Ir$^{4+}$ ion with a 3$d$ Ni cation and a one-dimensional crystal…

Materials Science · Physics 2018-10-19 Turan Birol , Kristjan Haule , David Vanderbilt

We probe the spectrum of elementary excitations in SrIrO$_3$ by using heterostructured [(SrIrO$_3$)$_m$/(SrTiO$_3$)$_l$] samples to approach the bulk limit. Our resonant inelastic x-ray scattering (RIXS) measurements at the Ir $L_3$-edge…

The magnetic excitations in electron doped (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ with $x = 0.03$ were measured using resonant inelastic X-ray scattering at the Ir $L_3$-edge. Although much broadened, well defined dispersive magnetic excitations…

Strongly Correlated Electrons · Physics 2016-06-15 Xuerong Liu , M. P. M. Dean , Z. Y. Meng , M. H. Upton , T. Qi , T. Gog , Y. Cao , J. Q. Lin , D. Meyers , H. Ding , G. Cao , H. P. Hill

Sr$_2$CuWO$_6$ is a double perovskite proposed to be at the border between two and three dimensional magnetism, with a square lattice of $S=\frac{1}{2}$ Cu$^{2+}$ ions. We have used inelastic neutron scattering to investigate the spin wave…

Strongly Correlated Electrons · Physics 2016-08-24 H. C. Walker , O. Mustonen , S. Vasala , D. T. Adroja , M. Karppinen

We report our investigation of the electronic and magnetic excitations of Sr$_3$NiIrO$_6$ by resonant inelastic x-ray scattering at the Ir L$_3$ edge. The intra-$t_{2g}$ electronic transitions are analyzed using an atomic model, including…

Strongly Correlated Electrons · Physics 2016-06-08 E. Lefrançois , A. -M. Pradipto , M. Moretti Sala , L. C. Chapon , V. Simonet , S. Picozzi , P. Lejay , S. Petit , R. Ballou

X-ray magnetic critical scattering measurements and specific heat measurements were performed on the perovskite iridate Sr$_3$Ir$_2$O$_7$. We find that the magnetic interactions close to the N\'{e}el temperature $T_N$ = 283.4(2) K are…

Strongly Correlated Electrons · Physics 2019-03-27 J. G. Vale , S. Boseggia , H. C. Walker , R. S. Springell , E. C. Hunter , R. S. Perry , S. P. Collins , D. F. McMorrow

We report a neutron scattering study of the magnetic order and dynamics of the bilayer perovskite Sr$_3$Fe$_2$O$_7$, which exhibits a temperature-driven metal-insulator transition at 340 K. We show that the Fe$^{4+}$ moments adopt…

The perovskite SrIrO3 is an exotic narrow-band metal owing to a confluence of the strengths of the spin-orbit coupling (SOC) and the electron-electron correlations. It has been proposed that topological and magnetic insulating phases can be…

Neutron diffraction, magnetization, resistivity, and heat capacity measurements on the 6H-perovskite Ba3BiRu2O9 reveal simultaneous magnetic and structural dimerization driven by strong magnetoelastic coupling. An isostructural but strongly…

Strongly Correlated Electrons · Physics 2015-06-03 Wojciech Miiller , Maxim Avdeev , Qingdi Zhou , Andrew J. Studer , Brendan J. Kennedy , Gordon J. Kearley , Chris D. Ling

We have used a combination of resonant magnetic x-ray scattering (RMXS) and x-ray absorption spectroscopy (XAS) to investigate the properties of the doped spin-orbital Mott insulator Sr2Ir(1-x)Rh(x)O4 (0.07 < x < 0.70). We show that…

Strongly Correlated Electrons · Physics 2014-02-12 J. P. Clancy , A. Lupascu , H. Gretarsson , Z. Islam , Y. F. Hu , D. Casa , C. S. Nelson , S. C. Lamarra , G. Cao , Young-June Kim

A three-orbital-model approach for studying spin wave excitations in the strongly spin-orbit coupled layered perovskite iridates is presented which provides a unified description of magnetic excitations as well as the electronic band…

Strongly Correlated Electrons · Physics 2017-04-05 Shubhajyoti Mohapatra , Jeroen van den Brink , Avinash Singh

Resonant inelastic X-ray scattering (RIXS) experiments performed at the oxygen-$K$ edge on the iridate perovskites {\SIOS} and {\SION} reveal a sequence of well-defined dispersive modes over the energy range up to $\sim 0.8$ eV. The…

Sr$_2$FeOsO$_6$ is an insulating double perovskite compound which undergoes antiferromagnetic transitions at 140 K ($T_{N1}$) and 67 K ($T_{N2}$). To study the underlying electronic and magnetic interactions giving rise to this behavior we…

Spin excitations are explored in the electron-doped spin-orbit Mott insulator (Sr$_{1-x}$La$_{x}$)$_3$Ir$_2$O$_7$. As this bilayer square lattice system is doped into the metallic regime, long-range antiferromagnetism vanishes, yet a…

Strongly Correlated Electrons · Physics 2016-09-14 Tom Hogan , Rebecca Dally , Mary Upton , J. P. Clancy , Kenneth Finkelstein , Young-June Kim , M. J. Graf , Stephen D. Wilson

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

Strongly Correlated Electrons · Physics 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

We have studied the magnetic excitations of electron-doped Sr$_{2-x}$La$_x$IrO$_4$ ($0 \leq x \leq 0.10$) using resonant inelastic x-ray scattering (RIXS) at the Ir L$_3$-edge. The long range magnetic order is rapidly lost with increasing…

Perovskite-type iridates SrIrO$_{3}$ and CaIrO$_{3}$ are a Dirac line node semimetal protected by crystalline symmetry, providing an interesting playground to investigate electron correlation effects on topological semimetals. The effect of…

Strongly Correlated Electrons · Physics 2019-11-14 Masamichi Negishi , Naoka Hiraoka , Daisuke Nishio-Hamane , Hidenori Takagi

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

Strongly Correlated Electrons · Physics 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

The collective magnetic excitations in the spin-orbit Mott insulator (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ ($x=0,\,0.01,\,0.04,\, 0.1$) were investigated by means of resonant inelastic x-ray scattering. We report significant magnon energy gaps at…

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