Related papers: Precise measurement of the Kerr coefficient using …
In Ref. [Phys. Rev. A 108, 053708], the scheme of quantum non-demolition measurement of optical quanta that uses a resonantly enhanced Kerr nonlinearity in the optical microresonator, pre-squeezing of the probe beam, and its parametric…
For astronomical instruments, accurate knowledge of the optical pointing and coupling are essential to characterize the alignment and performance of (sub-)systems prior to integration and deployment. Ideally, this requires the phase…
We analytically investigate the sensitivity of Kerr nonlinear phase estimation in a Mach-Zehnder interferometer with two-mode squeezed vacuum states. We find that such a metrological scheme could access a sensitivity scaling over the Boixo…
Pump-probe spectroscopy is central for exploring ultrafast dynamics of fundamental excitations, collective modes and energy transfer processes. Typically carried out using conventional diffraction-limited optics, pump-probe experiments…
A theory of pump-probe spectroscopy is developed in which optical fields drive two-photon Raman transitions between ground states of an ensemble of three-level $\Lambda $ atoms. Effects related to the recoil the atoms undergo as a result of…
Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…
Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…
Control of optical properties of materials by tuning their refractive index can revolutionize the current state-of-the-art technology to manipulate light propagation in the high loss media. Here we demonstrate active optical tuning of the…
Attosecond nonlinear Fourier transform (NFT) pump probe spectroscopy is an experimental technique which allows investigation of the electronic excitation, ionization, and unimolecular dissociation processes. The NFT spectroscopy utilizes…
Nonlinear spectroscopy is widely used to study the transient dynamics of molecules under strong light-matter coupling, though it remains unclear to what extent uncoupled intracavity molecules obscure signals from the strongly-coupled…
Strong nonlinearity at the single photon level represents a crucial enabling tool for optical quantum technologies. Here we report on experimental implementation of a strong Kerr nonlinearity by measurement-induced quantum operations on…
Photoluminescence spectroscopy of single InAs quantum dots at cryogenic temperatures (~14 K) is performed using a micron-scale optical fiber taper waveguide as a near-field optic. The measured collection efficiency of quantum dot…
High-power optical pulses experience self-focusing when propagating in a gaseous medium due to the manifestation of the cubic (Kerr-like) nonlinearity. The magnitude of this effect depends on the Kerr nonlinearity coefficient n2, which in…
We describe a pump-probe scheme with which the spatial asymmetry of dissociating molecular fragments --- as controlled by the carrier-envelope phase of an intense few-cycle laser pulse --- can be enhanced by an order of magnitude or more.…
Hyperspectral imaging provides spatially resolved spectral information. Utilising dual frequency combs as active illumination sources, hyperspectral imaging with ultra-high spectral resolution can be implemented in a scan-free manner when a…
We describe bichromatic superradiant pump-probe spectroscopy as a tomographic probe of the Wigner function of a dispersing particle beam. We employed this technique to characterize the quantum state of an ultracold atomic beam, derived from…
In this work we extend low frequency impulsive stimulated Raman microspectroscopy to the pre-electronic resonance regime. We use a broadband two color collinear pump probe scheme which can be readily extended to imaging. We discuss the…
Combined microwave-optical pump-probe methods are emerging to study the quantum state of spin qubit centers and the charge dynamics in semiconductors. A major hindrance is the limited bandwidth of microwave irradiation/detection circuitry…
Atomic vapors are systems well suited for nonlinear optics studies but very few direct measurements of their nonlinear refractive index have been reported. Here we use the z-scan technique to measure the Kerr coefficient, $n_2$, for a Cs…
Vacuum birefringence is one of the most striking predictions of strong field quantum electrodynamics: Probe photons traversing a strong field region can indirectly sense the applied "pump" electromagnetic field via quantum fluctuations of…