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We investigate the prospects of using two-mode intensity squeezed twin-beams, generated in Rb vapor, to improve the sensitivity of spectroscopic measurements by engaging two-photon Raman transitions. As a proof of principle demonstration,…

Atomic Physics · Physics 2021-04-21 Nikunjkumar Prajapati , Ziqi Niu , Irina Novikova

Photonic quantum technologies rely on the efficient generation and interference of indistinguishable photons. Exceptional achievements in this respect have been obtained by domain engineering of quasi-phase-matched parametric…

Optical pump-probe spectroscopy is a powerful tool for the study of non-equilibrium electronic dynamics and finds wide applications across a range of fields, from physics and chemistry to material science and biology. However, a shortcoming…

We study a nonlinear interferometer consisting of two consecutive parametric amplifiers, where all three optical fields (pump, signal and idler) are treated quantum mechanically, allowing for pump depletion and other quantum phenomena. The…

Quantum Physics · Physics 2018-12-27 Jefferson Flórez , Enno Giese , Davor Curic , Lambert Giner , Robert W. Boyd , Jeff S. Lundeen

Quantum metrology employs quantum resources to achieve measurement precision beyond classical limits. This work investigates a Mach--Zehnder interferometer incorporating a Kerr nonlinear phase shifter, with photon-added two-mode squeezed…

Quantum Physics · Physics 2026-02-20 Zekun Zhao , Qingqian Kang , Teng Zhao , Cunjin Liu , Xin Su , Liyun Hu

Ultrafast pump-probe spectroscopy is a powerful tool to study the nonequilibrium dynamics in high-Tc cuprate superconductors. The photo-induced quasiparticle (QP) dynamics revealed by pump-probe spectroscopy are sensitive to the near-Fermi…

Superconductivity · Physics 2015-06-22 Wei Li , Chunfeng Zhang , Xiaoyong Wang , Jak Chakhalian , Min Xiao

The accuracy of quantum measurements can be effectively improved by using both photon-added non-Gaussian operations and Kerr nonlinear phase shifters. Here, we employ coherent state mixed photon-added squeezed vacuum state as input into a…

Quantum Physics · Physics 2025-05-23 Zekun Zhao , Qingqian Kang , Shoukang Chang , Teng Zhao , Cunjin Liu , Xin Su , Liyun Hu

We numerically analyze the use of intense entangled twin beams for ultra-sensitive spectroscopic measurements in chemical and biological systems. The examined scheme makes use of intense frequency-modulated (chirped) entangled beams to…

Quantum Physics · Physics 2018-05-16 Jiří Svozilík , Jan Peřina , Roberto de J. León-Montiel

Optical pump-probe spectroscopy is a powerful tool to directly probe the carrier dynamics in materials down to sub-femtosecond resolution. To perform such measurement, while keeping the pump induced perturbation to the sample as small as…

We report here an experimental setup to perform three-pulse pump-probe measurements over a wide wavelength and temperature range. By combining two pump pulses in the visible (650-900 nm) and mid-IR (5-20 $\mu$m) range, with a broadband…

We propose a simple method to measure nonlinear Kerr refractive index in mid-infrared frequency range that avoids using sophisticated infrared detectors. Our approach is based on using a near-infrared probe beam which interacts with a…

Optics · Physics 2023-10-10 Dusan Lorenc , Zhanybek Alpichshev

Deeply sub-wavelength two-dimensional films may exhibit extraordinarily strong nonlinear effects. Here we show that 2D films exhibit the remarkable property of a phase-controllable nonlinearity, i.e., the amplitude of the nonlinear…

We mainly investigate the quantum measurement of Kerr nonlinearity in the driven-dissipative system. Without the dissipation, the measurement precision of the nonlinearity parameter $\chi$ scales as "super-Heisenberg scaling" $1/N^2$ with…

Quantum Physics · Physics 2022-09-22 Dong Xie , Chunling Xu , An Min Wang

The development of new quantum light sources requires robust and convenient methods of characterizing their joint spectral properties. Measuring the joint spectral intensity between a photon pair ignores any correlations in spectral phase…

Quantum Physics · Physics 2020-12-02 Bryn A. Bell , Gil Triginer Garces , Ian A. Walmsley

Two-photon loss mechanisms often accompany a Kerr nonlinearity. The kinetic inductance exhibited by superconducting transmission lines provides an example of a Kerr-like nonlinearity that is accompanied by a nonlinear resistance of the…

Quantum Physics · Physics 2009-11-11 Bernard Yurke , Eyal Buks

Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

Recent years have seen the development of quantum sensing concepts utilizing nonlinear interferometers based on correlated photon pairs generated by spontaneous parametric down-conversion (SPDC). Using SPDC far from frequency degeneracy…

Quantum Physics · Physics 2022-08-17 Chiara Lindner , Jachin Kunz , Simon J. Herr , Jens Kiessling , Sebastian Wolf , Frank Kühnemann

In this work quantum metrology techniques are applied to the imaging of objects with a non-uniform refractive spatial profile. A sensible improvement on the classical accuracy is shown to be found when the "Twin Beam State" (TWB) is used.…

Optics · Physics 2020-09-21 Giuseppe Ortolano , Ivano Ruo Berchera , Enrico Predazzi

Intense spatio-spectral twin beams generated in the regime with pump depletion are analyzed applying a suggested quantum model that treats the signal, idler and pump fields in the same way. The model assumes the signal and idler fields in…

Quantum Physics · Physics 2017-09-26 Jan Perina

We describe an ultrafast time resolved pump-probe spectroscopy setup aimed at studying the switching of nanophotonic structures. Both fs pump and probe pulses can be independently tuned over broad frequency range between 3850 and 21050…

Optics · Physics 2010-11-02 Tijmen G. Euser , Philip J. Harding , Willem L. Vos