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A neuroevolution potential (NEP) for the ternary $\alpha$-Fe--C--H system was developed based on a database generated from spin-polarized density functional theory (DFT) calculations, achieving empirical potential efficiency with DFT…

Materials Science · Physics 2025-10-23 Fan-Shun Meng , Shuhei Shinzato , Zhiqiang Zhao , Jun-Ping Du , Lei Gao , Zheyong Fan , Shigenobu Ogata

We introduce DeepDFT, a deep learning model for predicting the electronic charge density around atoms, the fundamental variable in electronic structure simulations from which all ground state properties can be calculated. The model is…

Computational Physics · Physics 2020-11-09 Peter Bjørn Jørgensen , Arghya Bhowmik

In high energy density physics (HEDP) and inertial confinement fusion (ICF), predictive modeling is complicated by uncertainty in parameters that characterize various aspects of the modeled system, such as those characterizing material…

The concept of the effective one-electron potentials (OEP) has been useful for many decades in efficient description of electronic structure of chemical systems, especially extended molecular aggregates such as interacting molecules in…

Chemical Physics · Physics 2020-02-04 Bartosz Błasiak , Joanna D. Bednarska , Marta Chołuj , Wojciech Bartkowiak

We present an evaluation of CSP-MACE-{\AA}, a machine learning interatomic potential intended to replace DFT in crystal structure prediction (CSP). We decompose the total energy into separate intramolecular and intermolecular components.…

Constant potential methods (CPM) enable computationally efficient simulations of the solid-liquid interface at conducting electrodes in molecular dynamics (MD). They have been successfully used, for example, to realistically model the…

Chemical Physics · Physics 2022-07-29 Ludwig J. V. Ahrens-Iwers , Mathijs Janssen , Shern R. Tee , Robert H. Meißner

The quality, consistency, and information content of training data is often what determines the practical value of machine-learning models for atomistic simulations. Yet, many widely used electronic-structure databases are assembled having…

The rapid development of computational materials science powered by machine learning (ML) is gradually leading to solutions to several previously intractable scientific problems. One of the most prominent is machine learning interatomic…

Materials Science · Physics 2025-05-27 Xiao Fu , Jing Xu , Qifan Yang , Xuhe Gong , Jingchen Lian , Liqi Wang , Zibin Wang , Ruijuan Xiao , Hong Li

A machine learning (ML) based equivariant neural network for constructing distributed charge models (DCMs) of arbitrary resolution, DCM-net, is presented. DCMs efficiently and accurately model the anisotropy of the molecular electrostatic…

Chemical Physics · Physics 2026-02-10 Eric D. Boittier , Markus Meuwly

In molecular simulations, neural network force fields aim at achieving \emph{ab initio} accuracy with reduced computational cost. This work introduces enhancements to the Deep Potential network architecture, integrating a message-passing…

Computational Physics · Physics 2024-04-09 Ruiqi Gao , Yifan Li , Roberto Car

Machine learning assisted modeling of the inter-atomic potential energy surface (PES) is revolutionizing the field of molecular simulation. With the accumulation of high-quality electronic structure data, a model that can be pretrained on…

Chemical Physics · Physics 2023-09-18 Duo Zhang , Hangrui Bi , Fu-Zhi Dai , Wanrun Jiang , Linfeng Zhang , Han Wang

Electrical properties (EPs) of tissues, conductivity and permittivity, are modulated by the ionic and water content, which change in presence of pathologies. Information on tissues EPs can be used e.g. as an endogenous biomarker in…

Progress in machine learning has facilitated the development of potentials that offer both the accuracy of first-principles techniques and vast increases in the speed of evaluation. Recently,"$\Delta$-machine learning" has been used to…

We propose a machine-learning-based (ML-based) method for efficiently predicting atomic diffusivity in crystals, in which the potential energy surface (PES) of a diffusion carrier is partially evaluated by first-principles calculations. To…

Materials Science · Physics 2020-06-24 Kazuaki Toyoura , Takeo Fujii , Kenta Kanamori , Ichiro Takeuchi

Computational modeling is an integral part of catalysis research. With it, new methodologies are being developed and implemented to improve the accuracy of simulations while reducing the computational cost. In particular, specific…

Materials Science · Physics 2024-08-28 Alexandre Boucher , Cameron Beevers , Bertrand Gauthier , Alberto Roldan

In this study, we propose to adopt a novel framework, Knowledge-integrated Machine Learning, for advancing Proton Exchange Membrane Water Electrolysis (PEMWE) development. Given the significance of PEMWE in green hydrogen production and the…

Machine Learning · Computer Science 2024-04-08 Xia Chen , Alexander Rex , Janis Woelke , Christoph Eckert , Boris Bensmann , Richard Hanke-Rauschenbach , Philipp Geyer

Reliable detection of event-related potentials (ERPs) at the single-trial level remains a major challenge due to the low signal-to-noise ratio EEG recordings. In this work, we investigate whether incorporating prior knowledge about ERP…

Signal Processing · Electrical Eng. & Systems 2026-03-24 Marek Zylinski , Bartosz Tomasz Smigielski , Gerard Cybulski

High-fidelity electron microscopy simulations required for quantitative crystal structure refinements face a fundamental challenge: while physical interactions are well-described theoretically, real-world experimental effects are…

A crucial aspect in the simulation of electrochemical interfaces consists in treating the distribution of electronic charge of electrode materials that are put in contact with an electrolyte solution. Recently, it has been shown how a…

Materials Science · Physics 2024-07-16 Andrea Grisafi , Mathieu Salanne

Quantum-mechanically-driven charge polarization and charge transfer are ubiquitous in biomolecular systems, controlling reaction rates, allosteric interactions, ligand-protein binding, membrane transport, and dynamically-driven structural…

Chemical Physics · Physics 2021-06-09 Susan R. Atlas