Related papers: Enhanced enantiomer discrimination with chiral sur…
We study the excitation of asymmetric-top (including chiral) molecules by two-color femtosecond laser pulses. In the cases of non-chiral asymmetric-top molecules excited by an orthogonally polarized two-color pulse, we demonstrate,…
Chiroptical enantioselective sensing is gaining traction across various applications. However, intrinsic molecular chiroptical responses are weak, and existing amplification approaches add synthesis, manufacturing, or operational complexity…
Plasmonic fields are usually considered non-chiral because of the transverse magnetic polarization of surface plasmon modes. We however show here that an optical lattice created from the intersection of two coherent surface plasmons…
Most large molecules are chiral in their structure: they exist as two enantiomers, which are mirror images of each other. Whereas the rovibronic sublevels of two enantiomers are almost identical, it turns out that the photoelectric effect…
Fine control of the chiral light-matter interaction at the nanoscale, by exploiting designed metamaterial architecture, represents a cutting-edge craft in the field of biosensing, quantum and classic nanophotonics. Recently, artificially…
Enantio-conversion with the help of electromagnetic fields is an essential issue due to the chirality-dependence of many chemical, biological, and pharmaceutical processes. Here, we propose a method for this issue based on a five-level…
Coupling between light and material excitations underlies a wide range of optical phenomena. Polaritons are eigenstates of a coupled system with hybridized wave function. Owing to their hybrid composition, polaritons exhibit at the same…
Spin-dependent, directional light-matter interactions form the basis of chiral quantum networks. In the solid state, quantum emitters commonly possess circularly polarised optical transitions with spin-dependent handedness. We demonstrate…
We introduce meta-diastereomers, hybrid systems where molecular chirality ($\leq 10$\,nm) and nanoscale chirality ($>100$\,nm) combine to create a new hierarchical chiral state with emergent optical properties. By coupling chiral…
We present a comprehensive study of enantioselective orientation of chiral molecules excited by a pair of delayed cross-polarized femtosecond laser pulses. We show that by optimizing the pulses' parameters, a significant (~ 10%) degree of…
Two-dimensional lattices of chiral nanoholes in a plasmonic film with lattice constants being slightly larger than light wavelength are proposed for effective control of polarization and spatial properties of light beams. Effective…
Unidirectional (chiral) emission of light from a circular dipole emitter into a waveguide is only possible at points of perfect circular polarisation (C points), with elliptical polarisations yielding a lower directional contrast. However,…
We introduce and theoretically analyze the concept of manipulating optical chirality via strong coupling of the optical modes of chiral nanostructures with excitonic transitions in molecular layers or semiconductors. With chirality being…
Conventional optical materials are characterized by either a dissipative response, which results in polarization-independent absorption, or by a gain response that leads to wave amplification. In this work, we study a peculiar class of…
A simple yet effective achiral platform using elliptical nanoholes for chiroptical analysis is demonstrated. Under linearly polarized excitation, an elliptical nanohole in a thin gold film can generate a localized chiral optical field for…
Controlling optical chirality at the subwavelength scales is essential for many applications of nanophotonic structures in polarization optics, sensing, and nonlinear photonics. Achieving a strong chiroptical response in planar dielectric…
Detection of chiral molecules requires amplification of chirality to measurable levels. Typically, amplification mechanisms are considered at the microscopic scales of individual molecules and their aggregates. Here we demonstrate chirality…
We propose a novel high resolution microscopy technique for enantio-specific detection of chiral samples down to sub-100 nm size, based on force measurement. We delve into the differential photo-induced optical force exerted on an achiral…
Topological photonic structures exhibit chiral edge states that are robust to disorder and sharp bends. When coupled to quantum emitters, these edge states generate directional light emission that enables unprecedented control of…
Developing effective methods to measure the enantiomeric excess of the chiral mixture is one of the major topics in chiral molecular researches, yet remains challenging. Enantiodetection method via two-dimensional (2D) spectroscopy based on…