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Simulations of colloidal suspensions consisting of mesoscopic particles and smaller species such as ions or depletants are computationally challenging as different length and time scales are involved. Here, we introduce a machine learning…

Soft Condensed Matter · Physics 2021-12-01 Gerardo Campos-Villalobos , Emanuele Boattini , Laura Filion , Marjolein Dijkstra

The melting of a binary system of charged particles confined in a {\it quasi}-one-dimensional parabolic channel is studied through Monte Carlo simulations. At zero temperature the particles are ordered in parallel chains. The melting is…

Soft Condensed Matter · Physics 2015-05-19 W. P. Ferreira , G. A. Farias , F. M. Peeters

Ultracold polar molecules in multilayered systems have been experimentally realized very recently. While experiments study these systems almost exclusively through their chemical reactivity, the outlook for creating and manipulating exotic…

Quantum Physics · Physics 2013-04-19 A. G. Volosniev , J. R. Armstrong , D. V. Fedorov , A. S. Jensen , N. T. Zinner

We study a chemical gelation model in two dimensions which includes both monomer aggregations and bond fluctuations. Our numerical simulation shows that a sol-gel transition occurs when an initial monomer concentration is above a critical…

Soft Condensed Matter · Physics 2007-05-23 Kenji Ohira , Masatoshi Sato , Mahito Kohmoto

We investigate the heterogeneous dynamics in a model, where chemical gelation and glass transition interplay, focusing on the dynamical susceptibility. Two independent mechanisms give raise to the correlations, which are manifested in the…

Soft Condensed Matter · Physics 2017-05-09 Antonio de Candia , Annalisa Fierro , Raffaele Pastore , Massimo Pica Ciamarra , Antonio Coniglio

We develop coarse-grained particle approaches for studying the elastic mechanics of vesicles with heterogeneous membranes having phase-separated domains. We perform simulations both of passive shape fluctuations and of active systems where…

Soft Condensed Matter · Physics 2023-02-28 David A. Rower , Paul J. Atzberger

We have investigated the rheology and structure of a gel formed from a mixture of non-Brownian particles and two immiscible liquids. The suspension of particles in a liquid undergoes gelation upon the addition of a small content of second,…

Soft Condensed Matter · Physics 2020-04-27 Sameer Huprikar , Saurabh Usgaonkar , Ashish K. Lele , Ashish V. Orpe

We discuss a class of models for particulate gels in which the particle contacts are described by an effective interaction combining a two-body attraction and a three-body angular repulsion. Using molecular dynamics, we show how varying the…

Soft Condensed Matter · Physics 2021-08-05 Minaspi Bantawa , Wayan A. Fontaine-Seiler , Peter D. Olmsted , Emanuela Del Gado

Rigidity percolation (RP) occurs when mechanical stability emerges in disordered networks as constraints or components are added. Here we discuss RP with structural correlations, an effect ignored in classical theories albeit relevant to…

Soft Condensed Matter · Physics 2019-08-07 Shang Zhang , Leyou Zhang , Mehdi Bouzid , D. Zeb Rocklin , Emanuela Del Gado , Xiaoming Mao

Colloidal dispersions are prized as model systems to understand basic properties of materials, and are central to a wide range of industries from cosmetics to foods to agrichemicals. Among the key developments in using colloids to address…

Soft Condensed Matter · Physics 2022-06-22 Jun Dong , Francesco Turci , Robert L. Jack , Malcolm A. Faers , C. Patrick Royall

Colloidal gel aging is investigated using very long runs of brownian dynamics simulations. The Asakura Oosawa description of the depletion interaction is used to model a simple colloid polymer mixture. Several regimes are identified during…

Soft Condensed Matter · Physics 2009-11-07 Rodolphe J. M. d'Arjuzon , William Frith , John R. Melrose

Motivated by recent experimental findings in chemical synthesis of colloidal particles, we draw an analogy between self-assembly processes occurring in biological systems (e.g. protein folding) and a new exciting possibility in the field of…

Soft Condensed Matter · Physics 2018-02-14 Achille Giacometti

We show that mixing a colloidal gel with larger, non-Brownian grains generates novel flow-switched bistability. Using a combination of confocal microscopy and rheology, we find that prolonged moderate shear results in liquefaction by…

Soft Condensed Matter · Physics 2023-05-17 Yujie Jiang , Soichiro Makino , John R. Royer , Wilson C. K. Poon

We investigate the phase behaviour of a two-dimensional colloidal model system of ultra-soft particles on a substrate which varies periodically along one spatial direction. Our calculations are based on mean-field density functional theory…

Soft Condensed Matter · Physics 2021-03-17 Alexander Kraft , Sabine H. L. Klapp

In this Rapid Communication we demonstrate the applicability of an augmented Gibbs ensemble Monte Carlo approach for the phase behavior determination of model colloidal systems with short-ranged depletion attraction and long-ranged…

Soft Condensed Matter · Physics 2007-05-23 P. Charbonneau , D. R. Reichman

Recent advances have shown that introducing dependency interactions between two superconducting networks can trigger abrupt, hysteretic normal-superconductor phase transitions. In this study, we demonstrate that such behavior can also arise…

The formation of colloidal gels is strongly dependent on the volume fraction of the system and the strength of the interactions between the colloids. Here we explore very dilute solutions by the means of numerical simulations, and show…

Soft Condensed Matter · Physics 2017-09-13 Samuel Griffiths , Francesco Turci , C. Patrick Royall

We report a computer simulation study of a model gel-former obtained by modifying the three-body interactions of the Stillinger-Weber potential for silicon. This modification reduces the average coordination number and consequently shifts…

Disordered Systems and Neural Networks · Physics 2015-05-27 Shibu Saw , Niels L. Ellegaard , Walter Kob , Srikanth Sastry

We present a density-functional study of a binary phase-separating mixture of soft core particles immersed in a random matrix of quenched soft core particles of larger size. This is a model for a binary polymer mixture immersed in a…

Soft Condensed Matter · Physics 2007-05-23 A. J. Archer , M. Schmidt , R. Evans

We here discuss the results of 3d MonteCarlo simulations of a minimal lattice model for gelling systems. We focus on the dynamics, investigated by means of the time autocorrelation function of the density fluctuations and the particle mean…

Soft Condensed Matter · Physics 2007-05-23 E. Del Gado , A. Fierro , L. de Arcangelis , A. Coniglio