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Collisional effects can play an essential role in the dynamics of plasma waves by setting a minimum damping rate and by interfering with wave-particle resonances. Kinetic simulations of the effects of electron-ion pitch angle scattering on…

Plasma Physics · Physics 2016-03-23 J. W. Banks , S. Brunner , R. L. Berger , T. M. Tran

Including quantum mechanical effects on the dynamics of nuclei in the condensed phase is challenging, because the complexity of exact methods grows exponentially with the number of quantum degrees of freedom. Efforts to circumvent these…

Chemical Physics · Physics 2015-06-23 Mariana Rossi , Hanchao Liu , Francesco Paesani , Joel Bowman , Michele Ceriotti

Atom probe tomography data is composed of a list of coordinates of the reconstructed atoms in the probed volume. The elemental identity of each atom is derived from time-of-flight mass spectrometry, with no local energetic or chemical…

The kinetic damping mechanism of low frequency transverse perturbations propagating parallel to the magnetic field in a magnetized warm electron plasma is simulated by means of electromagnetic (EM) Vlasov simulations. The short-time-scale…

Plasma Physics · Physics 2022-10-26 Anjan Paul , Devendra Sharma

We present low-energy electron diffraction (LEED) as elastic electron-atom scattering (EEAS) operating in a target crystal waveguide where a Coulombic carrier wave is wavenumber modulated by exchange-correlation (XC) interaction. Carrier…

Materials Science · Physics 2021-06-10 John Rundgren , Bo E. Sernelius , Wolfgang Moritz

The atomistic resolution recently achieved by ultrafast spectroscopies demands corresponding theoretical advances. Real-time time-dependent density-functional theory (RT-TDDFT) with Ehrenfest dynamics offers an optimal trade-off between…

Materials Science · Physics 2022-10-19 Jannis Krumland , Matheus Jacobs , Caterina Cocchi

1-D Eulerian Vlasov-Maxwell simulations are presented which show kinetic enhancement of stimulated Raman backscatter (SRBS) due to electron trapping in regimes of heavy linear Landau damping. The conventional Raman Langmuir wave is…

Plasma Physics · Physics 2012-11-13 David J. Strozzi , Ed A. Williams , A. Bruce Langdon , Abraham Bers

We theoretically investigate electron energy loss spectroscopy (EELS) of metallic nanoparticles in the optical frequency domain. Using a quasistatic approximation scheme together with a plasmon eigenmode expansion, we show that EELS can be…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Anton Hörl , Andreas Trügler , Ulrich Hohenester

A fully kinetic simulation approach, treating each plasma component based on the Vlasov equation, is adopted to study the disintegration of an initial density perturbation (IDP) into a number of ion-acoustic solitary waves (IASWs) in the…

Plasma Physics · Physics 2016-10-06 S. M. Jenab , F. Spanier

High energy electron beams can now be routinely focused to 1-2 {\AA} and offer the ability to obtain vibrational information from materials using monochromated electron energy-loss spectroscopy (EELS) in a scanning transmission electron…

Materials Science · Physics 2021-07-13 Kartik Venkatraman , Peter A. Crozier

An analytic description of laser-assisted electron-atom scattering (LAES) in an elliptically polarized field is presented using time-dependent effective range (TDER) theory to treat both electron-laser and electron-atom interactions…

Atomic Physics · Physics 2015-06-12 A. V. Flegel , M. V. Frolov , N. L. Manakov , Anthony F. Starace , A. N. Zheltukhin

Scanning transmission electron microscopy (STEM) combined with electron energy loss spectroscopy (EELS) has become a standard technique to map localized surface plasmon resonances with a nanometer spatial and a sufficient energy resolution…

Mesoscale and Nanoscale Physics · Physics 2020-06-02 Michal Horák , Tomáš Šikola

Recently, two reports have demonstrated the amazing possibility to probe vibrational excitations from nanoparticles with a spatial resolution much smaller than the corresponding free-space phonon wavelength using electron energy loss…

Materials Science · Physics 2017-12-13 Hugo Lourenço-Martins , Mathieu Kociak

A new analysis method has been developed for measurements of broadband, low-amplitude turbulent electron temperature fluctuations in fusion plasmas using individual radiometer channels of a Correlation Electron Cyclotron Emission (CECE)…

The underlying dielectric properties of materials, intertwined with intriguing phenomena such as topological polariton modes and anisotropic thermal conductivities, stem from the anisotropy in atomic vibrations. Conventionally, X-ray…

Electron energy-loss spectroscopy (EELS) and cathodoluminescence (CL) are widely used experimental techniques for characterization of nanoparticles. The discrete dipole approximation (DDA) is a numerically exact method for simulating…

Optics · Physics 2023-03-03 Alexander A. Kichigin , Maxim A. Yurkin

Electron energy loss spectroscopy (EELS) can be used to probe plasmon excitations in nanostructured materials with atomic-scale spatial resolution. For structures smaller than a few nanometers quantum effects are expected to be important,…

Mesoscale and Nanoscale Physics · Physics 2013-01-03 Kirsten Andersen , Karsten W. Jacobsen , Kristian S. Thygesen

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

We theoretically investigated electron energy loss spectroscopy (EELS) of ultraviolet surface plasmon modes in aluminum nanodisks. Using full-wave simulations, we studied the impact of diameter on the resonant modes of the nanodisks. We…