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Van der Waals heterostructures assembled from layers of 2D materials have attracted considerable interest due to their novel optical and electrical properties. Here we report a scattering-type scanning near field optical microscopy study of…

Atomic-level defects in van der Waals (vdW) materials are essential building blocks for quantum technologies and quantum sensing applications. The layered magnetic semiconductor CrSBr is an outstanding candidate for exploring optically…

Recently, the two-dimensional magnetic semiconductor CrSBr has attracted considerable attention due to its excellent air-stable property and high magnetic critical temperature. Here, we systematically investigate the electronic structure,…

Materials Science · Physics 2022-08-10 Xiuxian Yang , Ping Yang , Xiaodong Zhou , Wanxiang Feng , Yugui Yao

Monolayer and few-layer phosphorene are anisotropic quasi-two-dimensional (quasi-2D) van der Waals (vdW) semiconductors with a linear-dichroic light-matter interaction and a widely-tunable direct-band gap in the infrared frequency range.…

We report temperature-dependent reflectivity spectra of the layered van der Waals magnet CrSBr in the far-infrared region. Polarization-dependent measurements resolve the vibrational modes along the E$\|a$- and $b$-axes and reveal the clear…

Materials Science · Physics 2025-05-27 E. Uykur , A. A. Tsirlin , F. Long , M. Wenzel , M. Dressel , K. Mosina , Z. Sofer , M. Helm , S. Zhou

W-band ({\nu} ca. 94 GHz) electron paramagnetic resonance (EPR) spectroscopy was used for a single-crystal study of a star-shaped Fe3Cr single-molecule magnet (SMM) with crystallographically imposed trigonal symmetry. The high resolution…

Mesoscale and Nanoscale Physics · Physics 2013-09-13 L. Sorace , M. -E. Boulon , P. Totaro , A. Cornia , J. Fernandes-Soares , R. Sessoli

The van der Waals magnetic semiconductor CrSBr combines multistable magnetic order with strong light--matter coupling, enabling optical access to a rich and reconfigurable layered magnetic domain structure. A purely optical,…

The crystalline and optical anisotropy of low-symmetry two-dimensional (2D) materials can enable strong dichroic responses, enhancing polarization contrast for photonic and optoelectronic devices. Here, we unveil pronounced optical and…

Mesoscale and Nanoscale Physics · Physics 2026-05-18 Cédric A. Cordero-Silis , Daniel Vaquero , Teresa López-Carrasco , Harshan Madeshwaran , Marcos H. D. Guimarães

Excitons are fundamental excitations that govern the optical properties of semiconductors. Interacting excitons can lead to various emergent phases of matter and large nonlinear optical responses. In most semiconductors, excitons interact…

Magnetism in two-dimensional materials reveals phenomena distinct from bulk magnetic crystals, with sensitivity to charge doping and electric fields in monolayer and bilayer van der Waals magnet CrI3. Within the class of layered magnets,…

Tailoring magnetoresistance and magnetic anisotropy in van der Waals magnetic materials is essential for advancing their integration into technological applications. In this regard, strain engineering has emerged as a powerful and versatile…

Chromium thiophosphate (CrPS4), a monoclinic crystal of C_2^3 space group, is a ternary layered semiconductor with an optical bandgap of 1.4 eV and exhibits antiferromagnetism below 36 K. Despite its potential in optoelectronic and magnetic…

Chemical Physics · Physics 2021-07-16 Sujin Kim , Jinhwan Lee , Changgu Lee , Sunmin Ryu

Optical properties in van der Waals heterostructures based on monolayer transition-metal dichalcogenides (TMDs), are often dominated by excitonic transitions. While intrinsic spin-orbit coupling (SOC) and an isotropic band structure are…

Mesoscale and Nanoscale Physics · Physics 2024-02-07 Jiayu David Cao , Gaofeng Xu , Benedikt Scharf , Konstantin Denisov , Igor Zutic

The detection and manipulation of the spin configurations in layered magnetic semiconductors hold significant interest for developing spintronic devices in two-dimensional limit. In this letter, we report a systematical study on the…

Mesoscale and Nanoscale Physics · Physics 2025-08-01 Xiaohua Wu , Junyang Chen , Mingqiang Gu , Yujun Zhang , Shanmin Wang , Yanan Dai , Qihang Liu , Yue Zhao , Mingyuan Huang

Graphene is a privileged 2D platform for hosting confined light-matter excitations known as surface plasmon-polaritons (SPPs), as it possesses low intrinsic losses with a high degree of optical confinement. However, the inherently isotropic…

Van der Waals magnetic materials are an ideal platform to study low-dimensional magnetism. Opposed to other members of this family, the magnetic semiconductor CrSBr is highly resistant to degradation in air, which, besides its exceptional…

Polymorphism, commonly denoting the variety of molecular or crystal structures, is a vital element in many natural science disciplines. In van der Waals layered antiferromagnets, a new type of magnetic polymorphism is allowed by having…

Mesoscale and Nanoscale Physics · Physics 2024-10-07 Zeyuan Sun , Canyu Hong , Yi Chen , Zhiyuan Sheng , Shuang Wu , Zhanshan Wang , Bokai Liang , Wei-Tao Liu , Zhe Yuan , Yizheng Wu , Qixi Mi , Zhongkai Liu , Jian Shen , Shiwei Wu

Light-matter coupling in van der Waal's materials holds significant promise in realizing Bosonic condensation and superfluidity. The underlying semiconductor's crystal asymmetry, if any, can be utilized to form anisotropic half-light…

Among a huge variety of known two-dimensional materials, some of them have anisotropic crystal structures; examples include so different systems as a few-layer black phoshphorus (phosphorene), beryllium nitride BeN$_4$, van der Waals magnet…

Materials Science · Physics 2024-08-30 Alexander N. Rudenko , Mikhail I. Katsnelson

The two-dimensional character of van der Waals magnets allows for efficient control of their properties via proximity effects and electrical stimuli, making them promising candidates for application in spin-electronics. We use…