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The Van der Waals semiconductor metamagnet CrSBr offers an ideal platform for studying the interplay between optical and magnetic properties in the two-dimensional limit. Here, we carried out an exhaustive optical characterization of this…

The van der Waals layered semiconductor CrSBr, which exhibits A-type antiferromagnetism and a relatively high N\'{e}el temperature, has been successfully exfoliated into atomically thin sheets. In this study, we investigate the structural,…

Materials Science · Physics 2025-02-07 Huicong Li , Yali Yang , Zhonghao Xia , Yateng Wang , Jiacheng Wei , Jiangang He , Rongming Wang

In two-dimensional van der Waals magnetic materials, the interplay between magnetism and electron correlation can give rise to new ground states and lead to novel transport and optical properties. A fundamental question in these materials…

The discovery of atomically thin two-dimensional (2D) magnetic semiconductors has triggered enormous research interest recently. In this work, we use first-principles many-body perturbation theory to study a prototypical 2D ferromagnetic…

Materials Science · Physics 2022-02-01 Meng Wu , Zhenglu Li , Steven G. Louie

Understanding and controlling native defects is essential for unlocking the full potential of two-dimensional magnetic semiconductors. Here, angle-resolved photoemission spectroscopy (ARPES) and first-principles calculations are used to…

The layered, air-stable van der Waals antiferromagnetic compound CrSBr exhibits pronounced coupling between its optical, electronic, and magnetic properties. As an example, exciton dynamics can be significantly influenced by lattice…

The van der Waals material CrSBr stands out as a promising two-dimensional magnet. Especially, its high magnetic ordering temperature and versatile magneto-transport properties make CrSBr an important candidate for new devices in the…

Many-body excitons in CrSBr are attracting intense interest in view of their highly anisotropic magneto-optical coupling and their potential for novel optical interfaces within spintronic and magnonic devices. Characterizing the orbital…

Van der Waals (vdW) heterostructures composed of two-dimensional (2D) transition metal dichalcogenides (TMD) and vdW magnetic materials offer an intriguing platform to functionalize valley and excitonic properties in non-magnetic TMDs.…

CrSBr is a van der Waals magnetic semiconductor exhibiting antiferromagnetic order below 140 K. It has emerged as a promising platform for engineering 2D magnetism because its intertwined electronic, optical, and magnetic properties can be…

Controlling magnetic order via external fields or heterostructures enables precise manipulation and tracking of spin and exciton information, facilitating the development of high-performance optical spin valves. However, the weak…

Materials Science · Physics 2024-09-30 Jia Shi , Dan Wang , Nai Jiang , Ziqian Xin , Houzhi Zheng , Chao Shen , Xinping Zhang , Xinfeng Liu

CrSBr is an air-stable 2D van der Waals semiconducting magnet with great technological promise, but its atomic-scale magnetic interactions -- crucial information for high-frequency switching -- are poorly understood. We present an…

Materials Science · Physics 2022-07-18 A. Scheie , M. Ziebel , D. G. Chica , Y. J. Bae , Xiaoping Wang , A. I. Kolesnikov , Xiaoyang Zhu , X. Roy

The exploration of spin configurations and magnetoresistance in van der Waals magnetic semiconductors, particularly in the realm of thin-layer structures, is of paramount significance for the development of two-dimensional spintronic…

Mesoscale and Nanoscale Physics · Physics 2025-05-01 Ziqi Liu , Yichang Sun , Chengfeng Zhu , Canyu Hong , Yuchen Gao , Zeyuan Sun , Kenji Watanabe , Takashi Taniguchi , Shiwei Wu , Zuxin Chen , Pingfan Gu , Yu Ye

We use a combined generalized spectroscopic ellipsometry and density functional theory approach to determine and analyze the anisotropic dielectric functions of an $\alpha$-Ga$_2$O$_3$ thin film. The sample is grown epitaxially by…

The growing interest in 2D van der Waals (vdW) magnetic materials stems from their unique properties and potential applications in spintronics, magnonics and quantum information technologies. Among them, CrSBr is a semiconductor that stands…

Materials Science · Physics 2024-12-24 Sourav Dey , Dorye L. Esteras , José J. Baldoví

Quasiparticle condensates are among the most spectacular solid-state manifestations of quantum physics. Coupling macroscopic real-space wave functions to additional degrees of freedom, such as the electron spin, would add valuable control…

Single crystals of CrSbSe$_3$, a structurally pseudo-one-dimensional ferromagnetic semiconductor, were grown using a high-temperature solution growth technique and were characterized by x-ray diffraction, anisotropic, temperature- and…

Materials Science · Physics 2018-01-24 Tai Kong , Karoline Stolze , Ni Danrui , Satya K. Kushwaha , Robert J. Cava

CrSb is a layered antiferromagnet (AFM) with perpendicular magnetic anisotropy, a high N\'{e}el temperature, and large spin-orbit coupling (SOC), which makes it interesting for AFM spintronic applications. To elucidate the various…

Materials Science · Physics 2021-01-04 In Jun Park , Sohee Kwon , Roger K. Lake

The strong coupling between photons and matter excitations such as excitons, phonons, and magnons is of central importance in the study of light-matter interactions. Bridging the flying and stationary quantum states, the strong light-matter…

Among two-dimensional magnetic materials, CrSBr has attracted considerable attention owing to its coexistence of ferromagnetic and antiferromagnetic ordering, which depends sensitively on crystallographic orientation. An additional…

Materials Science · Physics 2026-05-26 Naresh Shyaga , Pankaj Bhardwaj , Rajib Sarkar , Jagadish Rajendran , Abhiram Soori , Dhavala Suri