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When electrolyte solutions are confined in micro- and nanochannels their conductivity is significantly different from those in a bulk phase. Here we revisit the theory of this phenomenon by focusing attention on the reduction in the ion…

Soft Condensed Matter · Physics 2023-11-08 Olga I. Vinogradova , Elena F. Silkina

The ion-induced long-range orientational order between water molecules recently observed in second harmonic scattering experiments and illustrated with large scale molecular dynamics simulations is quantitatively explained using the…

Chemical Physics · Physics 2018-03-29 Luc Belloni , Daniel Borgis , Maximilien Levesque

The conductivity of ionic solutions is arguably their most important trait, being widely used in electrochemical, biochemical, and environmental applications. The Debye-H\"uckel-Onsager theory successfully predicts the conductivity at very…

Soft Condensed Matter · Physics 2023-01-03 Yael Avni , Ram M. Adar , David Andelman , Henri Orland

We study swelling and structural properties of ionic microgel suspensions within a comprehensive coarse-grained model that combines the polymeric and colloidal natures of microgels as permeable, compressible, charged spheres governed by…

Soft Condensed Matter · Physics 2018-06-07 Tyler J. Weyer , Alan R. Denton

We derive the Hydrodynamics for a system of N active, spherical, underdamped particles, interacting through conservative forces. At the microscopic level, we represent the evolution of the particles in terms of the Kramers equation for the…

Statistical Mechanics · Physics 2022-03-15 Umberto Marini Bettolo Marconi , Andrea Puglisi , Lorenzo Caprini

Binary coagulation is an important process in aerosol dynamics by which two particles merge to form a larger one. The distribution of particle sizes over time may be described by the so-called Smoluchowski's coagulation equation. This…

Mathematical Physics · Physics 2021-06-25 Marina A. Ferreira

Ultracold plasmas are a promising candidate for the creation of strongly-coupled Coulomb systems. Unfortunately, the values of the coupling parameter Gamma_e actually achieved after photoionization of the neutral atoms remain relatively…

Plasma Physics · Physics 2022-11-23 Yurii V. Dumin , Anastasiia T. Lukashenko

We propose an efficient and fast numerical algorithm of finding a \emph{stationary} solution of large systems of aggregation-fragmentation equations of Smoluchowski type for concentrations of reacting particles. This method is applicable…

Computational Physics · Physics 2015-04-13 Vladimir Stadnichuk , Anna Bodrova , Nikolai Brilliantov

A new computational method is presented for study suspensions of charged soft particles undergoing fluctuating hydrodynamic and electrostatic interactions. The proposed model is appropriate for polymers, proteins and porous particles…

Soft Condensed Matter · Physics 2015-04-14 Juan P. Hernandez-Ortiz , Juan J. de Pablo

A binary fluid mixture in contact with lateral particle reservoirs is considered. By imposing different particle concentrations in these reservoirs, the system can be maintained under controlled non-equilibrium conditions. Previous…

Statistical Mechanics · Physics 2026-04-01 O. Politano , Alejandro L. Garcia , F. Baras , M. Malek Mansour

Water-in-Salt-Electrolytes (WiSEs) are an exciting class of concentrated electrolytes finding applications in energy storage devices because of their expanded electrochemical stability window, good conductivity and cation transference…

Polymer translocation experiments typically involve anionic polyelectrolytes such as DNA molecules driven through negatively charged nanopores. Quantitative modelling of polymer capture to the nanopore followed by translocation therefore…

Soft Condensed Matter · Physics 2017-10-11 Sahin Buyukdagli , Tapio Ala-Nissila

The nonlinear electrokinetic response of ionic solutions is important in nanofluidics. However, quantitatively understanding the mechanisms is still a challenging problem because of a lack of analytic approaches. Here, a general framework…

Fluid Dynamics · Physics 2023-05-26 Yuki Uematsu

The structure of an aqueous solution of sodium chloride at a planar electrode is investigated by integral equation techniques. With the central force water model the aqueous electrolyte is modelled as a mixture of sodium and chloride ions…

chem-ph · Physics 2009-10-28 M. Vossen , F. Forstmann

Experiments using the Surface Force Apparatus (SFA) have found anomalously long ranged charge-charge underscreening in concentrated salt solutions. Meanwhile, theory and simulations have suggested ion clustering to be the possible origin of…

Soft Condensed Matter · Physics 2024-08-13 David Ribar , Clifford E. Woodward , Sture Nordholm , Jan Forsman

For many real physico-chemical complex systems detailed mechanism includes both reversible and irreversible reactions. Such systems are typical in homogeneous combustion and heterogeneous catalytic oxidation. Most complex enzyme reactions…

Statistical Mechanics · Physics 2013-01-17 A. N. Gorban , E. M. Mirkes , G. S. Yablonsky

Particle-particle correlation functions in ionic systems control many of their macroscopic properties. In this work, we use stochastic density functional theory to compute these correlations, and then we analyze their long-range behavior.…

Statistical Mechanics · Physics 2025-02-05 Haggai Bonneau , Vincent Démery , Elie Raphaël

The dynamics and processes involved in particle-molecule scattering, including nuclear dynamics, are described and analyzed using various quantum information quantities throughout the different stages of the scattering. The main process…

Quantum Physics · Physics 2025-05-22 Martin Mendez , Federico M. Pont

A new approach is developed to integrate numerically the equations of motion for systems of interacting rigid polyatomic molecules. With the aid of a leapfrog framework, we directly involve principal angular velocities into the integration,…

Computational Physics · Physics 2007-05-23 Igor P. Omelyan

We demonstrate an archetypal Loschmidt-echo experiment involving thousands of droplets which interact in a reversible fashion via a viscous fluid. Firstly, we show that, unlike equilibrium systems, periodically driven microfluidic emulsions…

Soft Condensed Matter · Physics 2014-07-08 Raphaël Jeanneret , Denis Bartolo