Related papers: X-ray diffraction from chiral molecules with twist…
We demonstrate that an effect phenomenologically analogous to circular dichroism can arise even for dielectric and isotropic chiral spherical particles. By analyzing the polarimetry of light scattered from a chiral, lossless microsphere…
We propose an approach to probe coherent spin-state dynamics of molecules using circularly polarized hard x-ray pulses. For the dynamically aligned nitric oxide molecules in a coherent superposition spin-orbit coupled electronic state that…
Manifestations of orbital angular momentum induced effects in the diffraction of a radially polarized vector beam by an off-axis tilted aperture are studied both experimentally and theoretically. Experiments were carried out to extract the…
We study the resonant x-ray scattering at Si and Al K-edges from chiral materials, $\alpha$-quartz and $\alpha$-berlinite. We derive the general form of the scattering matrix for the dipole transition by summing up the local scattering…
Resonant inelastic X-ray scattering (RIXS) can probe localized excitations at selected atoms in materials, including particle-hole transitions between the valence and conduction bands. These transitions are governed by fundamental…
X-ray beams with orbital angular momentum (OAM) are a promising tool for x-ray characterization techniques. Beams with OAM have a helicity--an azimuthally varying phase--which leads to a gradient of the light field. New material properties…
Chiroptical effects using circularly polarized light produce signals that change sign when switching either molecular handedness (enantiosensitivity) or the light helicity (circular dichroism). Here, we break this…
Whether or not chiral interaction exists between the optical orbital angular momentum (OAM) and a chiral molecule remains unanswered. So far, such an interaction has not been observed experimentally. Here we present a T-matrix method to…
Chirality is ubiquitous in nature and fundamental in science, from particle physics to metamaterials.The most established technique of chiral discrimination - photoabsorption circular dichroism - relies on the magnetic properties of a…
We study diffraction of twisted matter waves (electrons and light ions carrying orbital angular momentum $\ell/\hbar=0,\pm1,\pm2,\ldots$ by circular and triangular apertures. Within the scalar Kirchhoff-Fresnel framework, circular apertures…
Chirality in the mid-infrared spectral range plays a crucial role across physical, chemical, and biological sciences, yet sources of chiral infrared light do not currently exist. Their development, using principles from the mature field of…
Recent studies demonstrated the violation of reciprocity in optical processes in low-symmetry magnetic crystals. In these crystals the speed of light can be different for counter-propagating beams. Correspondingly, they can show strong…
A thorough tensor analysis of the Bragg-forbidden reflection (00.3)$_h$ in corundum systems having a global center of inversion, like V$_2$O$_3$ and $\alpha$-Fe$_2$O$_3$, shows that anomalous x-ray resonant diffraction can access chiral…
Circular dichroism spectroscopy is an essential technique for understanding molecular structure and magnetic materials, but spatial resolution is limited by the wavelength of light, and sensitivity sufficient for single-molecule…
Resonant chiral dielectric metasurfaces can support circular dichroism exceeding that of natural materials, but their small dissipative losses simultaneously limit the maximization of circular dichroism, which inherently relies on…
Controlling and channelling light emissions from unpolarized quantum dots into specific directions with chiral polarization remains a key challenge in modern photonics. Stacked metasurface designs offer a potential compact solution for…
Understanding the scattering properties of various media is of critical importance in many applications, from secure, high-bandwidth communications to extracting information about biological and mineral particles dissolved in sea water. In…
Electron transmission through chiral molecules induced by circularly polarized light can be very different for mirror-image structures, a peculiar fact given that the electronic energy spectra of the systems are identical. We propose that…
X-ray circular dichroism, arising from the contrast in X-ray absorption between opposite photon helicities, serves as a spectroscopic tool to measure the magnetization of ferromagnetic materials and identify the handedness of chiral…
We demonstrate natural optical activity in disordered ensembles of non-chiral plasmonic resonators. We show that the statistical distributions of rotatory power and spatial dichroism are strongly dependent on the scattering mean free path…