Giant X-ray circular dichroism in a time-reversal invariant altermagnet
Abstract
X-ray circular dichroism, arising from the contrast in X-ray absorption between opposite photon helicities, serves as a spectroscopic tool to measure the magnetization of ferromagnetic materials and identify the handedness of chiral crystals. Antiferromagnets with crystallographic chirality typically lack X-ray magnetic circular dichroism because of time-reversal symmetry, yet exhibit weak X-ray natural circular dichroism. Here, we report the observation of giant natural circular dichroism in the Ni -edge X-ray absorption of NiTeO, a polar and chiral antiferromagnet with effective time-reversal symmetry. To unravel this intriguing phenomenon, we propose a phenomenological model that classifies the movement of photons in a chiral crystal within the same symmetry class as that of a magnetic field. The coupling of X-ray polarization with the induced magnetization yields giant X-ray natural circular dichroism, revealing the altermagnetism of NiTeO. Our findings provide evidence for the interplay between magnetism and crystal chirality in natural optical activity. Additionally, we establish the first example of a new class of magnetic materials exhibiting circular dichroism with time-reversal symmetry.
Keywords
Cite
@article{arxiv.2312.07081,
title = {Giant X-ray circular dichroism in a time-reversal invariant altermagnet},
author = {Jun Okamoto and Ru-Pan Wang and Yen-Yi Chu and Hung-Wei Shiu and Amol Singh and Hsiao-Yu Huang and Chung-Yu Mou and Sucitto Teh and Horng-Tay Jeng and Kai Du and Xianghan Xu and Sang-Wook Cheong and Chao-Hung Du and Chien-Te Chen and Atsushi Fujimori and Di-Jing Huang},
journal= {arXiv preprint arXiv:2312.07081},
year = {2024}
}
Comments
Accepted by Advanced Materials (2024.2.16) Revised title: Giant X-ray circular dichroism in a time-reversal invariant altermagnet Revised drafts: Main 14 pages, 4 figures, and SI 20 pages, 8 figures