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Time-dependent response theories are foundational to the development of algorithms that determine quantum properties of electronic excited states of molecules and periodic systems. They are employed in wave-function, density-functional, and…

Chemical Physics · Physics 2022-11-23 Martín A. Mosquera

A semiconductor quantum dot (QD) embedded within an optical microcavity is a system of fundamental importance within quantum information processing. The optimization of quantum coherence is crucial in such applications, requiring an…

Mesoscale and Nanoscale Physics · Physics 2020-02-06 A. Morreau , C. Joshi , E. A. Muljarov

The exploration of the root structure of coupled cluster equations holds both foundational and practical significance for computational quantum chemistry. This study provides insight into the intricate root structures of these non-linear…

Chemical Physics · Physics 2024-09-12 Svala Sverrisdóttir , Fabian M. Faulstich

Quantum coherence is one of the fundamental aspects distinguishing classical and quantum theories. Coherence between different energy eigenstates is particularly important, as it serves as a valuable resource under the law of energy…

Quantum Physics · Physics 2024-05-07 Naoto Shiraishi , Ryuji Takagi

Computationally efficient and accurate quantum mechanical approximations to solve the many-electron Schr\"odinger equation are at the heart of computational materials science. In that respect the coupled cluster hierarchy of methods plays a…

Materials Science · Physics 2022-01-11 Tina N. Mihm , Tobias Schäfer , Sai Kumar Ramadugu , Andreas Grüneis , James J. Shepherd

We consider a fermionic system for which there exist a single-reference configuration-interaction (CI) expansion of the ground state wave function that converges, albeit not necessarily rapidly, with respect to excitation number. We show…

Strongly Correlated Electrons · Physics 2020-01-13 Dominic Bergeron

Ground-state electronic structure calculations using Kohn-Sham density functional theory (KS-DFT) offer an unprecedented balance between efficiency and accuracy, now paradigmatic to the fields of quantum chemistry and condensed matter…

Chemical Physics · Physics 2026-04-14 Lucien Dupuy , Toni Chiti , Jérémy Morere , Emmanuel Fromager

Coherent state path integrals are applied to a many-body problem for non-relativistic electrons in a central potential and an external magnetic field; however, in comparison to previous coherent state path integrals, we definitely fix the…

Statistical Mechanics · Physics 2009-06-16 Bernhard Mieck

A model which combines the perturbative behavior of QCD with low energy phenomenology in a unified framework is developed. This is achieved by applying a similarity transformation to the QCD Hamiltonian which removes interactions between…

High Energy Physics - Phenomenology · Physics 2009-10-28 A. P. Szczepaniak , E. S. Swanson

Downfolding coupled cluster (CC) techniques have recently been introduced into quantum chemistry as a tool for the dimensionality reduction of the many-body quantum problem. As opposed to earlier formulations in physics and chemistry based…

Quantum Physics · Physics 2022-03-23 Nicholas P. Bauman , Karol Kowalski

We consider the relativistic electron-positron field interacting with itself via the Coulomb potential defined with the physically motivated, positive, density-density quartic interaction. The more usual normal-ordered Hamiltonian differs…

Mathematical Physics · Physics 2007-05-23 Elliott H. Lieb , Heinz Siedentop

We present a similarity transformation theory based on a polynomial form of a particle-hole pair excitation operator. In the weakly correlated limit, this polynomial becomes an exponential, leading to coupled cluster doubles. In the…

Strongly Correlated Electrons · Physics 2016-11-23 Matthias Degroote , Thomas M. Henderson , Jinmo Zhao , Jorge Dukelsky , Gustavo E. Scuseria

The recently introduced coupled cluster (CC) downfolding techniques for reducing the dimensionality of quantum many-body problems recast the CC formalism in the form of the renormalization procedure allowing, for the construction of…

Quantum Physics · Physics 2021-11-08 Nicholas P. Bauman , Karol Kowalski

Coupled cluster (CC) methods are among the most accurate methods in quantum chemistry. However, the standard CC linear response formulation is not gauge invariant resulting in errors when modelling properties like optical rotation and…

Chemical Physics · Physics 2018-03-13 Rolf H. Myhre

Cavity quantum electrodynamics provides an ideal platform to engineer and control light-matter interactions with polariton quasiparticles. In this work, we investigate collective phenomena in a system of many particles in a harmonic trap…

Quantum Physics · Physics 2023-06-21 V. Rokaj , S. I. Mistakidis , H. R. Sadeghpour

We propose a streamlined combination scheme of the transcorrelation (TC) and coupled cluster (CC) theory, which not only increases the convergence rate with respect to the basis set, but also extends the applicability of the lowest order CC…

Strongly Correlated Electrons · Physics 2021-07-28 Ke Liao , Thomas Schraivogel , Hongjun Luo , Daniel Kats , Ali Alavi

Using unitary transformations, we express the Kondo lattice Hamiltonian in terms of fermionic operators that annihilate the ground state of the interacting system and that represent the best possible approximations to the actual charged…

Condensed Matter · Physics 2009-10-28 J. M. Prats , F. Lopez-Aguilar

Quantum periodic cluster methods for strongly correlated electron systems are reformulated and developed. The reformulation and development are based on a canonical transformation which periodizes the fermions in the cluster space. The…

Strongly Correlated Electrons · Physics 2007-05-23 Tran Minh-Tien

We investigate the basis-set convergence of electronic correlation energies calculated using coupled cluster theory and a recently proposed finite basis-set correction technique. The correction is applied to atomic and molecular systems and…

Chemical Physics · Physics 2019-10-03 Andreas Irmler , Andreas Grüneis

We study quantum electrodynamics (QED) in the light-front dynamical form by using null-plane causal perturbation theory. We establish the equivalence with instant dynamics for the scattering processes, whose normalization allows to…

High Energy Physics - Theory · Physics 2022-08-17 O. A. Acevedo , B. M. Pimentel
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