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We develop a Hamiltonian formalism to study energy and position/momentum correlations between a single Stokes photon and a single material excitation that are created as a pair in the spontaneous Raman scattering process. Our approach…

Quantum Physics · Physics 2020-01-16 Kai Shinbrough , Yanting Teng , Bin Fang , Virginia O. Lorenz , Offir Cohen

Time-resolved spontaneous Raman spectroscopy serves as a probe for incoherent quasiparticle and collective excitation dynamics, and allows to distinguish symmetry changes across a photoinduced phase transition through the inelastic light…

Materials Science · Physics 2019-03-27 J. Zhu , R. B. Versteeg , P. Padmanabhan , P. H. M. van Loosdrecht

We report on the generation of a Raman cascade spanning the wavelength range of 523 to 1750 nm wavelength range, in a standard telecommunication graded-index multimode optical fiber. Despite the highly multimode nature of the pump, the…

Optics · Physics 2013-12-13 Hamed Pourbeyram , Govind P. Agrawal , Arash Mafi

A typical surface-enhanced Raman scattering (SERS) system relies on deeply subwavelength field localization in nanoscale plasmonic cavities to enhance both the excitation and emission of Raman-active molecules. Here, we demonstrate that a…

Quantum Physics · Physics 2025-05-27 Mikolaj K. Schmidt , Alexander A. High , Michael J. Steel

Stimulated Raman scattering is a well-known nonlinear process that can be harnessed to produce optical gain in a wide variety of media. This effect has been used to produce the first silicon-based lasers and high-gain amplifiers.…

Optics · Physics 2008-10-13 D. R. Solli , P. Koonath , B. Jalali

Frequency combs have revolutionized optical frequency metrology, allowing one to determine highly accurate transition frequencies of a wealth of molecular species. Despite a recognized scientific interest, these progresses have only…

We model spontaneous Raman scattering noise in polarization-encoded quantum communication channels co-propagating with classical signals using the depolarization channel. Utilizing NetSquid simulations, we validate the model against…

Quantum Physics · Physics 2025-04-10 Jake Smith , Roberto Proietti

We demonstrate how a narrowband pump and a broadband spectrum can be spatially multiplexed by selective coupling them in two distinct modes of a few-mode microstructure fiber. The first mode carries most of the input pump energy, and…

Raman spectroscopy uses light scattering to extract information on low-energy excitations of solids. The Raman process is described by diagrams which are fourth order in the light-matter interaction, and in particular the resonant…

Strongly Correlated Electrons · Physics 2024-01-30 Philipp Werner , Martin Eckstein , Naoto Tsuji

Stimulated Raman backscatter (SRS) is used as a remote sensor to quantify the instantaneous laser power after transfer from outer to inner cones that cross in a National Ignition Facility (NIF) gas-filled hohlraum plasma. By matching SRS…

We have developed a theory of the one-phonon intraband resonance Raman scattering (IRRS) in anisotropic quantum dots subjected to an arbitrarily directed magnetic field. The differential Raman cross section is obtained. The resonance…

Mesoscale and Nanoscale Physics · Physics 2010-01-08 A. V. Shorokhov , V. A. Margulis

Radiative transfer equations are derived and solved for the stimulated Raman scattering of water maser lines in the astrophysical plasmas with electron density of about 10^6 - 10^7 cm-3. In stimulated Raman scattering, the energy of water…

Astrophysics · Physics 2009-10-31 R. T. Gangadhara , Shuji Deguchi , H. Lesch

Within a generic model we analyze the Stokes linewidth in surface enhanced Raman scattering (SERS) from molecules embedded as bridges in molecular junctions. We identify four main contributions to the off-resonant Stokes signal and show…

Mesoscale and Nanoscale Physics · Physics 2016-06-30 Yi Gao , Michael Galperin , Abraham Nitzan

The small cross section of Raman scattering poses a great challenge for its direct study at the single-molecule level. By exploiting the high Franck-Condon factor of a common-mode resonance, choosing a large vibrational frequency difference…

We present a quantum-mechanical model that describes fiber-based frequency conversion by four-wave-mixing Bragg scattering in the presence of Raman interactions. In the case of continuous-wave pumps we find closed-form expressions for the…

Quantum Physics · Physics 2024-06-06 Mathias Linde Holst Korsgaard , Jacob Gade Koefoed , Karsten Rottwitt

Stimulated Raman scattering (SRS) in plasma in the degenerate regime is studied theoretically and numerically. Different from normal SRS with the non-degenerate eigen electrostatic mode excited, the degenerate SRS is developed at plasma…

Plasma Physics · Physics 2022-03-25 Yao Zhao , Suming Weng , Zhengming Sheng , Jianqiang Zhu

The throughput gains of extending the optical transmission bandwidth to the S+C+L-band are quantified using a Gaussian Noise model that accounts for inter-channel stimulated Raman scattering (ISRS). The impact of potential ISRS mitigation…

Signal Processing · Electrical Eng. & Systems 2020-06-17 Daniel Semrau , Eric Sillekens , Robert I. Killey , Polina Bayvel

Spontaneous vibrational Raman scattering is a ubiquitous form of light-matter interaction whose description necessitates quantization of the electromagnetic field. It is usually considered as an incoherent process because the scattered…

Quantum Physics · Physics 2023-07-18 Valeria Vento , Santiago Tarrago Velez , Anna Pogrebna , Christophe Galland

We report the observation of Raman solitons on numerical simulations of transient stimulated Raman scattering (TSRS) with small group velocity dispersion. The theory proceeds with the inverse scattering transform (IST) for initial-boundary…

Pattern Formation and Solitons · Physics 2009-10-31 M. Boiti , J-G. Caputo , J. Leon , F. Pempinelli

Exchange interactions govern the ordering between microscopic spins and the highest-frequency spin excitations - magnons at the edge of the Brillouin zone. As well known from spontaneous Raman scattering (RS) experiments in…

Strongly Correlated Electrons · Physics 2024-11-25 Anatolii E. Fedianin , Alexandra M. Kalashnikova , Johan H. Mentink