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We present a self-consistent quantum optics approach to calculating the surface enhanced Raman spectrum of molecules coupled to arbitrarily shaped plasmonic systems. Our treatment is intuitive to use and provides fresh analytical insight…

Optics · Physics 2017-06-26 Mohsen Kamandar Dezfouli , Stephen Hughes

Raman phonons are quantized molecular motions that arise from the inelastic scattering of light and mediate a wide range of spectroscopic and nonlinear optical phenomena. These can play a major role in frequency-conversion processes, but…

Optics · Physics 2026-05-01 Yi-Hao Chen , Frank Wise

Backward stimulated Raman scattering in gases provides a promising route to compression and amplification of a Stokes seed-pulse by counter-propagating against a pump-pulse, as has been already demonstrated in various platforms, mainly in…

Optics · Physics 2018-05-08 Manoj K. Mridha , David Novoa , Philip St. J. Russell

Stimulated Raman scattering (SRS) microscopy is a powerful label-free imaging technique that probes the vibrational response of chemicals with high specificity and sensitivity. High-power, quantum-enhanced SRS microscopes have been recently…

We report an investigation of perovskite-type SmScO3 and NdScO3 single crystals by Raman scattering in various scattering configurations and at different wavelengths. The reported Raman spectra, together with the phonon mode assignment, set…

Materials Science · Physics 2011-05-09 O. Chaix-Pluchery , J. Kreisel

The principle and experimental realization of a novel Raman spectroscopic technique entitled stimulated Raman phase shift (SRPS) spectroscopy was demonstrated. This technique depends on the measurement of the stimulated Raman scattering…

Optics · Physics 2024-03-07 Meng Qi , Wenrong Wang , Yuan-ji Li , Jin-xia Feng , Kuan-shou Zhang

Raman scattering, an inelastic scattering mechanism, provides information about molecular excitation energies and can be used to identify chemical compounds. Albeit being a powerful analysis tool, especially for label-free biomedical…

Raman scattering is a chemically selective probing mechanism with diverse applications in industry and clinical settings. Yet, most samples are optically opaque limiting the applicability of Raman probing at depth. Here, we demonstrate…

Strain is prominent in fabricated samples of two-dimensional semiconductors and it also serves as an exploitable tool for engineering their properties. However, quantifying strain and characterizing its spatially inhomogeneous distribution…

Materials Science · Physics 2014-09-01 Ruixiang Fei , Li Yang

A coherent microwave radiation, concomitant with experiments of stimulated Raman scattering (SRS) in weakly compressed hydrogen, had been observed; qualitative and quantitative results had been obtained, and are given in this article. .An…

Optics · Physics 2007-05-23 Boris Oksengorn

Surface enhanced Raman scattering (SERS) effects on tin dioxide in the form of bulk material, nanostructured thin films and colloidal solutions were investigated. Raman spectra are characterized by the three Raman scattering peaks at 478,…

Materials Science · Physics 2015-06-03 Enza Fazio , Fortunato Neri , Salvatore Savasta , Salvatore Spadaro , Sebastiano Trusso

Regular perturbation is applied to space-division multiplexing (SDM) on optical fibers and motivates a correlated rotation-and-additive noise (CRAN) model. For S spatial modes, or 2S complex-alphabet channels, the model has 4S(S+1) hidden…

Information Theory · Computer Science 2021-09-28 Francisco Javier García-Gómez , Gerhard Kramer

Stimulated Raman scattering (SRS) microscopy is a highly sensitive chemical imaging technique. However, the broader application of SRS has been limited by two key challenges: the reliance on low-noise but bulky solid-state laser sources and…

The interaction between molecules is commonly ignored in surface-enhanced Raman scattering (SERS). Under this assumption, the total SERS signal is described as the sum of the individual contributions of each molecule treated independently.…

Optics · Physics 2020-01-08 Yuan Zhang , Javier Aizpurua , Ruben Esteban

We demonstrate low-frequency interferometric impulsive stimulated Raman scattering (ISRS) imaging with high robustness to distortions by optical scattering. ISRS is a pump-probe coherent Raman spectroscopy that can capture Raman vibrational…

Fiber nonlinearities, that lead to nonlinear signal interference (NLI), are typically regarded as an instantaneous material response with respect to the optical field. However, in addition to an instantaneous part, the nonlinear fiber…

Signal Processing · Electrical Eng. & Systems 2021-04-07 Daniel Semrau , Eric Sillekens , Robert I. Killey , Polina Bayvel

We apply collective Raman scattering to create, store and retrieve spatially multimode light in warm rubidium-87 vapors. The light is created in a spontaneous Stokes scattering process. This is accompanied by the creation of counterpart…

Quantum Physics · Physics 2014-05-20 Radoslaw Chrapkiewicz , Wojciech Wasilewski

Propagation of light in a highly scattering medium is among the most fascinating optical effect that everyone experiences on an everyday basis and possesses a number of fundamental problems which have yet to be solved. Conventional wisdom…

The interaction between ultrashort light pulses and non-absorbing materials is dominated by Impulsive Stimulated Raman Scattering (ISRS). The description of ISRS in the context of pump\&probe experiments is based on effective classical…

Spectroscopic stimulated Raman scattering (SRS) imaging has become a useful tool finding a broad range of applications. Yet, wider adoption is hindered by the bulky and environmentally-sensitive solid-state optical parametric oscillator…

Optics · Physics 2021-08-20 Hongli Ni , Peng Lin , Yifan Zhu , Meng Zhang , Yuying Tan , Yuewei Zhan , Ji-Xin Cheng