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We study the behavior of negatively charged colloids with two positively charged polar caps close to a planar patterned surface. The competition between the different anisotropic components of the particle-particle interaction patterns is…

Soft Condensed Matter · Physics 2018-09-25 Emanuele Locatelli , Emanuela Bianchi

We study the formation and growth of equilibrium clusters in a suspension of weakly-charged colloidal particles and small non-adsorbing polymers. The effective potential is characterised by a short-range attraction and a long-range…

Soft Condensed Matter · Physics 2009-11-11 Rodrigo Sanchez , Paul Bartlett

We explore heat transport across an ion Coulomb crystal beyond the harmonic regime by tuning it across the structural phase transition between the linear and zigzag configurations. This demonstrates that the control of the spatial ion…

Quantum Physics · Physics 2014-06-16 Antonia Ruiz , Daniel Alonso , Martin B. Plenio , Adolfo del Campo

Metallic solids are a challenging target for wavefunction-based electronic structure theories and have not been studied in great detail by such methods. Here, we use coupled-cluster theory with single and double excitations (CCSD) to study…

Materials Science · Physics 2022-04-05 Verena A. Neufeld , Hong-Zhou Ye , Timothy C. Berkelbach

We use molecular dynamics with an embedded atom potential to study the behavior of palladium nanoclusters near the melting point in the microcanonical ensemble. We see transitions from both fcc and decahedral ground state structures to…

Other Condensed Matter · Physics 2007-05-23 D. Schebarchov , S. C. Hendy

In recent experiments on sodium chloride clusters structural transitions between nanocrystals with different cuboidal shapes were detected. Here we determine reaction pathways between the low energy isomers of one of these clusters,…

Condensed Matter · Physics 2007-05-23 Jonathan Doye , David Wales

Using the stabilized jellium model in two schemes of `relaxed' and `rigid', we have calculated the dissociation energies and the fission barrier heights for the binary fragmentations of singly-ionized and doubly-ionized Ag clusters. In the…

Materials Science · Physics 2009-11-10 M. Payami

Packing transitions in the lowest energy structures of Li clusters as a function of size have been identified via simulated annealing. For N>21, the large $p$ character of Li leads to unexpected ionic structures. At N~25, a packing pattern…

chem-ph · Physics 2009-10-22 Ming Wen Sung , Ryoichi Kawai , John H. Weare

Colloidal crystals formed by size-asymmetric binary particles co-assemble into a wide variety of colloidal compounds with lattices akin to ionic crystals. Recently, a transition from a compound phase with a sublattice of small particles to…

Soft Condensed Matter · Physics 2023-09-12 Ali Ehlen , Hector Lopez-Rios , Monica Olvera de la Cruz

The behavior of nuclear matter is studied at low densities and temperatures using classical molecular dynamics with three different sets of potentials with different compressibility. Nuclear matter is found to arrange in crystalline…

Nuclear Theory · Physics 2013-05-13 C. O. Dorso , P. A. Giménez Molinelli , J. I. Nichols , J. A. López

Exploration of metal clusters (MCs) adaptive to both aqueous and oil phases without disturbing their size is promising for a broad scope of applications. The state-of-the-art approach via ligand-binding may perturb MC size due to varied…

Chemical Physics · Physics 2019-04-26 Su-Yun Zhang , Zdravko Kochovski , Hui-Chun Lee , Yan Lu , Jie Zhang , Jian-Ke Sun , Jiayin Yuan

Geometry, electronic structure, and magnetic properties of methylthiolate-stabilized Au$_{25}$L$_{18}$ and MnAu$_{24}$L$_{18}$ (L = SCH$_3$) clusters adsorbed on noble-metal (111) surfaces have been investigated by using spin-polarized…

Atomic and Molecular Clusters · Physics 2015-06-03 Xi Chen , Mikkel Strange , Hannu Hakkinen

Ab initio calculations using the Perturbed Ion model, with correlation contributions included, are presented for nonstoichiometric (NaI)_nNa+ and (CsI)_nCs+ (n=1-14) cluster ions. The ground state and several low-lying isomers are…

Atomic and Molecular Clusters · Physics 2009-10-31 A. Aguado , A. Ayuela , J. M. Lopez , J. A. Alonso

We study theoretically large metal clusters containing vacancies. We propose an approach, which combines the Kohn-Sham results for monovacancy in a bulk of metal and analytical expansions in small parameters $c_{v}$ (relative concentration…

Mesoscale and Nanoscale Physics · Physics 2018-02-14 V. V. Pogosov , V. I. Reva

Polynomial machine learning potentials (MLPs) based on polynomial rotational invariants have been systematically developed for various systems and applied to efficiently predict crystal structures. In this study, we propose a robust…

Materials Science · Physics 2026-03-18 Hayato Wakai , Atsuto Seko , Isao Tanaka

A multitude of observed boron-based materials have outstanding superconducting, mechanical, and refractory properties. Yet, the structure, the composition, and the very existence of some reported metal boride (M-B) compounds have been a…

Materials Science · Physics 2014-10-03 A. G. Van Der Geest , A. N. Kolmogorov

We investigate the structure of 13-particle clusters in binary alloys for various size ratios and different concentrations via MD simulation. Our goal is to predict which systems are likely to form local icosahedral structures when rapidly…

Condensed Matter · Physics 2007-05-23 Stefano Cozzini , Marco Ronchetti

Effects of the single-electron tunneling and the Coulomb blockade in a cluster structure (the molecular transistor) are investigated theoretically. In the framework of the particle-in-a-box model for the spherical and disk-shaped gold…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Valentin V. Pogosov , Eugene V. Vasyutin

Physical mechanisms of structural transformations in deposited metallic clusters exposed to an electron beam of a transmission electron microscope (TEM) are studied theoretically and computationally. Recent TEM experiments with…

Atomic and Molecular Clusters · Physics 2023-09-20 Alexey V. Verkhovtsev , Yury Erofeev , Andrey V. Solov'yov

The prediction of energetically stable crystal structures formed by a given chemical composition is a central problem in solid-state physics. In principle, the crystalline state of assembled atoms can be determined by optimizing the energy…

Materials Science · Physics 2022-06-01 Minoru Kusaba , Chang Liu , Ryo Yoshida
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