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We present an experimental and theoretical study of the phase behavior of a binary mixture of colloids with opposite adsorption preferences in a critical solvent. As a result of the attractive and repulsive critical Casimir forces, the…

Soft Condensed Matter · Physics 2011-10-03 O. Zvyagolskaya , A. J. Archer , C. Bechinger

If colloidal solute particles are suspended in a solvent close to its critical point, they act as cavities in a fluctuating medium and thereby restrict and modify the fluctuation spectrum in a way which depends on their relative…

Soft Condensed Matter · Physics 2018-11-14 Anna Maciolek , Siegfried Dietrich

The critical Casimir effect provides a thermodynamic analogue of the well-known quantum mechanical Casimir effect. It acts between two surfaces immersed in a critical binary liquid mixture, and results from the confinement of concentration…

Soft Condensed Matter · Physics 2015-06-15 Van Duc Nguyen , Suzanne Faber , Zhibing Hu , Gerard H. Wegdam , Peter Schall

Spatial confinement of a near-critical medium changes its fluctuation spectrum and modifies the corresponding order parameter distribution. These effects result in effective, so-called critical Casimir forces (CCFs) acting on the confining…

Soft Condensed Matter · Physics 2014-03-24 T. F. Mohry , S. Kondrat , A. Maciolek , S. Dietrich

From experimental studies it is well-known that colloidal particles suspended in a near-critical binary solvent exhibit interesting aggregation phenomena, often associated with colloidal phase transitions, and assumed to be driven by…

Soft Condensed Matter · Physics 2015-06-19 John R. Edison , Nikos Tasios , Simone Belli , Robert Evans , Rene van Roij , Marjolein Dijkstra

We investigate the behavior of colloidal particles immersed in a binary liquid mixture of water and 2,6-lutidine in the presence of a chemically patterned substrate. Close to the critical point of the mixture, the particles are subjected to…

Soft Condensed Matter · Physics 2009-11-13 F. Soyka , O. Zvyagolskaya , C. Hertlein , L. Helden , C. Bechinger

We study the phase behavior of colloidal suspensions the solvents of which are considered to be binary liquid mixtures undergoing phase segregation. We focus on the thermodynamic region close to the critical point of the accompanying…

Soft Condensed Matter · Physics 2015-06-03 T. F. Mohry , A. Maciołek , S. Dietrich

Critical Casimir forces can play an important role for applications in nano-science and nanotechnology, owing to their piconewton strength, nanometric action range, fine tunability as a function of temperature, and exquisite dependence on…

The phase behavior of a single type of colloid C suspended in near-critical solvents is known to be very rich. Motivated in part by recent experiments we consider a mixture of two colloidal types C1 and C2 in a binary solvent close to its…

Soft Condensed Matter · Physics 2026-03-23 Nima Farahmand Bafi , Robert Evans , Anna Maciolek

The spatial suppression of order parameter fluctuations in a critical media produces Critical Casimir forces acting on confining surfaces. This scenario is realized in a critical binary mixture near the demixing transition point that…

Statistical Mechanics · Physics 2014-10-03 Oleg A. Vasilyev

Colloids immersed in a critical binary liquid mixture are subject to critical Casimir forces (CCFs) because they confine its concentration fluctuations and influence the latter via effective surface fields. To date, CCFs have only been…

Soft Condensed Matter · Physics 2013-09-04 Akira Furukawa , Andrea Gambassi , Siegfried Dietrich , Hajime Tanaka

We present a numerical study of the effective potential $V_\mathrm{eff}$ between two hard-sphere colloids dispersed in a solvent of interacting particles, for several values of temperature and solvent density, approaching the solvent…

Soft Condensed Matter · Physics 2013-04-08 Nicoletta Gnan , Emanuela Zaccarelli , Piero Tartaglia , Francesco Sciortino

We study theoretically and experimentally the solvent-mediated critical Casimir force acting on colloidal particles immersed in a binary liquid mixture of water and 2,6-lutidine and close to substrates which are chemically patterned with…

We consider an ensemble of spherical colloidal particles immersed in a near-critical solvent such as a binary liquid mixture close to its critical demixing point. The emerging long-ranged fluctuations of the corresponding order parameter of…

Soft Condensed Matter · Physics 2015-06-03 T. F. Mohry , A. Maciołek , S. Dietrich

If a fluctuating medium is confined, the ensuing perturbation of its fluctuation spectrum generates Casimir-like effective forces acting on its confining surfaces. Near a continuous phase transition of such a medium the corresponding order…

Soft Condensed Matter · Physics 2011-02-15 A. Gambassi , A. Maciolek , C. Hertlein , U. Nellen , L. Helden , C. Bechinger , S. Dietrich

We study the fluctuation-induced Casimir interactions in colloidal suspensions, especially between colloids immersed in a binary liquid close to its critical demixing point. To simulate these systems, we present a highly efficient cluster…

Soft Condensed Matter · Physics 2017-06-09 Hendrik Hobrecht , Alfred Hucht

We study the critical Casimir interaction between two spherical colloids immersed in a binary liquid mixture close to its critical demixing point. The surface of each colloid prefers one species of the mixture with the exception of a…

Statistical Mechanics · Physics 2020-04-22 Nima Farahmand Bafi , Piotr Nowakowski , Siegfried Dietrich

In soft and condensed matter physics, effective interactions often emerge as a result of the spatial confinement of a fluctuating field. For instance, microscopic particles in a binary liquid mixture are subject to critical Casimir forces…

Percolation and critical phenomena show common features such as scaling and universality. Colloidal particles, immersed in a solvent close to criticality, experience long-range effective forces, named critical Casimir forces. %These…

Soft Condensed Matter · Physics 2014-07-16 Nicoletta Gnan , Emanuela Zaccarelli , Francesco Sciortino

We experimentally demonstrate that critical Casimir forces in colloidal systems can be continuously tuned by the choice of boundary conditions. The interaction potential of a colloidal particle in a mixture of water and 2,6-lutidine has…

Soft Condensed Matter · Physics 2009-10-23 Ursula Nellen , Laurent Helden , Clemens Bechinger
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