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We report on a study of Dynamic Nuclear Polarization and electron and nuclear spin relaxation of atomic hydrogen and deuterium in solid molecular matrices of H$_{2}$, D$_{2}$, and HD mixtures. The electron and nuclear spin relaxation times…

Atomic and Molecular Clusters · Physics 2017-02-08 S. Sheludiakov , J. Ahokas , J. Järvinen , O. Vainio , L. Lehtonen , S. Vasiliev , D. M. Lee , V. V. Khmelenko

The solid effect is one of the simplest and most effective mechanisms for Dynamic Nuclear Polarization. It involves the exchange of polarization between one electron and one nuclear spin coupled via the hyperfine interaction. Even for such…

Strongly Correlated Electrons · Physics 2018-03-29 Ines Rodriguez-Arias , Alberto Rosso , Andrea De Luca

Dynamic nuclear polarization (DNP) is used in nuclear magnetic resonance (NMR) to transfer polarization from electron spins to nuclear spins. The resulting nuclear polarization enhancement can, in theory, be two or three orders of magnitude…

Quantum Physics · Physics 2015-10-14 Sarah Sheldon , David G. Cory

We have first successfully transferred the 129Xe polarization of natural isotopic composition to the proton of solid-state 1HCl via Spin Polarization-Induced Nuclear Overhauser Effect (SPINOE), by mixing the hyperpolarized 129Xe gas and the…

Soft Condensed Matter · Physics 2007-05-23 Xin Zhou , Jun Luo , Xian-ping Sun , Xi-zhi Zeng , Shang-wu Ding , Mai-li Liu , Ming-sheng Zhan

We polarize nuclear spins in a GaAs double quantum dot by controlling two-electron spin states near the anti-crossing of the singlet (S) and m_S=+1 triplet (T+) using pulsed gates. An initialized S state is cyclically brought into resonance…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. R. Petta , J. M. Taylor , A. C. Johnson , A. Yacoby , M. D. Lukin , C. M. Marcus , M. P. Hanson , A. C. Gossard

We theoretically study the dynamic polarization of lattice nuclear spins in GaAs double quantum dots containing two electrons. In our prior work [Phys. Rev. Lett. 104, 226807 (2010)] we identified three regimes of long-term dynamics,…

Mesoscale and Nanoscale Physics · Physics 2014-07-28 M. Gullans , J. J. Krich , J. M. Taylor , B. I. Halperin , M. D. Lukin

We propose a new mechanism for polarizing nuclear spins in quantum dots, based on periodic modulation of the hyperfine coupling by electric driving at the electron spin resonance frequency. Dynamical nuclear polarization results from…

Mesoscale and Nanoscale Physics · Physics 2008-04-14 M. S. Rudner , L. S. Levitov

Dynamic Nuclear Polarization (DNP) is to date the most effective technique to increase the nuclear polarization up to a factor $100,000$ opening disruptive perspectives for medical applications. In DNP, the nuclear spins are driven to an -…

Strongly Correlated Electrons · Physics 2015-08-26 Andrea De Luca , Alberto Rosso

We propose a new, more efficient, and potentially cost effective, solid-state nuclear spin hyperpolarization method combining the Cross Effect mechanism and electron spin optical hyperpolarization in rotating solids. We first demonstrate…

Quantum Physics · Physics 2022-01-25 Frederic Mentink-Vigier , Vinayak Rane , Thierry Dubroca , Krishnendu Kundu

This paper presents a theory describing the dynamic nuclear polarization (DNP) process associated with an arbitrary frequency swept microwave pulse. The theory is utilized to explain the integrated solid effect (ISE) as well as the newly…

An all-optical scheme to polarize nuclear spins in a single quantum dot is analyzed. The hyperfine interaction with randomly oriented nuclear spins presents a fundamental limit for electron spin coherence in a quantum dot; by cooling the…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 A. Imamoglu , E. Knill , L. Tian , P. Zoller

The electron-nuclei (hyperfine) interaction is central to spin qubits in solid state systems. It can be a severe decoherence source but also allows dynamic access to the nuclear spin states. We study a double quantum dot exposed to an…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Gunnar Petersen , Eric A. Hoffmann , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig

An extension of the original Overhauser effect to a more general nonequilibrium state was proposed by G. Feher, and demonstrated by Clark and Feher some forty years ago. It is suggested here that it might be possible to produce excess…

Materials Science · Physics 2007-05-23 Harry Suhl

An equation of state(EOS) of nuclear matter with explicit inclusion of a spin-isospin dependent force is constructed from a finite range, momentum and density dependent effective interaction. This EOS is found to be in good agreement with…

Nuclear Theory · Physics 2009-10-30 V. S. Uma Maheswari , D. N. Basu , J. N. De , S. K. Samaddar

We propose to use the spin-blockade regime in double quantum dots to reduce nuclear spin polarization fluctuations in analogy with optical Doppler cooling. The Overhauser shift brings electron levels in and out of resonance, creating…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. S. Rudner , L. S. Levitov

Dynamic nuclear polarisation (DNP) refers to a class of techniques used to increase the signal in nuclear magnetic resonance measurements by transferring spin polarisation from ensembles of highly polarised electrons to target nuclear…

Quantum Physics · Physics 2020-12-24 L. T. Hall , D. A. Broadway , A. Stacey , D. A. Simpson , J-P. Tetienne , L. C. L. Hollenberg

Sizable nuclear spin polarization is pumped in individual InP/GaInP dots in a wide range of external magnetic fields B_ext=0-5T by circularly polarized optical excitation. We observe nuclear polarization of up to ~40% at Bext=1.5T and…

We present an experimental study of the Dynamic Nuclear Polarization (DNP) of \si{} nuclei in silicon crystals of natural abundance doped with As in the temperature range 0.1-1 K and in strong magnetic field of 4.6 T. This ensures very high…

Mesoscale and Nanoscale Physics · Physics 2020-06-24 J. Jarvinen , D. Zvezdov , J. Ahokas , S. Sheludyakov , L. Lehtonen , S. Vasiliev , L. Vlasenko , Y. Ishikawa , Y. Fujii

We theoretically investigate dynamic nuclear spin polarization in a self-assembled quantum dot pumped optically by two laser beams. With the assumption that a noncollinear interaction between the hole spin and nuclear spins leads to nuclear…

Mesoscale and Nanoscale Physics · Physics 2013-06-07 Xiao-Feng Shi

We discuss the polarization dynamics during solid effect dynamic nuclear polarization (DNP) in a central spin model that consists of an electron surrounded by many nuclei. To this end we use a recently developed formalism and validate first…

Other Condensed Matter · Physics 2016-03-23 Daniel Wiśniewski , Alexander Karabanov , Igor Lesanovsky , Walter Köckenberger
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