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Dynamic nuclear polarization (DNP) is an out-of-equilibrium method for generating non-thermal spin polarization which provides large signal enhancements in modern diagnostic methods based on nuclear magnetic resonance. A particular instance…

This article reviews the physics and technology of producing large quantities of highly spin-polarized, or hyperpolarized, $^3$He nuclei using spin-exchange (SEOP) and metastability-exchange (MEOP) optical pumping, and surveys applications…

Atomic Physics · Physics 2018-01-17 T. R. Gentile , P. J. Nacher , B. Saam , T. G. Walker

We show that optical pumping of electron spins in individual InGaAs quantum dots leads to strong nuclear polarisation that we measure via the Overhauser shift (OHS) in magneto-photoluminescence experiments between 0 and 4T. We find a…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 P. -F. Braun , B. Urbaszek , T. Amand , X. Marie , O. Krebs , B. Eble , A. Lemaitre , P. Voisin

We analyze nuclear spin dynamics in quantum dots and defect centers with a bound electron under electron-mediated coupling between nuclear spins due to the hyperfine interaction ("J-coupling" in NMR). Our analysis shows that the Overhauser…

Mesoscale and Nanoscale Physics · Physics 2008-11-04 D. Klauser , W. A. Coish , Daniel Loss

We report measurements of enhanced tensor polarization on solid-state targets. The results here represent an increase in tensor polarization over that previously achieved in high energy and nuclear scattering experiments that focused on the…

Instrumentation and Detectors · Physics 2020-08-24 Dustin Keller , Don Crabb , Donal Day

Hyperfine interactions with a nuclear spin environment fundamentally limit the coherence properties of confined electron spins in the solid-state. Here, we show that a quantum interference effect in optical absorption from two electronic…

Mesoscale and Nanoscale Physics · Physics 2012-05-16 Mena Issler , Eric Kessler , Geza Giedke , Susanne Yelin , Ignacio Cirac , Mikhail Lukin , Atac Imamoglu

We theoretically investigate the controlled dynamic polarization of lattice nuclear spins in GaAs double quantum dots containing two electrons. Three regimes of long-term dynamics are identified, including the build up of a large difference…

Mesoscale and Nanoscale Physics · Physics 2012-11-07 M. Gullans , J. J. Krich , J. M. Taylor , H. Bluhm , B. I. Halperin , C. M. Marcus , M. Stopa , A. Yacoby , M. D. Lukin

We present a quantum mechanical theory of optically induced dynamic nuclear polarization applicable to quantum dots and other interacting spin systems. The exact steady state of the optically driven coupled electron-nuclear system is…

Mesoscale and Nanoscale Physics · Physics 2019-02-04 Thomas Nutz , Edwin Barnes , Sophia E. Economou

Dynamic nuclear polarization (DNP) is a method of enhancing NMR signals via the transfer of polarization from electron spins to nuclear spins using on-resonance microwave (MW) irradiation. In most cases, monochromatic continuous-wave (MCW)…

Chemical Physics · Physics 2022-11-17 Daphna Shimon , Kelly A. Cantwell , Linta Joseph , Chandrasekhar Ramanathan

Electron spin dephasing in a singly charged semiconductor quantum dot can partially be suppressed by periodic laser pulsing. We propose a semi-classical approach describing the decoherence of the electron spin polarization governed by the…

Mesoscale and Nanoscale Physics · Physics 2017-11-15 Natalie Jäschke , Andreas Fischer , E. Evers , V. V. Belykh , Alex Greilich , Manfred Bayer , Frithjof B. Anders

Nuclear electric resonance (NER) spectroscopy is currently experiencing a revival as a tool for nuclear spin-based quantum computing. Compared to magnetic or electric fields, local electron density fluctuations caused by changes in the…

Quantum Physics · Physics 2025-01-30 Johannes K. Krondorfer , Andreas W. Hauser

We study the spin dynamics in charged quantum dots in the situation where the resident electron is coupled to only about 200 nuclear spins and where the electron spin splitting induced by the Overhauser field does not exceed markedly the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 D. H. Feng , I. A. Akimov , F. Henneberger

Electron-nuclear spin interactions by pulsed optical pumping have been found to polarize the nuclear spin system, leading to the nuclei building up an intrinsic magnetic field known as the Overhauser field. Studies have indicated an…

Mesoscale and Nanoscale Physics · Physics 2025-02-04 Estefanio Kesto , Michael J. Dominguez , Vanessa Sih

We propose a scheme for the deterministic generation of steady-state entanglement between the two nuclear spin ensembles in an electrically defined double quantum dot. Due to quantum interference in the collective coupling to the electronic…

Mesoscale and Nanoscale Physics · Physics 2013-12-23 Martin J. A. Schuetz , Eric M. Kessler , Lieven M. K. Vandersypen , J. Ignacio Cirac , Geza Giedke

Single crystal silicon is an excellent system in which to explore dynamic nuclear polarization (DNP), as it exhibits a continuum of properties from metallic to insulating as a function of doping concentration and temperature. At low doping…

Materials Science · Physics 2011-09-09 Anatoly E. Dementyev , David G. Cory , Chandrasekhar Ramanathan

Linearly polarized light tuned slightly below the optical transition of the negatively charged exciton (trion) in a single quantum dot causes the spontaneous nuclear spin polarization (self-polarization) at a level close to 100%. The…

Mesoscale and Nanoscale Physics · Physics 2008-04-02 V. L. Korenev

We exploit spin noise spectroscopy (SNS) to directly observe build-up of dynamic nuclear polarization and relaxation of a perturbed nuclear spin-system to its equilibrium state in a single-shot experiment. The SNS experiments were performed…

We study a large ensemble of nuclear spins interacting with a single electron spin in a quantum dot under optical excitation and photon detection. When a pair of applied laser fields satisfy two-photon resonance between the two ground…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Dimitrije Stepanenko , Guido Burkard , Geza Giedke , Atac Imamoglu

The effect of nuclear spins in Fe/GaAs all-electrical spin-injection devices is investigated. At temperatures below 50 K, strong modifications of the non-local spin signal are found that are characteristic for hyperfine coupling between…

Mesoscale and Nanoscale Physics · Physics 2010-04-08 G. Salis , A. Fuhrer , S. F. Alvarado

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang