Related papers: Spin-orbit-dependent lifetimes of long-range Rydbe…
We describe the creation of a long-lived spin-orbit-coupled gas of quantum degenerate atoms using the most magnetic fermionic element, dysprosium. Spin-orbit-coupling arises from a synthetic gauge field created by the adiabatic following of…
Long-range Rydberg molecules are typically bound in wells formed in their oscillatory potential energy curves. In alkaline Rydberg molecules, bound vibrational states exist even when these potential wells are disrupted by level repulsion…
Long-range macrodimers formed by D-state cesium Rydberg atoms are studied in experiments and in calculations. Cesium 62DJ-62DJ Rydberg-atom macrodimers, bonded via long-range multipole interaction, are prepared by two-color…
We investigate the interaction between two rubidium atoms in highly excited Rydberg states, and find that very long-range potential wells exist. These wells are shown to support many bound states. We calculate the properties of the wells…
The formation of ultralong-range Rydberg molecules is a result of the attractive interaction between Rydberg electron and polarizable ground state atom in an ultracold gas. In the nondegenerate case the backaction of the polarizable atom on…
Ultralong-range Rydberg molecules, composed of an excited Rydberg atom and a ground-state atom, are characterized by large bond lengths, dipole moments, sensitivity to external fields, and an unusual binding mechanism based on low-energy…
We show that the recently observed class of long-range ion-Rydberg molecules can be divided into two families of states, which are characterised by their unique electronic structures resulting from the ion-induced admixture of quantum…
The theory is developed for one and two atom interactions when the atom has a Rydberg electron attached to a hyperfine split core state. This situation is relevant for some of the rare earth and alkaline earth atoms that have been proposed…
A remarkable property of Rydberg atoms is the possibility to create molecules formed by one highly excited atom and another atom in the ground state. The first realisation of such a Rydberg molecule has opened an active field of physical…
We report the creation of ultralong-range Sr$_2$ molecules comprising one ground-state $5s^2$ $^1S_0$ atom and one atom in a $5sns$ $^3S_1$ Rydberg state for $n$ ranging from 29 to 36. Molecules are created in a trapped ultracold atomic gas…
Arrays of Rydberg atoms interacting via dipole-dipole interactions offer a powerful platform for probing quantum many-body physics. However, these intrinsic interactions also determine and constrain the models -- and parameter regimes…
Attosecond noncollinear four wave mixing spectroscopy with one attosecond extreme ultraviolet (XUV) pulse and two few-cycle near-infrared (NIR) pulses was used to measure the autoionization decay lifetimes of inner valence electronic…
We explore the electronic structure and rovibrational properties of an ultralong-range triatomic Rydberg molecule formed by a Rydberg atom and a ground state heteronuclear diatomic molecule. We focus here on interaction of Rb($27s$) Rydberg…
The level structure of negative-ions near the electron detachment limit dictates the low-energy scattering of an electron with the parent neutral atom. We demonstrate that a single ultracold atom bound inside a Rydberg orbit forming an…
The exquisite properties of Rydberg levels make them particularly appealing for emerging quantum technologies. The lifetime of low-angular-momentum laser-accessible levels is however limited to a few $100\,\mu\mathrm{s}$ by optical…
Stability achieved by large angular momentum is ubiquitous in nature, with examples ranging from classical mechanics, over optics and chemistry, to nuclear physics. In atoms, angular momentum can protect excited electronic orbitals from…
We propose a new approach to excite ion-pair states of ultracold dimers. The central idea is a two-step process where first long-range Rydberg molecules are formed by photoassociation, which are then driven by stimulated emission towards…
The internal electric field of a Rydberg atom electron can bind a polar molecule to form a giant ultralong-range stable polyatomic molecule. Such molecules not only share their properties with Rydberg atoms, they possess huge permanent…
The coupling of an isolated quantum state to a continuum is typically associated with decoherence and decreased lifetime. Here, we demonstrate that Rydberg macrodimers, weakly bound pairs of Rydberg atoms, can overcome this dissipative…
We study the spontaneous dissociation of diatomic molecules produced in cold atomic gases via magnetically tunable Feshbach resonances. We provide a universal formula for the lifetime of these molecules that relates their decay to the…