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We present quantum algorithms for solving two problems regarding stochastic processes. The first algorithm prepares the thermal Gibbs state of a quantum system and runs in time almost linear in $\sqrt{N \beta/{\cal Z}}$ and polynomial in…

Quantum Physics · Physics 2017-01-11 Anirban Narayan Chowdhury , Rolando D. Somma

In computer simulations, quantum delocalization of atomic nuclei can be modeled making use of the Path Integral (PI) formulation of quantum statistical mechanics. This approach, however, comes with a large computational cost. By restricting…

Statistical Mechanics · Physics 2015-04-13 Karsten Kreis , Mark E. Tuckerman , Davide Donadio , Kurt Kremer , Raffaello Potestio

We consider Particle Gibbs (PG) as a tool for Bayesian analysis of non-linear non-Gaussian state-space models. PG is a Monte Carlo (MC) approximation of the standard Gibbs procedure which uses sequential MC (SMC) importance sampling inside…

Computation · Statistics 2018-04-18 Oliver Grothe , Tore Selland Kleppe , Roman Liesenfeld

Estimating thermal expectation values of quantum many-body systems is a central challenge in physics, chemistry, and materials science. Standard quantum Gibbs sampling protocols address this task by preparing the Gibbs state from scratch…

Quantum Physics · Physics 2026-03-24 Hongrui Chen , Jiaqing Jiang , Bowen Li , Lexing Ying

Classical simulations of quantum systems are notoriously difficult computational problems, with conventional state vector and tensor network methods restricted to quantum systems that feature only a small number of qudits. The recently…

Quantum Physics · Physics 2026-01-28 Ben Harper , Azar C. Nakhl , Thomas Quella , Martin Sevior , Muhammad Usman

The Markov property entails the conditional independence structure inherent in Gibbs distributions for general classical Hamiltonians, a feature that plays a crucial role in inference, mixing time analysis, and algorithm design. However,…

Quantum Physics · Physics 2025-04-04 Chi-Fang Chen , Cambyse Rouzé

Path integral molecular dynamics simulations, combined with an ab initio evaluation of interactions using electronic structure theory, incorporate the quantum mechanical nature of both the electrons and nuclei, which are essential to…

Chemical Physics · Physics 2016-02-15 Ondrej Marsalek , Thomas E. Markland

Preparing thermal (Gibbs) states is a common task in physics and computer science. Recent algorithms mimic cooling via system-bath coupling, where the cost is determined by mixing time, akin to classical Metropolis-like algorithms. However,…

Quantum Physics · Physics 2024-12-13 David Gamarnik , Bobak T. Kiani , Alexander Zlokapa

The dual tasks of quantum Hamiltonian learning and quantum Gibbs sampling are relevant to many important problems in physics and chemistry. In the low temperature regime, algorithms for these tasks often suffer from intractabilities, for…

Gibbs states (i.e., thermal states) can be used for several applications such as quantum simulation, quantum machine learning, quantum optimization, and the study of open quantum systems. Moreover, semi-definite programming, combinatorial…

Quantum Physics · Physics 2024-12-20 Norhan M. Eassa , Mahmoud M. Moustafa , Arnab Banerjee , Jeffrey Cohn

We present the path-integral solutions to the distributions in classical (Gibbs) and quantum (Wigner) statistical mechanics. The kernel of the distributions are derived in two ways - one by time slicing and defining the appropriate…

Statistical Mechanics · Physics 2016-08-24 Jose A. Magpantay , Cilicia Uzziel M. Perez

The quantum nature of nuclei plays an important role in the accurate modelling of light atoms such as hydrogen, but it is often neglected in simulations due to the high computational overhead involved. It has recently been shown that…

Computational Physics · Physics 2012-02-21 Michele Ceriotti , David E. Manolopoulos , Michele Parrinello

Gibbs sampling is a crucial computational technique used in physics, statistics, and many other scientific fields. For classical Hamiltonians, the most commonly used Gibbs sampler is the Metropolis algorithm, known for having the Gibbs…

Quantum Physics · Physics 2024-06-25 Jiaqing Jiang , Sandy Irani

Lindblad dynamics and other open-system dynamics provide a promising path towards efficient Gibbs sampling on quantum computers. In these proposals, the Lindbladian is obtained via an algorithmic construction akin to designing an artificial…

Quantum Physics · Physics 2025-03-07 Zhiyan Ding , Bowen Li , Lin Lin

Modern 4-wave mixing spectroscopies are expensive to obtain experimentally and computationally. In certain cases, the unfavorable scaling of quantum dynamics problems can be improved using a generalized quantum master equation (GQME)…

Chemical Physics · Physics 2024-05-16 Thomas Sayer , Andrés Montoya-Castillo

Quantum-based molecular dynamics (QMD) is a highly accurate and transferable method for material science simulations. However, the time scales and system sizes accessible to QMD are typically limited to picoseconds and a few hundred atoms.…

The contribution of nuclear quantum effects (NQEs) to the properties of various hydrogen-bound systems, including biomolecules, is increasingly recognized. Despite the development of many acceleration techniques, the computational overhead…

Chemical Physics · Physics 2024-07-08 Iryna Zaporozhets , Félix Musil , Venkat Kapil , Cecilia Clementi

Preparing ground states and thermal states is essential for simulating quantum systems on quantum computers. Despite the hope for practical quantum advantage in quantum simulation, popular state preparation approaches have been challenged.…

The quantum thermal average plays a central role in describing the thermodynamic properties of a quantum system. Path integral molecular dynamics (PIMD) is a prevailing approach for computing quantum thermal averages by approximating the…

Numerical Analysis · Mathematics 2024-06-25 Xuda Ye , Zhennan Zhou

Quantum computers solve intractable problems which classically require an exponentially long time to compute. With the development of large-scale experiments that claim quantum advantage, a vital issue has now emerged. What are the errors,…

Quantum Physics · Physics 2026-04-15 Ned Goodman , Alexander S. Dellios , Margaret D. Reid , Peter D. Drummond