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The total energy of the transverse spin-spiral wave as a function of the wave vector for all 3$d$ transition metal atomic chains has been calculated within {\it ab initio} density functional theory with generalized gradient approximation.…

Materials Science · Physics 2015-05-27 J. C. Tung , G. Y. Guo

Based on density functional theory band structure calculations, quantum Monte-Carlo simulations, and high-field magnetization measurements, we address the microscopic magnetic model of BaAg2Cu[VO4]2 that was recently proposed as a spin-1/2…

Materials Science · Physics 2012-06-19 Alexander A. Tsirlin , Angela Moeller , B. Lorenz , Yu. Skourski , H. Rosner

A site-selective $^{27}$Al nuclear magnetic resonance (NMR) study is carried out on the Kondo lattice compound CePtAl$_4$Ge$_2$, which crystallizes in a rhombohedral lattice with quasi-two-dimensional Ce layers forming a triangular lattice…

Strongly Correlated Electrons · Physics 2025-12-11 H. Sakai , S. Shin , S. Kambe , Y. Tokunaga , H. Harima , E. Pomjakushina , T. Park

Recently synthesized Rh-Ni trinuclear complexes hexacoordinated with sulfur ions, 3-aminopropanethiolate (apt) metalloligand [Ni{Rh(apt)$_{3}$}$_{2}$](NO$_{3}$)$_{n}$ ($n$ = 2, 3, 4), are found to be chemically interconvertible between the…

Strongly Correlated Electrons · Physics 2020-05-04 K. Yamagami , S. Imada , K. Yamanaka , T. Yaji , A. Tanaka , M. Kouno , N. Yoshinari , T. Konno , A. Sekiyama

In a straightforward application of molecular nanospintronics to quantum computing, single-molecule spin transistors can be used to measure and control nuclear spin qubits. A jump in the conductance occurs when the electronic spin inverts…

Mesoscale and Nanoscale Physics · Physics 2018-01-12 Salvador Cardona-Serra , Alejandro Gaita-Ariño , Maria Stamenova , Stefano Sanvito

We develop a microscopic theory of finite-temperature spin-nematic orderings in three-dimensional spatially anisotropic magnets consisting of weakly-coupled frustrated spin-1/2 chains with nearest-neighbor and next-nearest-neighbor…

Strongly Correlated Electrons · Physics 2013-02-19 Masahiro Sato , Toshiya Hikihara , Tsutomu Momoi

A Mn dopant in a III-V semiconductor produces a highly-entangled, coherent triplet ground state not fully captured by single-determinant theories of electron structure. We directly construct an analytic form for its ground-state…

Mesoscale and Nanoscale Physics · Physics 2025-12-02 Julian Zanon , Michael E. Flatté

It is found that all the zigzag chains except the nonmagnetic (NM) Ni and antiferromagnetic (AF) Fe chains which form a twisted two-legger ladder, look like a corner-sharing triangle ribbon, and have a lower total energy than the…

Materials Science · Physics 2009-11-13 J. C. Tung , G. Y. Guo

Collective motions in strongly interacting magnets involve many spins and are often described in terms of integer-spin excitations. However, in certain cases, the collective motion can behave as if these integer excitations break apart into…

Motivated by the recent experimental progress on the strong spin-orbit-coupled rare earth triangular antiferromagnet, we analyze the highly anisotropic spin model that describes the interaction between the spin-orbit-entangled Kramers'…

Strongly Correlated Electrons · Physics 2016-07-13 Yao-Dong Li , Xiaoqun Wang , Gang Chen

Structural and magnetic properties of a two-dimensional spin-$\frac{5}{2}$ frustrated triangular lattice antiferromagnet NH$_{4}$Fe(PO$_{3}$F)$_2$ are explored via x-ray diffraction, magnetic susceptibility, high-field magnetization, heat…

Materials Science · Physics 2025-02-11 S. Mohanty , K. M. Ranjith , C. S. Saramgi , Y. Skourski , B. Büchner , H. -J. Grafe , R. Nath

The compounds $Ln$AuAl$_4$Ge$_2$ ($Ln$ $=$ lanthanide) form in a structure that features two-dimensional triangular lattices of $Ln$ ions that are stacked along the crystalline $c$ axis. Together with crystal electric field effects,…

Strongly Correlated Electrons · Physics 2024-01-03 Keke Feng , Caleb Bush , Olatunde Oladehin , Minhyea Lee , Ryan Baumbach

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

We report on the microscopic magnetic model of a spin-1/2 magnet BaV$_3$O$_8$. In contrast to earlier phenomenological analysis, our density-functional band-structure calculations combined with quantum Monte-Carlo simulations establish a…

Materials Science · Physics 2014-01-09 Alexander A. Tsirlin

1H nuclear magnetic resonance (NMR) measurements in [YPc2]0, an organic compound formed by radicals stacking along chains, are presented. The temperature dependence of the macroscopic susceptibility, of the NMR shift and of the spin-lattice…

Strongly Correlated Electrons · Physics 2015-05-20 F. Branzoli , P. Carretta , M. Filibian , S. Klyatskaya , M. Ruben

The frustrated spin-1/2 model with weakly anisotropic ferromagnetic nearest-neighbor and antiferromagnetic next-nearest-neighbor exchanges is studied with use of variational mean-field approach, scaling estimates of the infrared…

Strongly Correlated Electrons · Physics 2009-11-13 D. V. Dmitriev , V. Ya. Krivnov

We investigate a highly frustrated spin-1 model on the triangular lattice, with nearest- and next-nearest-neighbor antiferromagnetic $S\cdot S$ interactions and nearest-neighbor $(S\cdot S)^2$ interactions. Using the density matrix…

Strongly Correlated Electrons · Physics 2022-09-21 Aaron Szasz , Chong Wang , Yin-Chen He

The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

Strongly Correlated Electrons · Physics 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

We explore the spin states in the quantum spin chain compound SrCo$_{2}$V$_{2}$O$_{8}$ up to 14.9 T and down to 50 mK, using single-crystal neutron diffraction. Upon cooling in zero-field, antiferromagnetic (AFM) order of N\'eel type…

Strongly Correlated Electrons · Physics 2019-07-05 L. Shen , O. Zaharko , J. O. Birk , E. Jellyman , Z. He , E. Blackburn

We report thermodynamic properties, magnetic ground state, and microscopic magnetic model of the spin-1 frustrated antiferromaget Li$_{2}$NiW$_{2}$O$_{8}$ showing successive transitions at $T_{\rm N1}\simeq 18$ K and $T_{\rm N2}\simeq 12.5$…

Materials Science · Physics 2016-07-14 K. M. Ranjith , R. Nath , M. Majumder , D. Kasinathan , M. Skoulatos , L. Keller , Y. Skourski , M. Baenitz , A. A. Tsirlin