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Complex Antiferromagnetic Order in the Metallic Triangular Lattice Compound SmAuAl$_4$Ge$_2$

Strongly Correlated Electrons 2024-01-03 v2 Materials Science

Abstract

The compounds LnLnAuAl4_4Ge2_2 (LnLn == lanthanide) form in a structure that features two-dimensional triangular lattices of LnLn ions that are stacked along the crystalline cc axis. Together with crystal electric field effects, magnetic anisotropy, and electron-mediated spin exchange interactions, this sets the stage for the emergence of strongly correlated spin and electron phenomena. Here we investigate SmAuAl4_4Ge2_2, which exhibits weak paramagnetism that strongly deviates from conventional Curie-Weiss behavior. Complex antiferromagnetic ordering emerges at TN1T_{\rm{N1}} == 13.2 K and TN2T_{\rm{N2}} == 7.4 K, where heat capacity measurements show that these transitions are first and second order, respectively. These measurements also reveal that the Sommerfeld coefficient is not enhanced compared to the nonmagnetic analog YAuAl4_4Ge2_2, consistent with the charge carrier quasiparticles exhibiting typical Fermi liquid behavior. The temperature-dependent electrical resistivity follows standard metallic behavior, but linear magnetoresistance unexpectedly appears within the ordered state. We compare these results to other LnLnAuAl4_4Ge2_2 materials, which have already been established as localized ff-electron magnets that are hosts for interesting magnetic and electronic phases. From this, SmAuAl4_4Ge2_2 emerges as a complex quantum spin metal, inviting further investigations into its properties and the broader family of related materials.

Keywords

Cite

@article{arxiv.2308.13945,
  title  = {Complex Antiferromagnetic Order in the Metallic Triangular Lattice Compound SmAuAl$_4$Ge$_2$},
  author = {Keke Feng and Caleb Bush and Olatunde Oladehin and Minhyea Lee and Ryan Baumbach},
  journal= {arXiv preprint arXiv:2308.13945},
  year   = {2024}
}

Comments

9 pages, 6 figures