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Liquid-liquid phase separation of liquids exhibiting interconversion between alternative states has been proposed as an underlying mechanism for fluid polyamorphism, and may be of relevance to protein function and intracellular…

Statistical Mechanics · Physics 2021-12-08 Betul Uralcan , Thomas J. Longo , Mikhail A. Anisimov , Frank H. Stillinger , Pablo G. Debenedetti

The interplay between the structure and dynamics of partially confined Lennard Jones (LJ) fluids, deep into the supercritical phase, is studied over a wide range of densities in the context of the Frenkel line (FL), which separates rigid…

Statistical Mechanics · Physics 2019-03-20 Kanka Ghosh , C. V. Krishnamurthy

We study a robust model of self-propelled rods interacting via volume exclusion and show that its collective dynamics encompasses both that of the corresponding Vicsek-style model (where local alignment is the sole interaction), and…

Soft Condensed Matter · Physics 2018-07-04 Xia-qing Shi , Hugues Chaté

We study a system of interacting active particles, propelled by colored noises, characterized by an activity time {\tau}, and confined by a single-well anharmonic potential. We assume pair-wise repulsive forces among particles, modelling…

Statistical Mechanics · Physics 2018-10-31 Lorenzo Caprini , Umberto Marini Bettolo Marconi , Andrea Puglisi

Active forces occurring within cells can drive crucial biological processes that involve spontaneous organization and shape change, such as cell division. Motivated by recent in vitro experiments of nematic droplets of cytoskeletal…

Soft Condensed Matter · Physics 2021-02-16 Fabian Jan Schwarzendahl , Pierre Ronceray , Kimberly L. Weirich , Kinjal Dasbiswas

The effect of confinement on the phase behaviour and structure of fluids made of biaxial hard particles (cuboids) is examined theoretically by means of Onsager second-order virial theory in the limit where the long particle axes are frozen…

Soft Condensed Matter · Physics 2022-06-07 Szabolcs Varga , Yuri Martinez-Raton , Enrique Velasco

Employing X-ray photon correlation spectroscopy we measure the kinetics and dynamics of a pressure-induced liquid-liquid phase separation (LLPS) in a water-lysozyme solution. Scattering invariants and kinetic information provide evidence…

Soft Condensed Matter · Physics 2021-07-13 M. Moron , A. Al-Masoodi , C. Lovato , M. Reiser , L. Randolph , G. Surmeier , J. Bolle , F. Westermeier , M. Sprung , R. Winter , M. Paulus , C. Gutt

Using molecular dynamics simulations we study the slow dynamics of a hard sphere fluid confined in a disordered porous matrix. The presence of both discontinuous and continuous glass transitions as well as the complex interplay between…

Soft Condensed Matter · Physics 2009-09-29 Jan Kurzidim , Daniele Coslovich , Gerhard Kahl

We present the Brownian dynamics simulation of active colloidal suspension in two dimensions, where the self-propulsion speed of a colloid is regulated according to the local density sensed by it. The role of concentration-dependent…

Soft Condensed Matter · Physics 2021-01-29 Francis Jose , Shalabh K. Anand , Sunil P. Singh

Low Reynolds number direct simulations of large populations of hydrodynamically interacting swimming particles confined between planar walls are performed. The results of simulations are compared with a theory that describes dilute…

Fluid Dynamics · Physics 2015-05-13 Juan P. Hernandez-Ortiz , Patrick T. Underhill , Michael D. Graham

We show that spontaneous density segregation in dense systems of aligning circle swimmers is a condensation phenomenon at odds with the phase separation scenarios usually observed in two-dimensional active matter. The condensates, which…

Soft Condensed Matter · Physics 2024-12-20 Yujia Wang , Bruno Ventéjou , Hugues Chaté , Xia-qing Shi

We combine numerical and analytical methods to study two dimensional active crystals formed by permanently linked swimmers and with two distinct alignment interactions. The system admits a stationary phase with quasi long range…

Soft Condensed Matter · Physics 2021-12-22 Chen Huang , Leiming Chen , Xiangjun Xing

It is found experimentally that the coexistence region of a vapor-liquid system or a binary mixture is substantially narrowed when the fluid is confined in a aerogel with a high degree of porosity (e.g. of the order of 95% to 99%). A…

Statistical Mechanics · Physics 2007-05-23 Rafael Salazar , Raul Toral , Amitabha Chakrabarti

The spontaneous emergence of collective flows is a generic property of active fluids and often leads to chaotic flow patterns characterised by swirls, jets, and topological disclinations in their orientation field. However, the ability to…

Soft Condensed Matter · Physics 2017-03-07 Tyler N. Shendruk , Amin Doostmohammadi , Kristian Thijssen , Julia M. Yeomans

We investigate finite-size effects on diffusion in confined fluids using molecular dynamics simulations and hydrodynamic calculations. Specifically, we consider a Lennard-Jones fluid in slit pores without slip at the interface and show that…

Computational Physics · Physics 2017-03-16 Pauline Simonnin , Benoit Noetinger , Carlos Nieto-Draghi , Virginie Marry , Benjamin Rotenberg

Phase coarsening is a fundamental process of microstructure evolution in multiphase materials. A thorough understanding of its kinetics is of great significance for material processing and performance. Generally, coarsening can be divided…

Materials Science · Physics 2022-04-27 Yue Li , Zhijun Wang , Xianghan Gao , Yujian Wang , Junjie Li , Jincheng Wang

We study theoretically the evaporation-driven phase separation of a binary fluid mixture in a thin film deposited on a moving substrate, as occurs in meniscus-guided deposition for solution-processed materials. Our focus is on rapid…

Soft Condensed Matter · Physics 2024-07-01 René de Bruijn , Anton A. Darhuber , Jasper J. Michels , Paul van der Schoot

Recently, there has been much interest in activity-induced phase separations in concentrated suspensions of "active Brownian particles" (ABPs), self-propelled spherical particles whose direction of motion relaxes through thermal rotational…

Soft Condensed Matter · Physics 2014-02-13 Joakim Stenhammar , Davide Marenduzzo , Rosalind J. Allen , Michael E. Cates

We study the steady states and the coarsening dynamics in a one dimensional driven non-conserved system modelled by the so called driven Allen-Cahn equation, which is the standard Allen-Cahn equation with an additional driving force. In…

Statistical Mechanics · Physics 2022-08-17 Rajiv G Pereira

Active matter is not only indispensable to our understanding of diverse biological processes, but also provides a fertile ground for discovering novel physics. Many emergent properties impossible for equilibrium systems have been…

Soft Condensed Matter · Physics 2022-05-27 Thibault Bertrand , Chiu Fan Lee