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We demonstrate in this paper that the recently discovered infinite-layer (IL) nickelates have much in common with a class of materials known as electrides. Oxide based electrides are compounds in which topotactic removal of loosely bound…

Superconductivity · Physics 2023-11-30 Kateryna Foyevtsova , Ilya Elfimov , George A. Sawatzky

The recent discovery of Ruddlesden--Popper (RP) nickelate thin-film superconductors has opened a new frontier in unconventional superconductivity. Its realization requires both compressive epitaxial strain and highly oxidative growth…

A promising route to tailoring the electronic properties of quantum materials and devices rests on the idea of orbital engineering in multilayered oxide heterostructures. Here we show that the interplay of interlayer charge imbalance and…

The electronic structure of a LaNiO$_3$ bilayer grown along the [111] direction and confined between insulating layers of LaAlO$_3$ is theoretically investigated using a combination of first principle calculations and effective…

Strongly Correlated Electrons · Physics 2012-06-28 Andreas Rüegg , Chandrima Mitra , Alexander A. Demkov , Gregory A. Fiete

The discovery of high-temperature superconductivity near 80 K in bilayer nickelate La$_3$Ni$_2$O$_7$ under high pressures has renewed the exploration of superconducting nickelate in bulk materials. The extension of superconductivity in…

Superconductivity · Physics 2024-03-28 Qing Li , Ying-Jie Zhang , Zhe-Ning Xiang , Yuhang Zhang , Xiyu Zhu , Hai-Hu Wen

The metal-insulator transition (MIT) of bulk rare-earth nickelates is accompanied by a simultaneous charge ordering (CO) transition. We have investigated low-frequency resistance fluctuations (noise) across the MIT and magnetic transition…

Strongly Correlated Electrons · Physics 2019-09-05 Gopi Nath Daptary , Siddharth Kumar , M. Kareev , J. Chakhalian , Aveek Bid , S. Middey

The $T^{\prime}$ infinite layered nickelates have recently garnered significant attention owing to the discovery of superconductivity in hole-doped RNiO$_2$ (R $=$ La, Pr, or Nd), which is the $n = \infty$ member of the series…

Strongly Correlated Electrons · Physics 2023-11-10 Dibyata Rout , Sanchayeta Ranajit Mudi , Suman Karmakar , Rajeev Rawat , Surjeet Singh

The recent discovery of Sr-doped infinite-layer nickelate $\textrm{NdNiO}_2$ [D. Li et al. Nature 572, 624 (2019)] offers an exciting platform for investigating unconventional superconductivity in nickelatebased compounds. In this work, we…

Strongly Correlated Electrons · Physics 2020-05-19 Zhao Liu , Zhi Ren , W. Zhu , Z. F. Wang , Jinlong Yang

The recent discovery of high-$T_c$ superconductivity in Ruddlesden-Popper (RP) nickelates has motivated extensive efforts to explore higher $T_c$ superconductors. Here, we systematically investigate Nd-doped La$_3$Ni$_2$O$_7$ using density…

Superconductivity · Physics 2026-01-06 Cui-Qun Chen , Wenyuan Qiu , Zhihui Luo , Meng Wang , Dao-Xin Yao

The discovery of superconductivity with a critical temperature of about 80~K in La$_{3}$Ni$_{2}$O$_{7}$ single crystals under pressure has received enormous attention. La$_{3}$Ni$_{2}$O$_{7}$ is not superconducting under ambient pressure…

Superconductivity · Physics 2024-09-12 Zhe Liu , Mengwu Huo , Jie Li , Qing Li , Yuecong Liu , Yaomin Dai , Xiaoxiang Zhou , Jiahao Hao , Yi Lu , Meng Wang , Hai-Hu Wen

Recently, a signature of high-temperature superconductivity above the liquid nitrogen temperature (77 K) was reported for $La_{3}Ni_{2}O_{7-\delta}$ under pressure. This finding immediately stimulated intense interest in the possible…

Superconductivity · Physics 2025-06-13 Dan Zhao , Yanbing Zhou , Mengwu Huo , Yu Wang , Linpeng Nie , Ye Yang , Jianjun Ying , Meng Wang , Tao Wu , Xianhui Chen

The discovery of pressure-induced superconductivity in two- and three-layer Ruddlesden-Popper nickelates has generated significant interest in these materials as a platform for unconventional superconductivity. While their ground state…

We conduct first-principles simulations of La$_3$Ni$_2$O$_7$, a nickelate in which recent experiments have shown signs of high-temperature superconductivity. Within the hydrostatic pressure range where superconductivity is observed, we find…

Superconductivity · Physics 2026-02-25 Daan Verraes , Tom Braeckevelt , Nick Bultinck , Veronique Van Speybroeck

The electronic structure of La2NiO4+d, where additional oxygen interstitials are forming stripes along (1,1,0), are presented. Spin-polarized calculations show that ferromagnetism on Ni sites is reduced near the stripes and enhanced far…

Materials Science · Physics 2017-01-04 Thomas Jarlborg , Antonio Bianconi

We elucidate the electronic structure and quantum many-body instabilities of the monolayer nickelate La2NiO4 under hydrostatic pressure using a combination of density functional theory, dynamical mean-field theory (DFT+DMFT), and random…

Strongly Correlated Electrons · Physics 2025-11-20 Shu-Hong Tang , Han-Yu Wang , Da-Yong Liu , Feng Lu , Wei-Hua Wang , H. -Q. Lin , Liang-Jian Zou

The observation of superconductivity in infinite layer nickelate (Nd,Sr)NiO$_{2}$ thin films has led to rapid theoretical and experimental investigations of these copper-oxide-analogue systems [1-15]. Superconductivity has also been found…

The extent to which electronic dimensionality influences magnetism and superconductivity in Ruddlesden-Popper (RP) nickelates remains unsettled. Here we report high-precision crystallographic-axis-resolved dc transport measurements on…

Strongly Correlated Electrons · Physics 2026-05-19 Feiyang Liu , Lixing Chen , Enkang Zhang , Ying-Jie Zhang , Jun Zhao

We consider a two-dimensional electron gas (2DEG) formed at a near-ferroelectric interface and strongly coupled to polar phonons. Through a self-consistent microscopic many-body calculation, we show that the coupled system stabilizes a…

Strongly Correlated Electrons · Physics 2026-03-04 Fei Yang , Zhi-Yang Wang , Long-Qing Chen

The recent discovery of pressure-induced superconductivity in the bilayer La$_3$Ni$_2$O$_7$ (LNO) has opened a new platform for the study of unconventional superconductors. In this publication, we investigate theoretically the whole family…

Superconductivity · Physics 2023-10-30 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Thomas A. Maier , Elbio Dagotto

Evidence of superconductivity (SC) has recently been reported in pressurized La3Ni2O7 and La4Ni3O10, providing a new platform to explore high-temperature superconductivity. However, while zero resistance state has been observed,…