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We report on a comprehensive study of the electronic and magnetic structure of the striped nickelate La5/3Sr1/3NiO4. The investigation is carried out using band structure calculations based on density functional theory. A magnetic structure…

Strongly Correlated Electrons · Physics 2008-02-25 U. Schwingenschlogl , C. Schuster , R. Fresard

The discovery of high-$T_c$ superconductivity in Ruddlesden-Popper nickelates has sparked substantial effort towards understanding unconventional electronic states beyond a traditional cuprate-like d^9 configurational ground state. An…

Charge order is a central feature of the physics of cuprate superconductors and is known to arise from a modulation of holes with primarily oxygen character. Low-valence nickelate superconductors also host charge order, but the electronic…

Strongly Correlated Electrons · Physics 2023-03-29 Y. Shen , J. Sears , G. Fabbris , J. Li , J. Pelliciari , M. Mitrano , W. He , Junjie Zhang , J. F. Mitchell , V. Bisogni , M. R. Norman , S. Johnston , M. P. M. Dean

The quasi-two-dimensional nickelate La4Ni3O8 (La-438) is an anion deficient n=3 Ruddlesden-Popper (R-P) phase that consists of trilayer networks of square planar Ni ions, formally assigned as Ni1+ and Ni2+ in a 2:1 ratio. While previous…

Strongly Correlated Electrons · Physics 2016-08-17 Junjie Zhang , Yu-Sheng Chen , D. Phelan , Hong Zheng , M. R. Norman , J. F. Mitchell

Strongly-correlated transition-metal oxides are widely known for their various exotic phenomena. This is exemplified by rare-earth nickelates such as LaNiO$_{3}$, which possess intimate interconnections between their electronic, spin, and…

Using the DFT+dynamical mean-field theory approach we study the effects of electronic correlations and doping on the normal state electronic structure of the double-layer nickelate superconductor La$_3$Ni$_2$O$_7$ under pressure. In…

Strongly Correlated Electrons · Physics 2026-04-27 I. V. Leonov

Density functional theory is used to investigate the effect of biaxial strain on the structural, electronic and magnetic properties of [111]-oriented NdNiO$_3$, as a representative of the rare-earth perovskites that undergo…

Materials Science · Physics 2025-07-29 Alexander Lione , Jorge Íñiguez-González , Nicholas C. Bristowe

Controlled introduction of oxygen vacancies offers an effective route to induce metal-to-insulator transition in strongly correlated rare-earth nickelates ($R$NiO$_3$) at room temperature. However, the role played by the rare-earth cations…

Materials Science · Physics 2024-12-30 Devang Bhagat , Ranga Teja Pidathala , Badri Narayanan

We introduce ultrafast low-energy electron diffraction (ULEED) in backscattering for the study of structural dynamics at surfaces. Using a tip-based source of ultrashort electron pulses, we investigate the optically-driven transition…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 S. Vogelgesang , G. Storeck , S. Schramm , K. Rossnagel , S. Schäfer , C. Ropers

The recent discovery of superconductivity with a transition temperature $T_c$ exceeding 40 K in La$_3$Ni$_2$O$_7$ and (La,Pr)$_{3}$Ni$_2$O$_7$ thin films at ambient pressure marks a significant breakthrough in the field of nickelate…

Superconductivity · Physics 2026-01-07 Xunwu Hu , Wenyuan Qiu , Cun-Qun Chen , Zhihui Luo , Dao-Xin Yao

We use density functional plus $U$ methods to study the effects of a tensile or compressive substrate strain on the charge-ordered insulating phase of LuNiO$_3$. The numerical results are analyzed in terms of a Landau energy function, with…

Strongly Correlated Electrons · Physics 2015-06-03 Zhuoran He , Andrew J. Millis

Determining the electronic structure of La$_3$Ni$_2$O$_7$ is an essential step towards uncovering their superconducting mechanism. It is widely believed that the bilayer apical oxygens play an important role in the bilayer La$_3$Ni$_2$O$_7$…

Superconductivity · Physics 2025-04-30 Yuxin Wang , Yi Zhang , Kun Jiang

TThe isotope effect is a powerful probe of electron-phonon interactions in solid-state systems, offering key insights into how atomic mass influences emergent quantum states. Here, the impact of oxygen isotope substitution ($^{16}{\rm…

In pursuit of rational control of orbital polarization, we present a combined experimental and theoretical study of single unit cell superlattices of the correlated metal LaNiO$_3$ and the band insulator LaAlO$_3$. Polarized x-ray…

Strongly Correlated Electrons · Physics 2012-01-23 J. W. Freeland , Jian Liu , M. Kareev , B. Gray , J. W. Kim , P. Ryan , R. Pentcheva , J. Chakhalian

The intrinsic electronic properties of La$_3$Ni$_2$O$_{7}$ have been selectively investigated by nuclear quadrupole resonance (NQR) at the La(2) site outside the NiO$_2$ bilayers. The La(2)$_{\rm a}$ site of the ideal La$_3$Ni$_2$O$_{7}$ is…

Strongly Correlated Electrons · Physics 2025-04-18 Mitsuharu Yashima , Nina Seto , Yujiro Oshita , Masataka Kakoi , Hiroya Sakurai , Yoshihiko Takano , Hidekazu Mukuda

By using the pulsed-laser-ablation technique, we have successfully grown the La$_{3}$Ni$_{2}$O$_{7-\delta}$ thin films with $c$-axis orientation perpendicular to the film surface. X-ray diffraction shows that the (00l) peaks can be well…

Superconductivity · Physics 2025-10-10 Yuecong Liu , Mengjun Ou , Haifeng Chu , Huan Yang , Qing Li , Yingjie Zhang , Hai-Hu Wen

A hypothetical layered oxide La_2NiMO_6 where NiO_2 and MO_2 planes alternate along the c-axis of ABO_3 perovskite lattice is considered theoretically. Here, M denotes a trivalent cation Al, Ga,... such that MO_2 planes are insulating and…

Strongly Correlated Electrons · Physics 2010-05-11 Jiri Chaloupka , Giniyat Khaliullin

Systematically controlling the superconducting transition temperature ($T_\text{c}$) in the bilayer Ruddlesden-Popper nickelate La$_3$Ni$_2$O$_7$ remains a significant challenge. Here, we address this by synthesizing high-quality…

Motivated by the recent discovery of superconductivity in the pentalayer nickelate Nd$_6$Ni$_5$O$_{12}$ [Nature Materials 10.1038], we calculate its electronic structure and superconducting critical temperature. We find that electronic…

Superconductivity · Physics 2022-09-08 Paul Worm , Liang Si , Motoharu Kitatani , Ryotaro Arita , Jan M. Tomczak , Karsten Held

In this work, we investigate collective electronic fluctuations and, in particular, the possibility of the charge density wave ordering in an infinite-layer NdNiO$_2$. We perform advanced many-body calculations for the ab-initio…

Strongly Correlated Electrons · Physics 2024-06-03 Evgeny A. Stepanov , Matteo Vandelli , Alexander I. Lichtenstein , Frank Lechermann