Related papers: Forbidden second harmonics in centrosymmetric bila…
Second-order nonlinear optical processes are fundamental to photonics, spectroscopy, and information technologies, with material platforms playing a pivotal role in advancing these applications. Here, we demonstrate the exceptional…
The inherently weak nonlinear optical response of bulk materials remains a fundamental limitation in advancing photonic technologies. Nanophotonics addresses this challenge by tailoring the size and morphology of nanostructures to…
Layered NbOX$_2$ ($X=\mathrm{Cl,\,Br,\,I}$), a member of the van der Waals ferroelectric family, exhibits intrinsic ferroelectricity and pronounced nonlinear optical responses, making it a promising candidate for integrated nanophotonics…
Second Harmonic Generation Microscopy (SHG) is generally acknowledged as a powerful tool for the label-free 3D visualization of tissues and advanced materials, with one of its most popular applications being collagen imaging. Although the…
Nonlinear optical generation has been a well-established way to realize frequency conversion in nonlinear optics, whereas previous studies were just focusing on the scalar light fields. Here we report a concise yet efficient experiment to…
Two-dimensional (2D) materials serve as exceptional platforms for controlled second harmonic generation (SHG), an important nonlinear optical phenomenon with diverse applications. Current approaches to SHG control often depend on…
High harmonic generation (HHG) in crystals has revealed a wealth of perspectives such as all-optical mapping of the electronic band structure, ultrafast quantum information and the creation of novel all-solid-state attosecond sources.…
We report terahertz (THz) second harmonic generation (SHG) in superconductors (SC) with inversion symmetric equilibrium states that forbid even-order nonlinearities. Such SHG signal is observed in single-pulse emission by periodic driving…
High-power infrared laser systems with broadband tunability are of great importance due to their wide range of applications in spectroscopy and free-space communications. These systems require nonlinear optical (NLO) crystals for wavelength…
Nonlinear optical phenomena in nanostructured materials have been challenging our perceptions of nonlinear optical processes that have been explored since the invention of lasers. For example, the ability to control optical field…
Remarkable optical and electrical properties of two-dimensional (2D) materials, such as graphene and transition-metal dichalcogenide (TMDC) monolayers, offer vast technological potential for novel and improved optoelectronic nanodevices,…
Optical frequency conversion processes in nonlinear materials are limited in wavelength by the accessible phase matching and the required high pump powers. In this letter, we report a novel broadband phase matching (PM) technique in high…
High-harmonic spectroscopy driven by circularly-polarized laser pulses and their counter-rotating second harmonic is a new branch of attosecond science which currently lacks quantitative interpretations. We extend this technique to the…
Material systems with lone-pair electrons have long been a treasure trove in the search for large second harmonic generation effects. Revealing the origin of second harmonic generation in nonlinear optical materials can provide theoretical…
In the second-order response regime, the Hall voltage can be nonzero without breaking the time-reversal symmetry, as long as the system is noncentrosymmetric. There are multiple mechanisms with different scaling rules that contribute to the…
Dynamic phase-only beam shaping with a liquid crystal spatial light modulator is a powerful technique for tailoring the beam's intensity profile or wave front. While shaping and controlling the light field is a highly researched topic,…
High-harmonic generation (HHG) is a strong-field phenomenon that is sensitive to the attosecond dynamics of tunnel ionization and coherent transport of electron-hole pairs in solids. While the foundations of solid HHG have been established,…
Layered van der Waals (vdW) materials have emerged as a promising platform for nanophotonics due to large refractive indexes and giant optical anisotropy. Unlike conventional dielectrics and semiconductors, the absence of covalent bonds…
The enhanced electric field at plasmonic resonances in nanoscale antennas can lead to efficient harmonic generation, especially when the plasmonic geometry is asymmetric on either inter-particle or intra-particle levels. The planar…
Intense efforts have been made in recent years to realize nonlinear optical interactions at the single-photon level. Much of this work has focused on achieving strong third-order nonlinearities, such as by using single atoms or other…