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We have observed an electronic energy level crossing in a molecular nanomagnet (MNM) using muon-spin relaxation. This effect, not observed previously despite several muon studies of MNM systems, provides further evidence that the spin…

Strongly Correlated Electrons · Physics 2015-05-27 T. Lancaster , J. S. Moeller , S. J. Blundell , F. L. Pratt , P. J. Baker , T. Guidi , G. A. Timco , R. E. P. Winpenny

Finite-temperature spin transport in integrable isotropic spin chains (i.e., spin chains with continuous nonabelian symmetries) is known to be superdiffusive, with anomalous transport properties displaying remarkable robustness to isotropic…

Statistical Mechanics · Physics 2024-12-10 Catherine McCarthy , Sarang Gopalakrishnan , Romain Vasseur

A single nuclear spin holds the promise of being a long-lived quantum bit or quantum memory, with the high fidelities required for fault-tolerant quantum computing. We show here that such promise could be fulfilled by a single phosphorus…

We scrutinize the magnetic properties of $\kappa$-(BEDT-TTF)$_2$Hg(SCN)$_2$Cl through its first-order metal-insulator transition at $T_{\rm CO}=30$ K by means of $^1$H nuclear magnetic resonance (NMR). While in the metal we find…

Strongly Correlated Electrons · Physics 2020-04-08 A. Pustogow , T. Le , H. -H. Wang , Yongkang Luo , E. Gati , H. Schubert , M. Lang , S. E. Brown

It has been shown that inter-spin interaction strengths in a spins-1/2 chain can be evaluated by accessing one of the edge spins only. We demonstrate this experimentally for the simplest case, a three-spin chain, with nuclear magnetic…

Direct evidence of quantum coherence in a single-molecule magnet in frozen solution is reported with coherence times as long as T2 = 630 ns. We can strongly increase the coherence time by modifying the matrix in which the single-molecule…

Materials Science · Physics 2008-10-28 C. Schlegel , J. van Slageren , M. Manoli , E. K. Brechin , M. Dressel

We report on the coherent excitation of the ultranarrow $^{1}\mathrm{S}_0$-$^{3}\mathrm{P}_2$ magnetic quadrupole transition in $^{88}\mathrm{Sr}$. By confining atoms in a state insensitive optical lattice, we achieve excitation fractions…

Coherent interactions at a distance provide a powerful tool for quantum simulation and computation. The most common approach to realize an effective long-distance coupling 'on-chip' is to use a quantum mediator, as has been demonstrated for…

Mesoscale and Nanoscale Physics · Physics 2016-10-11 T. A. Baart , T. Fujita , C. Reichl , W. Wegscheider , L. M. K. Vandersypen

We investigate decoherence due to pure dephasing of a localized spin qubit interacting with a nuclear spin bath. Although in the limit of a very large magnetic field the only decoherence mechanism is spectral diffusion due to dipolar…

Mesoscale and Nanoscale Physics · Physics 2009-06-18 L. Cywinski , W. M. Witzel , S. Das Sarma

Pulsed electron paramagnetic resonance spectroscopy of the photoexcited, metastable triplet state of the oxygen-vacancy center in silicon reveals that the lifetime of the ms = \pm1 sub-levels differ significantly from that of the ms =0…

We show that by averaging over transitions to multiple hyperfine levels, quadrupole shifts and dominant Zeeman effects exactly cancel whenever the nuclear spin, I, is at least as large as the total electronic angular momentum, J. The…

Quantum Physics · Physics 2014-11-04 M. D. Barrett

Frequency references based on solid state spins promise simplicity, compactness, robustness, multifunctionality, ease of integration, and high densities of emitters. Nitrogen-vacancy (NV) centers in diamond are a natural candidate, but the…

We propose a mechanism for very slow coherent oscillations of current and nuclear spins in a quantum dot system, that may qualitatively explain some recent experimental observations. We concentrate on an experimentally relevant double dot…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Sigurdur I. Erlingsson , Oleg N. Jouravlev , Yuli V. Nazarov

Superconducting magnets enable precise control of nuclear and electron spins, and are used in experiments that explore biological and condensed matter systems, and fundamental atomic particles. In high-precision applications, a common view…

Quantum Physics · Physics 2016-07-06 J. W. Britton , B. C. Sawyer , J. G. Bohnet , H. Uys , M. J. Biercuk , J. J. Bollinger

We report a successful measurement of the magnetic field-induced spin singlet-triplet transition in silicon-based coupled dot systems. Our specific experimental scheme incorporates a lateral gate-controlled Coulomb-blockaded structure in Si…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 S. D. Lee , S. J. Kim , J. S. Kang , Y. B. Cho , J. B. Choi , Sooa Park , S. -R. Eric Yang , S. J. Lee , T. H. Zyung

Long coherence times are key to the performance of quantum bits (qubits). Here, we experimentally and theoretically show that the Hahn-echo coherence time (T2) of electron spins associated with divacancy defects in 4H-SiC reaches 1.3 ms,…

Mesoscale and Nanoscale Physics · Physics 2016-10-03 Hosung Seo , Abram L. Falk , Paul V. Klimov , Kevin C. Miao , Giulia Galli , David D. Awschalom

Quantum phase transition in the one-dimensional period-two and uniform quantum compass model are studied by using the pseudo-spin transformation method and the trace map method. The exact solutions are presented, the fidelity, the…

Strongly Correlated Electrons · Physics 2009-11-13 Ke-Wei Sun , Yu-Yu Zhang , Qing-Hu Chen

Electron spins and photons are complementary quantum-mechanical objects that can be used to carry, manipulate and transform quantum information. To combine these resources, it is desirable to achieve the coherent coupling of a single spin…

Mesoscale and Nanoscale Physics · Physics 2015-09-15 J. J. Viennot , M. C. Dartiailh , A. Cottet , T. Kontos

Spin-electronic devices are poised to become part of mainstream microelectronic technology .Downsizing them, however, faces the intrinsic difficulty that as ferromagnets become smaller, it becomes more difficult to stabilize their magnetic…

A heavy hole confined to an InGaAs quantum dot promises the union of a stable spin and optical coherence to form a near perfect, high-bandwidth spin-photon interface. Despite theoretical predictions and encouraging preliminary measurements,…

Quantum Physics · Physics 2018-07-04 L. Huthmacher , R. Stockill , E. Clarke , M. Hugues , C. Le Gall , M. Atatüre