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We measure nuclear and electron spin-polarized H and D densities of at least 10$^{19}\, cm^{-3}$ with $\sim$10 ns lifetimes, from the photodissociation of HBr and DI with circularly-polarized UV light pulses. This density is $\sim$6 orders…

Nuclear spin optical rotation (NSOR) is a recently developed technique for detection of nuclear magnetic resonance via rotation of light polarization, instead of the usual long-range magnetic fields. NSOR signals depend on hyperfine…

Chemical Physics · Physics 2012-02-21 Junhui Shi , Suvi Ikäläinen , Juha Vaara , Michael V. Romalis

The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom.…

Mesoscale and Nanoscale Physics · Physics 2023-09-08 Lukas M. Veldman , Evert W. Stolte , Mark P. Canavan , Rik Broekhoven , Philip Willke , Laëtitia Farinacci , Sander Otte

In this work, we devise a fast and effective nuclear spin hyperpolarization scheme, which is in principle magnetic field and temperature independent. We use this scheme to experimentally demonstrate polarizations of up to 66% for phosphorus…

We briefly discuss the status of double parton scattering (DPS) on both theoretical and experimental sides and summarize the state of the naive DPS model, where the scatterers are taken completely independent. We then elaborate on some of…

High Energy Physics - Phenomenology · Physics 2015-08-12 Tomas Kasemets

Linearly polarized light tuned slightly below the optical transition of the negatively charged exciton (trion) in a single quantum dot causes the spontaneous nuclear spin polarization (self-polarization) at a level close to 100%. The…

Mesoscale and Nanoscale Physics · Physics 2008-04-02 V. L. Korenev

Physical systems reach thermal equilibrium through energy exchange with their environment, and for spins in solids the relevant environment is almost always the host lattice in which they sit. However, recent studies motivated by…

We show that detuned optical pulse trains with a modest spectral width can polarize nuclear spins in InAs quantum dots. The pulse bandwidth is large enough to excite a coherent superposition of both electron spin eigenstates in these…

Quantum Physics · Physics 2015-05-27 S. G. Carter , Sophia E. Economou , A. Shabaev , A. S. Bracker

The distribution is calculated of the electron spin polarization under current-driven spin injection from a probe to a ferromagnetic film. It is shown that the main parameters determining difference of the spin polarization from the…

Materials Science · Physics 2009-12-15 S. G. Chigarev , E. M. Epshtein , Yu. V. Gulyaev , A. I. Panas , V. G. Shofman , P. E. Zilberman

We present an experimental study of the dynamics underlying the buildup and decay of dynamical nuclear spin polarization in a single semiconductor quantum dot. Our experiment shows that the nuclei can be polarized on a time scale of a few…

Optics · Physics 2007-08-02 P. Maletinsky , A. Badolato , A. Imamoglu

Understanding the joint dynamics of electron and nuclear spins is central to core concepts in solid-state magnetic resonance - such as spin-lattice relaxation and dynamic nuclear polarization - but a generalization that capitalizes on…

Quantum Physics · Physics 2021-06-16 Santiago Bussandri , Pablo R. Zangara , Rodolfo H. Acosta , Carlos A. Meriles

The main source of decoherence for an electron spin confined to a quantum dot is the hyperfine interaction with nuclear spins. To analyze this process theoretically we diagonalize the central spin Hamiltonian in the high magnetic B-field…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Oleksandr Tsyplyatyev , Daniel Loss

Electron transport in a new low-dimensional structure - the nuclear spin polarization induced quantum wire (NSPI QW) is theoretically studied. In the proposed system the local nuclear spin polarization creates the effective hyperfine field…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Yu. V. Pershin , S. N. Shevchenko , I. D. Vagner , P. Wyder

Diamond-based quantum sensors have enabled high-resolution NMR spectroscopy at the microscale in scenarios where fast molecular motion averages out dipolar interactions among target nuclei. However, in samples with low-diffusion, ubiquitous…

Quantum Physics · Physics 2025-08-26 Carlos Munuera-Javaloy , Ander Tobalina , Jorge Casanova

Nuclear spins are an important source of dephasing for electron spin qubits in GaAs quantum dots. Most studies of their dynamics have focused on the relatively slow longitudinal polarization. We show, based on a semiclassical model and…

Mesoscale and Nanoscale Physics · Physics 2015-09-30 Christian Dickel , Sandra Foletti , Vladimir Umansky , Hendrik Bluhm

We theoretically investigate dynamic nuclear spin polarization in a self-assembled quantum dot pumped optically by two laser beams. With the assumption that a noncollinear interaction between the hole spin and nuclear spins leads to nuclear…

Mesoscale and Nanoscale Physics · Physics 2013-06-07 Xiao-Feng Shi

Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots lead to nuclear spin polarization that is qualitatively different from the well known optical orientation phenomena. By carrying out a…

Mesoscale and Nanoscale Physics · Physics 2014-10-03 A. Högele , M. Kroner , C. Latta , M. Claassen , I. Carusotto , C. Bulutay , A. Imamoglu

We use field-cycling-assisted dynamic nuclear polarization and continuous radio-frequency (RF) driving over a broad spectral range to demonstrate magnetic-field-dependent activation of nuclear spin transport from strongly-hyperfine-coupled…

Taking inspiration from NMR spectroscopy, periodic irradiation schemes have recently shown remarkable performance when implemented into pulsed dynamic nuclear polarization (DNP) sequences. This has prompted considerable interest in…

A broad effort is underway to improve the sensitivity of nuclear magnetic resonance through the use of dynamic nuclear polarization. Nitrogen-vacancy (NV) centers in diamond offer an appealing platform because these paramagnetic defects can…