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Single crystals of the Kitaev spin-liquid candidate $\alpha$-RuCl$_3$ have been studied to determine low-temperature bulk properties, structure and the magnetic ground state. Refinements of x-ray diffraction data show that the low…

Strongly Correlated Electrons · Physics 2016-04-27 H. B. Cao , A. Banerjee , J. -Q. Yan , C. A. Bridges , M. D. Lumsden , D. G. Mandrus , D. A. Tennant , B. C. Chakoumakos , S. E. Nagler

We report X-ray diffraction and magnetic susceptibility studies of the structural phase transition in $\alpha$-RuCl$_{3}$. By utilizing a single crystal sample with predominantly single twin domain, we show that $\alpha$-RuCl$_{3}$ goes…

Strongly Correlated Electrons · Physics 2023-11-08 Subin Kim , Ezekiel Horsley , Jacob P. C. Ruff , Beatriz D. Moreno , Young-June Kim

$\alpha$-RuCl$_3$, a well-known candidate material for Kitaev quantum spin liquid, is prone to stacking disorder due to the weak van der Waals bonding between the honeycomb layers. After a decade of intensive experimental and theoretical…

$\alpha$-RuCl$_3$ is considered to be the top candidate material for the experimental realization of the celebrated Kitaev model. It is however known that additional interactions beyond the Kitaev model trigger in $\alpha$-RuCl$_3$, a…

$\alpha$-RuCl$_3$ is a candidate Kitaev material that exhibits zigzag antiferromagnetic ordering below 7 K. One contentious issue regarding this material is its bulk structure in the low-temperature phase. Recently, it has become generally…

Materials Science · Physics 2026-01-27 Seung-Ju Hong , Tae Yun Kim , Cheol-Hwan Park

We discuss the implications that new magnetocaloric, thermal expansion and magnetostriction data in $\alpha$-RuCl$_{3}$ single crystals have on its temperature-field phase diagram and uncover the magnetic-field dependence of an apparent…

Recent studies have brought $\alpha$-RuCl$_3$ to the forefront of experimental searches for materials realizing Kitaev spin-liquid physics. This material exhibits strongly anisotropic exchange interactions afforded by the spin-orbit…

Strongly Correlated Electrons · Physics 2018-02-21 Stephen M. Winter , Kira Riedl , David Kaib , Radu Coldea , Roser Valenti

We report a comprehensive single-crystal neutron diffraction investigation of the Kitaev quantum magnet $\alpha$-RuCl$_{3}$ under hydrostatic pressure. Utilizing a He-gas pressure cell, we successfully applied an ideal hydrostatic pressure…

Strongly Correlated Electrons · Physics 2023-04-04 Xiao Wang , Fengfeng Zhu , Navid Qureshi , Ketty Beauvois , Junda Song , Thomas Mueller , Thomas Brückel , Yixi Su

We present initial Raman spectroscopy experiments on exfoliated flakes of $\alpha$-RuCl$_3$, from tens of nm thick down to single layers. Besides unexpectedly finding this material to be air stable, in the thinnest layers we observe the…

Strongly Correlated Electrons · Physics 2019-12-11 Boyi Zhou , Yiping Wang , Gavin B. Osterhoudt , Paige Kelly , David Mandrus , Rui He , Kenneth S. Burch , Erik A. Henriksen

Two-dimensional (2D) materials with intrinsic ferromagnetism provide unique opportunity to engineer new functionalities in nano-spintronics. One such material is CrI$_3$, showing long-range magnetic order in monolayer with the Curie…

Strongly Correlated Electrons · Physics 2019-09-20 Yu Liu , Lijun Wu , Xiao Tong , Jun Li , Jing Tao , Yimei Zhu , C. Petrovic

We present high-resolution thermal-expansion and specific-heat measurements of single crystalline alpha-RuCl3. An extremely hysteretic structural transition expanding over 100 K is observed by thermal- expansion along both crystallographic…

Strongly Correlated Electrons · Physics 2018-09-26 Mingquan He , Xiao Wang , Liran Wang , Frédéric Hardy , Thomas Wolf , Peter Adelmann , Thomas Brückel , Yixi Su , Christoph Meingast

We report X-ray diffraction and resonant elastic X-ray scattering (REXS) studies on two $\alpha$-RuCl$_{3}$ crystals with distinct magnetic transition temperatures: T$_{N}$=7.3K and 6.5K. We find that the sample with T$_{N}$=6.5K exhibits a…

Strongly Correlated Electrons · Physics 2024-03-08 Subin Kim , Ezekiel Horsley , Christie Nelson , Jacob Ruff , Young-June Kim

The layered honeycomb magnet $\alpha$-RuCl$_3$ is the most promising candidate for a Kitaev quantum spin liquid (KQSL) that can host charge-neutral Majorana fermions. Recent studies have shown significant sample dependence of thermal…

Recent experiments revealed that monolayer $\alpha$-RuCl$_3$ can be obtain by chemical exfoliation method and exfoliation or restacking of nanosheets can manipulate the magnetic properties of the materials. In this present paper, the…

Recently, there have been increasingly hot debates on whether there exists a quantum spin liquid in the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ in high magnetic field. To investigate this issue, we perform the ultralow-temperature thermal…

Strongly Correlated Electrons · Physics 2018-02-14 Y. J. Yu , Y. Xu , K. J. Ran , J. M. Ni , Y. Y. Huang , J. H. Wang , J. S. Wen , S. Y. Li

The layered honeycomb magnet $\alpha$-RuCl$_3$ has attracted intense scrutiny as a prime candidate for realizing the Kitaev quantum spin liquid, yet a consensus on its microscopic Hamiltonian remains elusive due to the material's extreme…

Kitaev quantum spin liquids have attracted significant attention in condensed matter physics over the past decade. To understand their emergent quantum phenomena, high-quality single crystals of substantial size are essential. Here, we…

Strongly Correlated Electrons · Physics 2025-02-18 Bowen Zhang , Xiangjun Li , Limin Yan , Wenbo Li , Nana Li , Jianfa Zhao , Xiaobing Liu , Shun-Li Yu , Zhiwei Hu , Wenge Yang , Runze Yu

The spin-orbit assisted Mott insulator $\alpha$-RuCl3 is proximate to the coveted quantum spin liquid (QSL) predicted by the Kitaev model. In the search for the pure Kitaev QSL, reducing the dimensionality of this frustrated magnet by…

We investigated the thermal transport properties of two $\alpha$-RuCl$_3$ crystals with different degrees of stacking disorder to understand the origin of the previously reported oscillatory feature in the field dependence of thermal…

Materials Science · Physics 2024-01-17 Heda Zhang , Andrew May , Hu Miao , Brian Sales , David Mandrus , Stephen Nagler , Michael McGuire , Jiaqiang Yan

Measurements of the magnetic Gr\"uneisen parameter ($\Gamma_B$) and specific heat on the Kitaev material candidate $\alpha$-RuCl$_3$ are used to access in-plane field- and temperature-dependence of the entropy up to 12 T and down to 1 K. No…

Strongly Correlated Electrons · Physics 2020-08-28 S. Bachus , D. A. S. Kaib , Y. Tokiwa , A. Jesche , V. Tsurkan , A. Loidl , S. M. Winter , A. A. Tsirlin , R. Valenti , P. Gegenwart
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