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(TaSe4)2I, a quasi-one-dimensional (1D) crystal, shows a characteristic temperature-driven metal-insulator phase transition. Above the charge density wave (CDW) temperature Tc, (TaSe4)2I has been predicted to harbor a Weyl semimetal phase.…

Using {\it ab initio} density functional theory, we study the lattice phase transition of quasi-one-dimensional (TaSe$_4$)$_2$I. In the undistorted state, the strongly anisotropic semimetal band structure presents two non-equivalent Weyl…

Materials Science · Physics 2020-05-14 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Shuai Dong , Elbio Dagotto

The electronic-structural modulations of Ir$_{1-x}$Pt$_x$Te$_2$ (0 $\leqq x\leqq$ 0.12) have been examined by resonant elastic x-ray scattering (REXS) and resonant inelastic x-ray scattering (RIXS) techniques at both the Ir and Te edges.…

Strongly Correlated Electrons · Physics 2018-07-04 K. Takubo , K. Yamamoto , Y. Hirata , H. Wadati , T. Mizokawa , R. Sutarto , F. He , K. Ishii , Y. Yamasaki , H. Nakao , Y. Murakami , G. Matsuo , H. Ishii , M. Kobayashi , K. Kudo , M. Nohara

The transition-metal dichalcogenide tantalum disulphide (1$T$-TaS$_2$) hosts a commensurate charge density wave (CCDW) at temperatures below 165~K where it also becomes insulating. The low temperature CCDW phase can be driven into a…

We investigate electronic instabilities in 2H-TaS\textsubscript{2} and a self-intercalated variant, 2H$^\dagger$-Ta\textsubscript{1+$\delta$}S\textsubscript{2}. In conventional samples, which we determine to be slightly hole-doped, spectral…

We report temperature-dependent transport and x-ray diffraction measurements of the influence of Ti hole doping on the charge density wave (CDW) in 1T-Ta(1-x)Ti(x)S(2). Confirming past studies, we find that even trace impurities eliminate…

The dynamics of the photoinduced commensurate to incommensurate charge density wave (CDW) phase transition in 4Hb-TaSe2 are investigated by femtosecond electron diffraction. In the perturbative regime the CDW reforms on a 150 ps timescale,…

Strongly Correlated Electrons · Physics 2015-06-11 N. Erasmus , M. Eichberger , K. Haupt , I. Boshoff , G. Kassier , R. Birmurske , H. Berger , J. Demsar , H. Schwoerer

The transition metal dichalcogenides 1T-TaS$_2$ and 1T-TaSe$_2$ have been extensively studied for the complicated correlated electronic properties. The origin of different surface electronic states remains controversial. We apply scanning…

Strongly Correlated Electrons · Physics 2022-01-11 Wenhao Zhang , Zongxiu Wu , Kunliang Bu , Ying Fei , Yuan Zheng , Jingjing Gao , Xuan Luo , Zheng Liu , Yu-ping Sun , Yi Yin

We investigate the structural and electronic reconstruction associated with the commensurate charge-density-wave (CCDW) phase in bulk and monolayer 1T-TaS2 using density functional theory (DFT) and Wannier-based tight-binding modeling.…

Mesoscale and Nanoscale Physics · Physics 2026-04-17 S. K. Behera , A. Swain , P. C. Ramamurthy

A variety of experiments have been carried out to establish the origin of the chiral charge-density wave transition in 1T-TiSe$_2$, which in turn has led to contradictory conclusions on the origin of this transition. Some studies suggest…

Materials Science · Physics 2020-10-05 Darshana Wickramaratne , Richard Schaller , Gary Wiederrecht , Goran Karapetrov , I. I. Mazin

Coexistence of localized and extended excitations is central to the macroscopic properties of correlated materials. For 5d transition metal compounds, electron correlations alone generally do not lead to a metal-insulator (Mott) transition,…

Transition metal dichalcogenides have recently emerged as promising two-dimensional materials with intriguing electronic properties. Existing calculations of intrinsic phonon-limited electronic transport so far have concentrated on the…

Materials Science · Physics 2017-10-05 Nicki Frank Hinsche , Kristian Sommer Thygesen

We study the coupled charge-lattice dynamics in the commensurate charge density wave (CDW) phase of the layered compound 1T-TaS$_{2}$ driven by an ultrashort laser pulse. For describing its electronic structure, we employ a tight-binding…

Strongly Correlated Electrons · Physics 2018-12-27 Tatsuhiko N. Ikeda , Hirokazu Tsunetsugu , Kenji Yonemitsu

1$T$-TaSe$_2$ is widely believed to host a Mott metal-insulator transition in the charge density wave (CDW) phase according to the spectroscopic observation of a band gap that extends across all momentum space. Previous investigations…

Strongly Correlated Electrons · Physics 2023-04-17 C. J. Sayers , G. Cerullo , Y. Zhang , C. E. Sanders , R. T. Chapman , A. S. Wyatt , G. Chatterjee , E. Springate , D. Wolverson , E. Da Como , E. Carpene

We present a state-of-the-art x-ray diffraction study of the charge density wave order in 1T-TaS2 as a function of temperature and pressure. Our results prove that the charge density wave, which we characterize in terms of wave vector,…

Strongly Correlated Electrons · Physics 2013-03-27 T. Ritschel , J. Trinckauf , G. Garbarino , M. Hanfland , M. v. Zimmermann , H. Berger , B. Buechner , J. Geck

Suppressing of an ordered state that competes with superconductivity is one route to enhance superconducting transition temperatures. Whereas the effect of suppressing magnetic states is still not fully understood, materials featuring…

Low-dimensional electron systems, as realized naturally in graphene or created artificially at the interfaces of heterostructures, exhibit a variety of fascinating quantum phenomena with great prospects for future applications. Once…

Strongly Correlated Electrons · Physics 2016-08-03 T. Ritschel , J. Trinckauf , K. Koepernik , B. Büchner , M. v. Zimmermann , H. Berger , Y. I. Joe , P. Abbamonte , J. Geck

Most metallic transition metal dichalcogenides undergo charge density wave (CDW) instabilities with similar or identical ordering vectors in bulk and in single layer, albeit with different critical temperatures. Metallic 1T-TiTe$_2$ is a…

In the quasi-2D electron systems of the layered transition metal dichalcogenides (TMD) there is still a controversy about the nature of the transitions to charge-density wave (CDW) phases, i.e. whether they are described by a Peierls-type…

Strongly Correlated Electrons · Physics 2014-05-02 Jixia Dai , Eduardo Calleja , Jacob Alldredge , Xiangde Zhu , Lijun Li , Wenjian Lu , Yuping Sun , Thomas Wolf , Helmuth Berger , Kyle McElroy

Recently, intercalation emerges as an effective way to manipulate ground-state properties and enrich quantum phase diagrams of layered transition metal dichalcogenides (TMDCs). In this work, we focus on fully Ta-intercalated bilayer…

Materials Science · Physics 2023-04-07 Tiantian Luo , Maoping Zhang , Jifu Shi , Feipeng Zheng