Related papers: Controlling Nonadiabatic Transitions Through Engin…
The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…
We investigate a simple and robust scheme for choosing the phases of adiabatic electronic states smoothly (as a function of geometry) so as to maximize the performance of ab initio non-adiabatic dynamics methods. Our approach is based upon…
Quantum coherent control of ultrafast bond making and the subsequent molecular dynamics is crucial for the realization of a new photochemistry, where a shaped laser field is actively driving the chemical system in a coherent way from the…
Reaching a given target quantum state with high fidelity and fast operation speed close to the quantum limit represents an important goal in quantum information science. Here, we experimentally demonstrate superadiabatic quantum driving to…
In this manuscript we report on adiabatic pumping in quasiperiodic stiffness modulated beams. We show that distinct topological states populating nontrivial gaps can nucleate avoided crossings characterized by edge-to-edge transitions. Such…
We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort…
Nonadiabatic dynamics around an avoid crossing or a conical intersection play a crucial role in the photoinduced processes of most polyatomic molecules. The present work shows that the topological phase in conical intersection makes the…
Adiabatic pulses are used extensively to enable robust control of quantum operations. We introduce a new approach to adiabatic control that uses the superadiabatic quality or $Q$-factor as a performance metric to design robust, high…
We study finite-time Landau-Zener transitions at a singlet-triplet level crossing in a GaAs double quantum dot, both experimentally and theoretically. Sweeps across the anticrossing in the high driving speed limit result in oscillations…
We work out the theory and applications of a fast quasi-adiabatic approach to speed up slow adiabatic manipulations of quantum systems by driving a control parameter as near to the adiabatic limit as possible over the entire protocol…
Motivated by the intriguing possibilities of steering ultrafast non-adiabatic processes through the geometric properties of bands in quantum materials by laser pulses, we extend a wave-packet transport theory, previously well-established in…
We present a digitized implementation of rapid adiabatic passage based on a train of weak, frequency-varying ultrafast pulses. Analytic conditions on the subpulse Rabi frequencies and detunings are derived to reproduce the continuous-time…
In this paper we evaluate the performance of two superadiabatic stimulated Raman adiabatic passage (STIRAP) protocols derived from Gaussian and sin-cos pulses, under dissipation and Ornstein-Uhlenbeck noise in the energy levels. We find…
The techniques of shortcuts to adiabaticity have been proposed to accelerate the "slow" adiabatic processes in various quantum systems with the applications in quantum information processing. In this paper, we study the counter-diabatic…
Stimulated Raman Adiabatic Passage (STIRAP) is a widely used method for adiabatic population transfer in a multilevel system. In this work, we study STIRAP under novel conditions and focus on the fractional, F-STIRAP, which is known to…
The controlled transfer of nuclear state population using two x-ray laser pulses is investigated theoretically. The laser pulses drive two nuclear transitions in a nuclear three-level system facilitating coherent population transfer via the…
We present a new class of control pulses designed to transfer co-located ensembles without relying on frequency selectivity, thereby allowing much faster state-transitions. A geometric approach allows us to construct sequences which are…
The pace and unpredictability of evolution are critically relevant in a variety of modern challenges: combating drug resistance in pathogens and cancer, understanding how species respond to environmental perturbations like climate change,…
We study spin-phonon coupled dynamics in the vicinity of a sloped conical intersection created by laser coupling the electronic (spin) and vibrational degrees of freedom of a pair of trapped Rydberg ions. We show that the shape of the…
We consider an adiabatic population transfer process that resembles the well established stimulated Raman adiabatic passage (STIRAP). In our system, the states have nonzero angular momentums $J$, therefore, the coupling laser fields induce…