Related papers: Controlling Nonadiabatic Transitions Through Engin…
Implementation of quantum logical gates for multilevel system is demonstrated through decoherence control under the quantum adiabatic method using simple phase modulated laser pulses. We make use of selective population inversion and…
We investigate geometric phase (GP) effects in nonadiabatic transitions through a conical intersection (CI) in an N-dimensional linear vibronic coupling (ND-LVC) model. This model allows for the coordinate transformation encompassing all…
We report an ultrafast and efficient way to create the maximum coherence between the two lower states in a -like atomic systems, driven by two nonlinearly chirped few-cycle pulses. The phenomenon of coherent population trapping and…
Conical intersections are crossing points or lines between two or more adiabatic electronic potential energy surfaces in the multi-dimensional coordinate space of colliding atoms and molecules. Conical intersections and corresponding…
We present a novel scheme for coherent manipulation of populations and robust creation of arbitrary coherent superposition of metastable states of a quantum system with lambda configuration of operating energy levels using laser pulses with…
Nonadiabaticity, i.e., the effect of mixing electronic states by nuclear motion, is a central phenomenon in molecular science. The strongest nonadiabatic effects arise due to the presence of conical intersections of electronic energy…
Conical intersections (CIs) are seen as the main mediators of nonadiabatic transitions; yet, mixed quantum-classical (MQC) simulations rarely, if ever, sample geometries with exactly degenerate electronic energies. Here we show that this…
Controlling the phase space of particle beams is essential for the generation of high-quality, ultrashort electron beams in plasma-based accelerators. Accurately diagnosing the transient energy chirp, which evolves rapidly at the onset of…
This work theoretically investigates possibilities of using the Stimulated Raman Adiabatic Passage (STIRAP) and its variants to control a coherent superposition of quantum states. We present a generalization of the so-called fractional…
A novel chirped pulse control scheme is presented based on Coherent Anti-Stokes Raman Spectroscopy (C-CARS) aiming at maximizing the vibrational coherence in atoms and molecules. The scheme utilizes chirping of the three incoming pulses,…
We report and propose a simple scheme to achieve efficient and fast coherent population transfer (CPT) by utilizing either a nonlinearly chirped Gaussian shaped few-cycle laser pulse or an unchirped sinc-shaped few-cycle laser pulse. The…
Resonant transverse driving of a two-level system as viewed in the rotating frame couples two degenerate states at the Rabi frequency, an amazing equivalence that emerges in quantum mechanics. While spectacularly successful at controlling…
The rates and outcomes of virtually all photophysical and photochemical processes are determined by Conical Intersections. These are regions of degeneracy between electronic states on the nuclear landscape of molecules where electrons and…
Exciton pulses transport excitation and entanglement adiabatically through Rydberg aggregates, assemblies of highly excited light atoms, which are set into directed motion by resonant dipole-dipole interaction. Here, we demonstrate the…
Scaling of quantum gates remains a central challenge in quantum information science. Ultrafast gates based on spin-dependent kicks provide a promising approach for trapped-ion systems. However, these gates require laser pulses with both…
Transitions in an artificial atom, driven non-adiabatically through an energy-level avoided crossing, can be controlled by carefully engineering the driving protocol. We have driven a superconducting persistent-current qubit with a…
We apply the inversely-engineered control method based on Lewis-Riesenfeld invariants to control mixed states of a two-level quantum system. We show that the inversely-engineered control passages of mixed states - and pure states as special…
The first step in the coherent control of a photoinduced binary reaction is bond making or photoassociation. We have recently demonstrated coherent control of bond making in multi-photon femtosecond photoassociation of hot magnesium atoms,…
Conical intersections are ubiquitous in polyatomic molecules and responsible for a wide range of phenomena in chemistry and physics. We introduce and implement a local diabatic representation for the correlated electron-nuclear dynamics…
We have proposed and demonstrated a fast and robust method of population transfer between two quantum states using a quadratically chirped laser source. Incorporating the Jaynes-Cummings in a full quantum description of the interaction, and…