Related papers: Revealing Electron-Ytterbium Interactions through …
Controlling molecular binding at the level of single atoms is one of the holy grails of quantum chemistry. Rydberg macrodimers -- bound states between highly excited Rydberg atoms -- provide a novel perspective in this direction. Resulting…
Divalent atoms provide excellent means for advancing control in Rydberg atom-based quantum simulation and computing, due to the second optically active valence electron available. Particularly promising in this context are circular Rydberg…
We present a new mechanism contributing to the detection of photoassociated long-range Rydberg molecules via pulsed-field ionization: ionic products, created by the decay of a long-range Rydberg molecule, modify the excitation spectrum of…
A remarkable property of Rydberg atoms is the possibility to create molecules formed by one highly excited atom and another atom in the ground state. The first realisation of such a Rydberg molecule has opened an active field of physical…
We present a comprehensive theoretical study of the electronic structures of the Yb atom and the Yb$_2$ molecule, respectively, focusing on their ground and lowest-lying electronically excited states. Our study includes various…
We report on the observation of highly excited ($\nu \sim 100)$ vibrational states of a trilobite ultralong-range Rydberg molecule in $^{87}$Rb. These states manifest spectroscopically in a regularly spaced series of peaks red-detuned from…
Rydberg excitons, the solid-state counterparts of Rydberg atoms, have sparked considerable interest in harnessing their quantum application potentials, whereas a major challenge is realizing their spatial confinement and manipulation.…
Rydberg atoms are currently a very fast advancing quantum platform. For many interesting and demanding applications, including quantum computation, fast detection of a Rydberg excitation or a Rydberg qubit for information readout would be…
Stability achieved by large angular momentum is ubiquitous in nature, with examples ranging from classical mechanics, over optics and chemistry, to nuclear physics. In atoms, angular momentum can protect excited electronic orbitals from…
We review Rydberg aggregates, assemblies of a few Rydberg atoms exhibiting energy transport through collective eigenstates, considering isolated atoms or assemblies embedded within clouds of cold ground-state atoms. We classify Rydberg…
A non-resonant microwave dressing field at 38.465 GHz was used to eliminate the static electric dipole moment difference between the $49s_{1/2}$ and $48s_{1/2}$ Rydberg states of $^{87}$Rb in dc fields of approximately 1 V/cm. The reduced…
We present high-resolution spectroscopy of Rb$_\text{2}$ ultralong-range Rydberg molecules bound by mixed singlet-triplet electron-neutral atom scattering. The mixing of the scattering channels is a consequence of the hyperfine interaction…
Molecular bonds can be divided into four primary types: ionic, covalent, van der Waals and hydrogen bonds. At ultralow temperatures a novel binding type emerges paving the way for novel molecules and ultracold chemistry [1,2]. The…
Rydberg atom-based radio frequency electromagnetic field sensors are drawing wide-spread interest because of their unique properties, such as small size, dielectric construction, and self-calibration. These photonic sensors use lasers to…
We report on the observation of two vibrational series of pure trilobite rubidium Rydberg molecules. They are created via three-photon photoassociation and lie energetically more than 15 GHz below the atomic 22$F$ state of rubidium. In…
We present a study of the Rydberg spectrum in \ts{166}Er for series connected to the $4f^{12} (^3H_6) 6s$, $J_c=13/2 $ and $J_c=11/2 $ ionic core states using an all-optical detection based on electromagnetically induced transparency in an…
Exceptional points are special parameter points in spectra of open quantum systems, at which resonance energies degenerate and the associated eigenvectors coalesce. Typical examples are Rydberg systems in parallel electric and magnetic…
The interaction between atoms and a quantized radiation field is fundamentally important in quantum optics and quantum information science. Due to their unusual properties, Rydberg atoms are promising building blocks for two-qubit gates and…
Neutral atom qubits with Rydberg-mediated interactions are a leading platform for developing large-scale coherent quantum systems. In the majority of experiments to date, the Rydberg states are not trapped by the same potential that…
Trilobite molecules are ultralong-range Rydberg molecules formed when a high angular momentum Rydberg electron scatters off of a ground-state atom. Their unique electronic structure and highly oscillatory potential energy curves support a…