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Solute-surface interactions have garnered considerable interest in recent years as a novel control mechanism for driving unique fluid dynamics and particle transport with potential applications in fields such as biomedicine, the development…

Fluid Dynamics · Physics 2023-05-05 Jian Teng , Bhargav Rallabandi , Jesse T. Ault

In this article, we study numerically the dispersion of colloids in a two-dimensional cellular flow in the presence of an imposed mean salt gradient. Owing to the additional scalar, the colloids do not follow exactly the Eulerian flow…

Fluid Dynamics · Physics 2022-09-23 Romain Volk , Michaël Bourgoin , Charles-Édouard Bréhier , Florence Raynal

In this letter, we characterize experimentally the diffusiophoretic motion of colloids and lambda- DNA toward higher concentration of solutes, using microfluidic technology to build spatially- and temporally-controlled concentration…

Soft Condensed Matter · Physics 2010-04-09 J. Palacci , B. Abecassis , C. Cottin-Bizonne , C. Ybert , L. Bocquet

The cellular environment, characterized by its intricate composition and spatial organization, hosts a variety of organelles, ranging from membrane-bound ones to membraneless structures that are formed through liquid-liquid phase…

Soft Condensed Matter · Physics 2026-03-09 Gregor Häfner , Marcus Müller

In this work, we numerically investigate the impact of two-dimensional solute gradients on the distribution of colloidal particles, i.e., colloidal banding, induced via diffusiophoresis. The solute gradients are generated by spatially…

Soft Condensed Matter · Physics 2023-01-11 Ritu R. Raj , C. Wyatt Shields , Ankur Gupta

The separation of colloidal particles based solely on their surface properties is a highly challenging task. This study demonstrates that diffusiophoresis and diffusioosmosis enable the continuous separation of carboxylate polystyrene…

Active diffusiophoresis - swimming through interaction with a self-generated, neutral, solute gradient - is a paradigm for autonomous motion at the micrometer scale. We study this propulsion mechanism within a linear response theory.…

Statistical Mechanics · Physics 2015-05-30 Benedikt Sabass , Udo Seifert

We study analytically the joint dispersion of Gaussian patches of salt and colloids in linear flows, and how salt gradients accelerate or delay colloid spreading by diffusiophoretic effects. Because these flows have constant gradients in…

Concentration gradients play a critical role in embryogenesis, bacterial locomotion, as well as the motility of active particles. Particles develop concentration profiles around them by dissolution, adsorption, or the reactivity of surface…

Under a thermodynamic gradient, for example, the concentration or temperature gradients, the colloidal particles immersed in the solvent can exhibit a directional migration along or against the gradient -- phoresis, a cross transport…

Soft Condensed Matter · Physics 2026-03-31 Yuxing Jiao , Qing Yang , Mingcheng Yang

We investigate the diffusiophoresis of a non-polarizable droplet laden with soluble ionic surfactant, for which the surface charge arises from adsorption of surfactant at the fluid-fluid interface. Unlike previous studies that assume either…

Fluid Dynamics · Physics 2026-02-09 Subrata Majhi , Somnath Bhattacharyya

Dissipative particle dynamics (DPD) belongs to a class of models and computational algorithms developed to address mesoscale problems in complex fluids and soft matter in general. It is based on the notion of particles that represent…

Statistical Mechanics · Physics 2017-05-24 Pep Español , Patrick B Warren

In both biological and artificial systems, concentration gradients can serve as a convenient mechanism for manipulating particles and generating motility. Particles that interact with a solute will move along its gradient; if they…

Soft Condensed Matter · Physics 2011-07-21 Gareth P. Alexander , Andrea J. Liu

Gradient-driven diffusion in crowded, multicomponent mixtures is a topic of high interest because of its role in biological processes such as transport in cell membranes. In partially phase-separated solutions, gradient-driven diffusion…

Soft Condensed Matter · Physics 2017-02-15 Prithviraj Nandigrami , Brandy Grove , Andrew Konya , Robin L. B. Selinger

Molecular dynamics simulation is a prominent way of analyzing the dynamic properties of a system. The molecular dynamics simulation of diffusion, an important transport property, of dilute solution of cysteine in SPCE water at five…

Chemical Physics · Physics 2018-09-25 Hem Prasad Bhusal , Narayan Prasad Adhikari

Using Stokesian dynamics simulations, we examine the flow of a monodisperse, neutrally buoyant, homogeneous suspension of non-Brownian solid spheres in simple shear, starting from a large number of independent hard-sphere distributions and…

Materials Science · Physics 2019-06-19 M. Marchioro , A. Acrivos

A migration of charged particles relative to a solvent, caused by a gradient of salt concentration and termed a diffusiophoresis, is of much interest being exploited in many fields. Existing theories deal with diffusiophoresis of passive…

Soft Condensed Matter · Physics 2024-10-15 Evgeny S. Asmolov , Olga I. Vinogradova

The controlled transport of colloids in dead-end structures is a key capability that can enable a wide range of applications, such as bio-chemical analysis, drug delivery and underground oil recovery. This letter presents a new trapping…

We reveal an unreported physical mechanism that enables the pre-concentration, sorting and characterization of charged polystyrene nanobeads and liposomes dispersed in a continuous flow within a straight micron-sized channel. Initially, a…

In a binary fluid mixture, the concentration gradient of a heavier molecular solute leads to a diffusive flux of solvent and solute to achieve thermodynamic equilibrium. If the solute concentration decreases with height, the system is…