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Dual-comb microscopy (DCM), based on a combination of dual-comb spectroscopy (DCS) with two-dimensional spectral encoding (2D-SE), is a promising method for scan-less confocal laser microscopy giving an amplitude and phase image contrast…

Terahertz two-dimensional coherent spectroscopy (THz-2DCS) is transforming our ability to probe, visualize, and control quantum materials far from equilibrium. This emerging technique brings multi-dimensional resolution to the ultrafast…

Superconductivity · Physics 2026-02-09 Chuankun Huang , Martin Mootz , Liang Luo , Ilias E. Perakis , Jigang Wang

For the first time to our knowledge, a dual-comb laser based on thin-disk technology and its application to direct frequency comb spectroscopy are presented. The peak power (0.6 MW) and the average power (12 W) of our Yb:YAG thin-disk…

Laser based ranging (LiDAR) - already ubiquitously used in industrial monitoring, atmospheric dynamics, or geodesy - is key sensor technology. Coherent laser ranging, in contrast to time-of-flight approaches, is immune to ambient light,…

We introduce a novel laser-scanning optical microscopy technique that employs optical-frequency-comb (OFC) lasers. This method facilitates multimodal spectroscopic imaging by analyzing interferograms produced via a dual-comb spectroscopic…

We introduce a new parallelized approach to photothermal microscopy that utilizes mid-infrared dual-comb lasers, enabling simultaneous measurements at hundreds of wavelengths. This technology allows for high-speed, label-free chemical…

Two-photon resonance transition technology has been proven to have a wide range of applications,it's limited by the available wavelength of commercial lasers.The application of optical comb technology with direct two-photon transition…

Atomic Physics · Physics 2022-04-27 Lin Dan , Hao Xu , Ping Guo , Jianye Zhao

Dual THz comb spectroscopy has the potential to be used as universal THz spectroscopy with high spectral resolution, high spectral accuracy, and broad spectral coverage; however, the requirement for dual stabilized femtosecond lasers…

Instrumentation and Detectors · Physics 2019-08-06 Guoqing Hu , Tatsuya Mizuguchi , Ryo Oe , Kazuki Nitta , Xin Zhao , Takeo Minamikawa , Ting Li , Zheng Zheng , Takeshi Yasui

Hyperspectral imaging is a technique that allows for the creation of multi-color images. At terahertz wavelengths, it has emerged as a prominent tool for a number of applications, ranging from non-ionizing cancer diagnosis and…

A fluorescence correlation spectroscopy (FCS) system based on two independent measurement volumes is presented. The optical setup and data acquisition hardware are detailed, as well as a complete protocol to control the location, size and…

Optics · Physics 2009-08-26 P. Ferrand , M. Pianta , A. Kress , A. Aillaud , H. Rigneault , D. Marguet

We present a detection scheme for diffusing wave spectroscopy (DWS) based on a two cell geometry that allows efficient ensemble averaging. This is achieved by putting a fast rotating diffuser in the optical path between laser and sample. We…

Soft Condensed Matter · Physics 2009-11-11 P. Zakharov , F. Cardinaux , F. Scheffold

Multidimensional coherent spectroscopy (MDCS) has been established in quantum chemistry as a powerful tool for studying the nonlinear response and nonequilibrium dynamics of molecular systems. More recently, the technique has also been…

Strongly Correlated Electrons · Physics 2025-05-12 Jiyu Chen , Philipp Werner

Four-wave-mixing-based quantum cascade laser frequency combs (QCL-FC) are a powerful photonic tool, driving a recent revolution in major molecular fingerprint regions, i.e. mid- and far-infrared domains. Their compact and frequency-agile…

Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…

Atomic Physics · Physics 2018-06-13 Bachana Lomsadze , Steven T. Cundiff

The phase information provided by the beat note between frequency combs and two continuous-wave lasers is used to extrapolate the phase evolution of comb modes found in a spectral region obtained via nonlinear broadening. This thereafter…

We present a complex-valued electric field model for experimentally observed cavity transmission in coherent cavity-enhanced (CE) multiplexed spectroscopy (i.e., dual-comb spectroscopy, DCS). The transmission model for CE-DCS differs from…

Instrumentation and Detectors · Physics 2018-08-03 Adam J. Fleisher , David A. Long , Joseph T. Hodges

Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the…

Deep learning methods are developing rapidly in coded aperture snapshot spectral imaging (CASSI). The number of parameters and FLOPs of existing state-of-the-art methods (SOTA) continues to increase, but the reconstruction accuracy improves…

Image and Video Processing · Electrical Eng. & Systems 2023-08-04 Zeyu Cai , Chengqian Jin , Feipeng Da

We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…