Related papers: Quantum-optimal nonlinear microscopy with classica…
Spectroscopic stimulated Raman scattering (SRS) imaging has become a useful tool finding a broad range of applications. Yet, wider adoption is hindered by the bulky and environmentally-sensitive solid-state optical parametric oscillator…
Properties of quantum states have disclosed new technologies, ranging from quantum information to quantum metrology. Among them a recent research field is quantum imaging, addressed to overcome limits of classical imaging by exploiting…
This work presents a quantum-limited optomechanical sensing platform for real-time detection and discrimination of chiral molecules, based on a multilayer hybrid plasmonic-mechanical resonator. Leveraging quantum zero-point motion and…
Spectroscopy is a crucial laboratory technique for understanding quantum systems through their interactions with electromagnetic radiation. Particularly, spectroscopy is capable of revealing the physical structure of molecules, leading to…
Quantum metrology experiments in atomic physics and quantum optics have demonstrated measurement accuracy beyond the shot-noise limit via multi-particle entanglement. At the same time, electron microscopy, an essential tool for…
Nonlinear interactions between single quantum particles are at the heart of any quantum information system, including analog quantum simulation and fault-tolerant quantum computing. This remains a particularly difficult problem for photonic…
In the quantum process of stimulated Raman scattering (SRS), a laser photon propagating in a resonance medium undergoes multifold conversions into a Stokes photon and back. The nontrivial ``cooperative'' behavior of the Stokes component of…
The low efficiency of Raman spectroscopy can be overcome by placing the active molecules in the vicinity of scatterers, typically rough surfaces or nanostructures with various shapes. This surface-enhanced Raman scattering (SERS) leads to…
The interaction between ultrashort light pulses and non-absorbing materials is dominated by Impulsive Stimulated Raman Scattering (ISRS). The description of ISRS in the context of pump\&probe experiments is based on effective classical…
Far-field optical microscopy using focused light is an important tool in a number of scientific disciplines including chemical, (bio)physical and biomedical research, particularly with respect to the study of living cells and organisms.…
Label-free vibrational imaging by stimulated Raman scattering (SRS) provides unprecedented insight into real-time chemical distributions in living systems. Specifically, SRS in the fingerprint region can resolve multiple chemicals in a…
Label-free imaging of rapidly moving, sub-diffraction sized structures has important applications in both biology and material science, as it removes the limitations associated with fluorescence tagging. However, unlabeled nanoscale…
The correlations of fluctuations are key to studying fundamental quantum physics and quantum many-body dynamics. They are also useful information for understanding and combating decoherence in quantum technology. Nonlinear spectroscopy and…
Spin noise spectroscopy (SNS) is a new method for studying magnetic resonance and spin dynamics based on measuring the Faraday rotation noise. In strong contrast with methods of nonlinear optics, the spectroscopy of spin noise is considered…
Absorption spectroscopy is routinely used to characterise chemical and biological samples. For the state-of-the-art in absorption spectroscopy, precision is theoretically limited by shot-noise due to the fundamental Poisson-distribution of…
Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…
One of the main characteristics of optical imaging systems is the spatial resolution, which is restricted by the diffraction limit to approximately half the wavelength of the incident light. Along with the recently developed classical…
Optomechanical systems provide a unique platform for observing quantum behavior of macroscopic objects. However, efforts towards realizing nonlinear behavior at the single photon level have been inhibited by the small size of the radiation…
Surface-enhanced Raman scattering (SERS) is a critical tool for chemical sensing and spectroscopy, and a key question is how to optimally design nanostructures for maximizing SERS. We present fundamental limits on spatially-averaged SERS…
We present multi-color imaging by stimulated Raman scattering (SRS) enabled by an ultrafast fiber-based light source with integrated amplitude modulation and frame-to-frame wavelength tuning. With a relative intensity noise level of -153.7…