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We present a novel approach to investigate the long-time stochastic dynamics of multi-dimensional classical systems, in contact with a heat-bath. When the potential energy landscape is rugged, the kinetics displays a decoupling of short and…

Soft Condensed Matter · Physics 2013-05-29 O. Corradini , P. Faccioli , H. Orland

We introduce a variational implementation of cluster perturbation theory (CPT) to address the dynamics of spin systems driven out of equilibrium. We benchmark the method with the quantum Ising model subject to a sudden quench of the…

Strongly Correlated Electrons · Physics 2016-12-07 Mohammad Zhian Asadzadeh , Michele Fabrizio , Enrico Arrigoni

Quantum computers hold great promise for arriving at exact simulations of nuclear dynamical processes (e.g., scattering and reactions) that are paramount to the study of nuclear matter at the limit of stability and to explaining the…

Heterogeneous nucleation is a process wherein extrinsic impurities facilitate freezing by lowering nucleation barriers and constitutes the dominant mechanism for crystallization in most systems. Classical nucleation theory (\textsc{Cnt})…

Soft Condensed Matter · Physics 2026-05-12 Fernanda Sulantay Vargas , Sarwar Hussain , Amir Haji-Akbari

Including quantum mechanical effects on the dynamics of nuclei in the condensed phase is challenging, because the complexity of exact methods grows exponentially with the number of quantum degrees of freedom. Efforts to circumvent these…

Chemical Physics · Physics 2015-06-23 Mariana Rossi , Hanchao Liu , Francesco Paesani , Joel Bowman , Michele Ceriotti

Small pre-structured seeds introduced into an undercooled fluid are known to increase the crystal nucleation rate by some orders of magnitude, if the structure of the seeds is commensurate with the bulk crystalline phase. The presence of…

Soft Condensed Matter · Physics 2017-10-06 S. Jungblut , C. Dellago

An essential parameter of the Classical Nucleation Theory (CNT) is the surface energy between a critical-size nucleus and the ambient phase, $\sigma$. In condensed matter, this parameter cannot be experimentally determined independently of…

Soft Condensed Matter · Physics 2019-03-13 Daniel R. Cassar

The classical nucleation theory (CNT) concept of a nucleus as a fragment of the bulk new phase fails for nanosized nuclei. An extension of CNT taking into account the properties of the transition region between coexisting bulk phases is…

Chemical Physics · Physics 2017-06-09 Nikolay V. Alekseechkin

The formation of inorganic cloud particles takes place in several atmospheric environments including those of warm, hot, rocky and gaseous exoplanets, brown dwarfs, and AGB stars. The cloud particle formation needs to be triggered by the…

Earth and Planetary Astrophysics · Physics 2022-12-07 J. P. Sindel , D. Gobrecht , Ch. Helling , L. Decin

A widely spread method of crystal preparation is to precipitate it from a supersaturated solution. In such a process, control of solution concentration is of paramount importance. Nucleation process, polymorph selection, and crystal habits…

Soft Condensed Matter · Physics 2019-07-10 Tarak Karmakar , Pablo M. Piaggi , Michele Parrinello

Magnetic molecules, modelled as finite-size spin systems, are test-beds for quantum phenomena and could constitute key elements in future spintronics devices, long-lasting nanoscale memories or noise-resilient quantum computing platforms.…

Quantum Physics · Physics 2021-03-16 A. Chiesa , F. Tacchino , M. Grossi , P. Santini , I. Tavernelli , D. Gerace , S. Carretta

We propose to test the concept of seeded vacuum decay in cosmology using an analogue gravity Bose-Einstein condensate system. The role of the nucleation seed is played by a vortex within the condensate. We present two complementary…

High Energy Physics - Theory · Physics 2019-10-02 Thomas P. Billam , Ruth Gregory , Florent Michel , Ian G. Moss

The behavior of nuclear matter is studied at low densities and temperatures using classical molecular dynamics with three different sets of potentials with different compressibility. Nuclear matter is found to arrange in crystalline…

Nuclear Theory · Physics 2013-05-13 C. O. Dorso , P. A. Giménez Molinelli , J. I. Nichols , J. A. López

Numerical simulations of clusters of galaxies provide a unique way to follow the dynamics of these systems. The models reveal many characteristics of the merging process of subclusters: shock structure and strength, temperature distribution…

Astrophysics · Physics 2007-05-23 Sabine Schindler

This paper presents an automatic method for data classification in nuclear physics experiments based on evolutionary computing and vector quantization. The major novelties of our approach are the fully automatic mechanism and the use of…

Nuclear Experiment · Physics 2020-12-02 D. Dell'Aquila , M. Russo

Vapour-liquid equilibria (VLE) and the influence of an inert carrier gas on homogeneous vapour to liquid nucleation are investigated by molecular simulation for quaternary mixtures of carbon dioxide, nitrogen, oxygen, and argon. Canonical…

Atmospheric and Oceanic Physics · Physics 2015-05-14 Martin Horsch , Zengyong Lin , Thorsten Windmann , Hans Hasse , Jadran Vrabec

In classical computational chemistry, the coupled-cluster ansatz is one of the most commonly used $ab~initio$ methods, which is critically limited by its non-unitary nature. The unitary modification as an ideal solution to the problem is,…

Quantum Physics · Physics 2017-03-01 Yangchao Shen , Xiang Zhang , Shuaining Zhang , Jing-Ning Zhang , Man-Hong Yung , Kihwan Kim

First-principles calculations of high-temperature spin dynamics in solids in the context of nuclear magnetic resonance (NMR) is a long-standing problem, whose conclusive solution can significantly advance the applications of NMR as a…

Statistical Mechanics · Physics 2018-12-19 Grigory A. Starkov , Boris V. Fine

We use the kinetic theory of nucleation to explore the properties of dust nucleation in sub-saturated vapors. Due to radiation losses, the sub-critical clusters have a smaller temperature compared to their vapor. This alters the dynamical…

Astrophysics · Physics 2015-05-13 Davide Lazzati

Accurate estimate of nucleation rate is crucial for the study of ice nucleation and ice-promoting/anti-freeze strategies. Within the framework of Classical Nucleation Theory (CNT), the estimate of ice nucleation rate is very sensitive to…

Soft Condensed Matter · Physics 2021-07-07 Chaohong Wang , Hao Wang , Jianyang Wu , Zhisen Zhang