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The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…

We have developed a hyperspectral imaging scheme that involves a combination of dual-comb spectroscopy and Hadamard-transform-based single-pixel imaging. The scheme enables us to obtain 12,000 hyperspectral images of amplitude and phase at…

We experimentally demonstrate four-wave-mixing spectroscopy using frequency combs. The experiment uses a geometry where excitation pulses and four-wave-mixing signals generated by a sample co-propagate. We separate them in the radio…

Optics · Physics 2017-08-02 Bachana Lomsadze , Steven T. Cundiff

We propose a linear optical quantum computation scheme using time-frequency degree of freedom. In this scheme, a qubit is encoded in single-photon frequency combs, and manipulation of the qubits is performed using time-resolving detectors,…

Quantum Physics · Physics 2023-06-13 Tomohiro Yamazaki , Tomoaki Arizono , Toshiki Kobayashi , Rikizo Ikuta , Takashi Yamamoto

A high-resolution broad-spectral-bandwidth spectrometer on a chip would create new opportunities for gas-phase molecular fingerprinting, especially in environmental sensing. A resolution high enough to observe transitions at atmospheric…

Optical frequency combs based on mode-locked lasers have revolutionised the field of metrology and precision spectroscopy by providing precisely calibrated optical frequencies and coherent pulse trains. Amplification of the pulsed output…

Atomic Physics · Physics 2014-01-17 Jonas Morgenweg , Itan Barmes , Kjeld S. E. Eikema

Electro-optic frequency combs were employed to rapidly interrogate an optomechanical sensor, demonstrating spectral resolution substantially exceeding that possible with a mode-locked frequency comb. Frequency combs were generated using an…

Optics · Physics 2022-04-01 D. A. Long , B. J. Reschovsky , F. Zhou , Y. Bao , T. W. LeBrun , J. J. Gorman

Coherent Raman microscopy provide label-free imaging by interrogating the intrinsic vibration of biomolecules. Nevertheless, trade-off between high chemical-specificity and high imaging-speed currently exists in transition from spectroscopy…

Optics · Physics 2017-10-11 Kun Chen , Tao Wu , Tao Chen , Tian Zhou , Haoyun Wei , Yan Li

A four-wave-mixing, frequency-comb-based, hyperspectral imaging technique that is spectrally precise, potentially rapid, and can in principle be applied to any material, is demonstrated in a near-diffraction-limited microscopy application.

Optics · Physics 2021-07-21 Brad C. Smith , Bachana Lomsadze , Steven T. Cundiff

Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…

Optics · Physics 2016-09-13 Xin Zhao , Guoqing Hu , Bofeng Zhao , Cui Li , Yingling Pan , Ya Liu , Takeshi Yasui , Zheng Zheng

In this Letter, we propose a new approach to process high-dimensional quantum information encoded in a photon frequency domain. In contrast to previous approaches based on nonlinear optical processes, no active control of photon energy is…

Quantum Physics · Physics 2020-07-16 Chaohan Cui , Kaushik P. Seshadreesan , Saikat Guha , Linran Fan

The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…

Optics · Physics 2023-07-19 Vicente Duran , Santiago Tainta , Victor Torres-Company

Optical frequency combs, coherent light sources that connect optical frequencies with microwave oscillations, have become the enabling tool for precision spectroscopy, optical clockwork and attosecond physics over the past decades. Current…

Optics · Physics 2017-03-21 S. -W. Huang , J. Yang , M. Yu , B. H. McGuyer , D. -L. Kwong , T. Zelevinsky , C. W. Wong

Miniaturized spectrometry system is playing an essential role for materials analysis in the development of in-situ or portable sensing platforms across research and industry. However, there unavoidably exists trade-offs between the…

Optical frequency combs have attracted attention as optical frequency rulers due to their tooth-like discrete spectra together with their inherent mode-locking nature and phase-locking control to a frequency standard. Based on this concept,…

Frequency combs have revolutionized optical frequency metrology, allowing one to determine highly accurate transition frequencies of a wealth of molecular species. Despite a recognized scientific interest, these progresses have only…

To meet the challenges of high-resolution molecular spectroscopy, increasingly sophisticated spectroscopic techniques were developed. For a long time FTIR and laser-based spectroscopies were used for these studies. The recent development of…

We demonstrate a new technique for the experimental measurement of the spectral coherence of microresonator optical frequency combs. Specifically, we use a spectral interference method, typically used in the context of supercontinuum…

Realizing multiply resonant photonic crystal cavities with large free spectral range is key to achieve integrated devices with highly efficient nonlinear response, such as frequency conversion, four-wave mixing, and parametric oscillation.…

The optical microresonator-based frequency comb (microcomb) provides a versatile platform for nonlinear physics studies and has wide applications ranging from metrology to spectroscopy. Deterministic quantum regime is an unexplored aspect…

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