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Spectroscopy is the basic tool for studying molecular physics and realizing bio-chemical sensing. However, it is challenging to realize sub-femtometer resolution spectroscopy over broad bandwidth. In this paper, broadband and…

Optics · Physics 2022-12-19 Bingxin Xu , Yangyang Wan , Xinyu Fan , Zuyuan He

Molecular fingerprinting through absorption spectroscopy is a powerful analytical method. Wide spectral ranges are explored with Doppler-limited resolution. Fast data acquisition, accurate measurements of frequency, intensity, and line…

Optics · Physics 2008-08-20 Julien Mandon , Guy Guelachvili , Nathalie Picqué

Optical frequency combs consist of equally spaced discrete optical frequency components and are essential tools for optical communications and for precision metrology, timing and spectroscopy. To date, wide-spanning combs are most often…

We report the upgrade and operation of a frequency-comb-assisted high-resolution mid-infrared molecular spectrometer allowing us to combine high spectral purity, SI-traceability, wide tunability and high sensitivity. An optical frequency…

Optical frequency combs generated by multiple four-wave mixing of two stabilized single-frequency lasers in optical fibers are proposed for use as high precision frequency markers, calibration of astrophysical spectrometers and metrology.…

Optics · Physics 2009-11-13 Flavio C. Cruz

Dual-comb spectroscopy can provide broad spectral bandwidth and high spectral resolution in a short acquisition time, enabling time-resolved measurements. Specifically, spectroscopy in the mid-infrared wavelength range is of particular…

We have developed a dispersive spectrometer using a compact immersion grating for direct frequency comb spectroscopy in the long-wave infrared region of 8-10 {\mu}m. A frequency resolution of 463 MHz is achieved, which is the highest…

Instrumentation and Detectors · Physics 2019-02-20 Kana Iwakuni , Thinh Q. Bui , Justin Niedermeyer , Takashi Sukegawa , Jun Ye

Dual Comb Spectroscopy proved its versatile capabilities in molecular fingerprinting in different spectral regions, but not yet in the ultraviolet (UV). Unlocking this spectral window would expand fingerprinting to the electronic energy…

Supersonic engine development requires accurate and detailed measurements of fluidic and thermodynamic parameters to optimize engine designs and benchmark computational fluid dynamic (CFD) simulations. Here, we demonstrate that dual…

We show that the use of an optical frequency comb probe leads to dramatically improved bandwidth (as high as 12+/-1 MHz) for the detection of modulated radio frequencies in Rydberg atom-based electrometry.

Mechanical frequency combs are poised to bring the applications and utility of optical frequency combs into the mechanical domain. So far, their main challenge has been strict requirements on drive frequencies and power, which complicate…

Quantum cascade laser (QCL) frequency combs have revolutionized mid-infrared (MIR) spectroscopy by their high brightness and fast temporal resolution, and are a promising technology for fully-integrated and cost-effective sensors. As for…

Broadband and high-resolution spectroscopy in the visible and ultraviolet is central to advances in multiple fields, including fundamental quantum physics, biology, atmospheric science and astronomy. Traditionally, these measurements are…

Detection of individual molecules is the ultimate goal of any chemical sensor. In the case of gas detection, such resolution has been achieved in advanced nanoscale electronic solid-state sensors, but it has not been possible so far in…

Mesoscale and Nanoscale Physics · Physics 2021-04-09 Ning An , Teng Tan , Zheng Peng , Chenye Qin , Zhongye Yuan , Lei Bi , Changrui Liao , Yiping Wang , Yunjiang Rao , Giancarlo Soavi , Baicheng Yao

Mid-infrared dual-comb spectroscopy has the potential to supplant conventional high-resolution Fourier transform spectroscopy in applications that require high resolution, accuracy, signal-to-noise ratio, and speed. Until now, dual-comb…

Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb…

The advent of optical frequency standards with ultimate uncertainties in the low 1x10$^{-18}$ requires femtosecond frequency combs to support a similar level of resolution in the spectral transfer and the computation of optical frequency…

Instrumentation and Detectors · Physics 2022-05-31 Matias Risaro , Paolo Savio , Marco Pizzocaro , Filippo Levi , Davide Calonico , Cecilia Clivati

High speed optical telecommunication is enabled by wavelength division multiplexing, whereby hundreds of individually stabilized lasers encode the information within a single mode optical fiber. In the seek for larger bandwidth the optical…

We describe a coherent mid-infrared continuum source with 700 cm-1 usable bandwidth, readily tuned within 600 - 2500 cm-1 (4 - 17 \mum) and thus covering much of the infrared "fingerprint" molecular vibration region. It is based on…

Quantum Physics · Physics 2015-06-04 Fritz Keilmann , Sergiu Amarie

We introduce a novel laser-scanning optical microscopy technique that employs optical-frequency-comb (OFC) lasers. This method facilitates multimodal spectroscopic imaging by analyzing interferograms produced via a dual-comb spectroscopic…

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